Novel L-DOPA-Derived Poly(ester amide)s: Monomers, Polymers, and the First L-DOPA-Functionalized Biobased Adhesive Tape
The synthesis, characterization, and testing of a range of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optim...
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| Veröffentlicht in: | Macromolecular rapid communications. 2014-01, Vol.35 (1), p.71-76 |
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| creator | Manolakis, Ioannis Noordover, Bart A. J. Vendamme, Richard Eevers, Walter |
| description | The synthesis, characterization, and testing of a range of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased L‐DOPA‐containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)‐based materials.
A family of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is the subject of this work. The developed synthetic platform allows for facile synthesis, targets a wide range of structures and provides good control over the molecular and thermal properties of the resulting polymers. A particular composition containing L‐DOPA and fatty acid dimer residues is tested in terms of its adhesive performance with promising results. |
| doi_str_mv | 10.1002/marc.201300750 |
| format | Article |
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A family of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is the subject of this work. The developed synthetic platform allows for facile synthesis, targets a wide range of structures and provides good control over the molecular and thermal properties of the resulting polymers. A particular composition containing L‐DOPA and fatty acid dimer residues is tested in terms of its adhesive performance with promising results.</description><identifier>ISSN: 1022-1336</identifier><identifier>EISSN: 1521-3927</identifier><identifier>DOI: 10.1002/marc.201300750</identifier><identifier>PMID: 24265232</identifier><language>eng</language><publisher>Weinheim: Blackwell Publishing Ltd</publisher><subject>adhesive properties ; Adhesives ; Amides - chemistry ; Applied sciences ; bio-inspired polymers ; Exact sciences and technology ; L-DOPA ; Levodopa - chemistry ; Magnetic Resonance Spectroscopy ; Organic polymers ; Physicochemistry of polymers ; poly(ester amide)s ; polycondensation ; Polyesters - chemistry ; Polymers ; Polymers with particular properties ; Preparation, kinetics, thermodynamics, mechanism and catalysts ; Tissue Adhesives</subject><ispartof>Macromolecular rapid communications., 2014-01, Vol.35 (1), p.71-76</ispartof><rights>2013 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim</rights><rights>2015 INIST-CNRS</rights><rights>2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.</rights><rights>Copyright 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c4740-a97e01e6f4c707795acd2709a3dda5f244cacaf01475f112c1ac51a0834e2a883</citedby><cites>FETCH-LOGICAL-c4740-a97e01e6f4c707795acd2709a3dda5f244cacaf01475f112c1ac51a0834e2a883</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fmarc.201300750$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fmarc.201300750$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,4010,27900,27901,27902,45550,45551</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=28068121$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24265232$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Manolakis, Ioannis</creatorcontrib><creatorcontrib>Noordover, Bart A. J.</creatorcontrib><creatorcontrib>Vendamme, Richard</creatorcontrib><creatorcontrib>Eevers, Walter</creatorcontrib><title>Novel L-DOPA-Derived Poly(ester amide)s: Monomers, Polymers, and the First L-DOPA-Functionalized Biobased Adhesive Tape</title><title>Macromolecular rapid communications.</title><addtitle>Macromol. Rapid Commun</addtitle><description>The synthesis, characterization, and testing of a range of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is presented, using a widely applicable, straightforward chemistry. A model system is used to study and establish the monomer and polymer synthetic protocols, and to provide a set of optimum reaction conditions. It is further shown that fully biobased L‐DOPA‐containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)‐based materials.
A family of novel bio‐inspired L‐DOPA‐derived poly(ester amide)s is the subject of this work. The developed synthetic platform allows for facile synthesis, targets a wide range of structures and provides good control over the molecular and thermal properties of the resulting polymers. A particular composition containing L‐DOPA and fatty acid dimer residues is tested in terms of its adhesive performance with promising results.</description><subject>adhesive properties</subject><subject>Adhesives</subject><subject>Amides - chemistry</subject><subject>Applied sciences</subject><subject>bio-inspired polymers</subject><subject>Exact sciences and technology</subject><subject>L-DOPA</subject><subject>Levodopa - chemistry</subject><subject>Magnetic Resonance Spectroscopy</subject><subject>Organic polymers</subject><subject>Physicochemistry of polymers</subject><subject>poly(ester amide)s</subject><subject>polycondensation</subject><subject>Polyesters - chemistry</subject><subject>Polymers</subject><subject>Polymers with particular properties</subject><subject>Preparation, kinetics, thermodynamics, mechanism and catalysts</subject><subject>Tissue Adhesives</subject><issn>1022-1336</issn><issn>1521-3927</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqNkd1v0zAUxSMEYh_wyiOKhJA2iZTrrzjhrXR0ILqtQgUerTvH0bwlcbGbjfLX45KuIF5AfvCV_Dvn-t6TJM8IjAgAfd2i1yMKhAFIAQ-SfSIoyVhJ5cNYA6UZYSzfSw5CuAaAggN9nOxRTnNBGd1P7s7drWnSWXZyMR9nJ8bbW1Olc9esj0xYGZ9iaytzHN6kZ65zrfHh1a_XocKuSldXJp1aH1b3JtO-0yvrOmzsj-j11rpLDLEYV1cmRPt0gUvzJHlUYxPM0-19mHyevltM3mezi9MPk_Es01xyyLCUBojJa64lSFkK1BWVUCKrKhQ15VyjxhoIl6ImhGqCWhCEgnFDsSjYYXI0-C69-9bHkVRrgzZNg51xfVCEl5zFDUH5P2jccRFPRF_8hV673seJN5RkgpXAZKRGA6W9C8GbWi29jYGtFQG1SU9t0lO79KLg-da2v2xNtcPv44rAyy2AQWNTe-y0Db-5AvKCUBK5cuDubGPW_2irzsafJn9-Ihu0Nub_fadFf6NyyaRQX89PFYeP5Avkc7VgPwEabr8x</recordid><startdate>201401</startdate><enddate>201401</enddate><creator>Manolakis, Ioannis</creator><creator>Noordover, Bart A. 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J.</creatorcontrib><creatorcontrib>Vendamme, Richard</creatorcontrib><creatorcontrib>Eevers, Walter</creatorcontrib><collection>Istex</collection><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>ProQuest Computer Science Collection</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Macromolecular rapid communications.</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Manolakis, Ioannis</au><au>Noordover, Bart A. 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It is further shown that fully biobased L‐DOPA‐containing adhesive tapes can be fabricated, which are positively evaluated in terms of their adhesive properties. The newly developed synthetic protocol constitutes a versatile platform for accessing and tailoring a plethora of relevant structures, including a variety of potentially biocompatible poly(ethylene glycol)‐based materials.
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| subjects | adhesive properties Adhesives Amides - chemistry Applied sciences bio-inspired polymers Exact sciences and technology L-DOPA Levodopa - chemistry Magnetic Resonance Spectroscopy Organic polymers Physicochemistry of polymers poly(ester amide)s polycondensation Polyesters - chemistry Polymers Polymers with particular properties Preparation, kinetics, thermodynamics, mechanism and catalysts Tissue Adhesives |
| title | Novel L-DOPA-Derived Poly(ester amide)s: Monomers, Polymers, and the First L-DOPA-Functionalized Biobased Adhesive Tape |
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