Halogenated organic pollutants in particulate matters emitted during recycling of waste printed circuit boards in a typical e-waste workshop of Southern China
•Levels and patterns of PBDEs, PCDD/Fs and PBDD/Fs associated with PM were presented.•BDE-47, -99, and -209 were the dominant PBDE congeners.•Concentrations of PBDD/Fs were higher than PCDD/Fs.•E-waste recycling represents a strong source of PBDEs and dioxins. Air particle samples collected from a t...
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| Veröffentlicht in: | Chemosphere (Oxford) 2014-01, Vol.94, p.143-150 |
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| creator | Ren, Zhaofang Xiao, Xiao Chen, Deyi Bi, Xinhui Huang, Bo Liu, Ming Hu, Jianfang Peng, Ping’an Sheng, Guoying Fu, Jiamo |
| description | •Levels and patterns of PBDEs, PCDD/Fs and PBDD/Fs associated with PM were presented.•BDE-47, -99, and -209 were the dominant PBDE congeners.•Concentrations of PBDD/Fs were higher than PCDD/Fs.•E-waste recycling represents a strong source of PBDEs and dioxins.
Air particle samples collected from a typical workshop of Southern China engaged in recycling waste printed circuit boards were analyzed for PBDEs, PCDD/Fs, and PBDD/Fs. The concentrations and profiles of these compounds were presented. Concentrations of ∑PBDEs, ∑PCDD/Fs and ∑PBDD/Fs in this workshop were 948ngm−3, 317pgm−3 (14.5pg WHO-TEQm−3) and 481pgm−3 (91.3pg I-TEQm−3), respectively. BDEs-47, -99, and -209 were the dominant PBDE congeners, and the relatively high levels of octa- and nona-BDEs might be generated from the degradation of BDE-209. The levels of 2,3,7,8-PCDD/Fs and 2,3,7,8-PBDD/Fs were much higher than those in the atmospheric environment, and concentrations of PBDD/Fs were higher than those of PCDD/Fs. These findings suggest that the primitive recycling method represents a strong source of halogenated organic pollutants to the ambient atmosphere of an e-waste recycling locale. |
| doi_str_mv | 10.1016/j.chemosphere.2013.09.065 |
| format | Article |
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Air particle samples collected from a typical workshop of Southern China engaged in recycling waste printed circuit boards were analyzed for PBDEs, PCDD/Fs, and PBDD/Fs. The concentrations and profiles of these compounds were presented. Concentrations of ∑PBDEs, ∑PCDD/Fs and ∑PBDD/Fs in this workshop were 948ngm−3, 317pgm−3 (14.5pg WHO-TEQm−3) and 481pgm−3 (91.3pg I-TEQm−3), respectively. BDEs-47, -99, and -209 were the dominant PBDE congeners, and the relatively high levels of octa- and nona-BDEs might be generated from the degradation of BDE-209. The levels of 2,3,7,8-PCDD/Fs and 2,3,7,8-PBDD/Fs were much higher than those in the atmospheric environment, and concentrations of PBDD/Fs were higher than those of PCDD/Fs. These findings suggest that the primitive recycling method represents a strong source of halogenated organic pollutants to the ambient atmosphere of an e-waste recycling locale.</description><identifier>ISSN: 0045-6535</identifier><identifier>EISSN: 1879-1298</identifier><identifier>DOI: 10.1016/j.chemosphere.2013.09.065</identifier><identifier>PMID: 24367823</identifier><identifier>CODEN: CMSHAF</identifier><language>eng</language><publisher>Kidlington: Elsevier Ltd</publisher><subject>Air Pollutants - analysis ; Air Pollutants, Occupational - analysis ; Applied sciences ; Atmosphere - chemistry ; Atmospheric pollution ; China ; Dioxins ; Dispersed sources and other ; Electronic Waste ; Exact sciences and technology ; Halogenated Diphenyl Ethers - analysis ; Particulate Matter - analysis ; PBDEs ; Pollution ; Pollution sources. Measurement results ; POPs ; Printed circuit boards ; Recycling ; Waste Management</subject><ispartof>Chemosphere (Oxford), 2014-01, Vol.94, p.143-150</ispartof><rights>2013 Elsevier Ltd</rights><rights>2015 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c407t-2cae3899cf0231a027560e36e3237ea089906daca54e4062907c6fc0a0f3340f3</citedby><cites>FETCH-LOGICAL-c407t-2cae3899cf0231a027560e36e3237ea089906daca54e4062907c6fc0a0f3340f3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.chemosphere.2013.09.065$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3548,4022,27921,27922,27923,45993</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=28079103$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24367823$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Ren, Zhaofang</creatorcontrib><creatorcontrib>Xiao, Xiao</creatorcontrib><creatorcontrib>Chen, Deyi</creatorcontrib><creatorcontrib>Bi, Xinhui</creatorcontrib><creatorcontrib>Huang, Bo</creatorcontrib><creatorcontrib>Liu, Ming</creatorcontrib><creatorcontrib>Hu, Jianfang</creatorcontrib><creatorcontrib>Peng, Ping’an</creatorcontrib><creatorcontrib>Sheng, Guoying</creatorcontrib><creatorcontrib>Fu, Jiamo</creatorcontrib><title>Halogenated organic pollutants in particulate matters emitted during recycling of waste printed circuit boards in a typical e-waste workshop of Southern China</title><title>Chemosphere (Oxford)</title><addtitle>Chemosphere</addtitle><description>•Levels and patterns of PBDEs, PCDD/Fs and PBDD/Fs associated with PM were presented.•BDE-47, -99, and -209 were the dominant PBDE congeners.•Concentrations of PBDD/Fs were higher than PCDD/Fs.•E-waste recycling represents a strong source of PBDEs and dioxins.
Air particle samples collected from a typical workshop of Southern China engaged in recycling waste printed circuit boards were analyzed for PBDEs, PCDD/Fs, and PBDD/Fs. The concentrations and profiles of these compounds were presented. Concentrations of ∑PBDEs, ∑PCDD/Fs and ∑PBDD/Fs in this workshop were 948ngm−3, 317pgm−3 (14.5pg WHO-TEQm−3) and 481pgm−3 (91.3pg I-TEQm−3), respectively. BDEs-47, -99, and -209 were the dominant PBDE congeners, and the relatively high levels of octa- and nona-BDEs might be generated from the degradation of BDE-209. The levels of 2,3,7,8-PCDD/Fs and 2,3,7,8-PBDD/Fs were much higher than those in the atmospheric environment, and concentrations of PBDD/Fs were higher than those of PCDD/Fs. These findings suggest that the primitive recycling method represents a strong source of halogenated organic pollutants to the ambient atmosphere of an e-waste recycling locale.</description><subject>Air Pollutants - analysis</subject><subject>Air Pollutants, Occupational - analysis</subject><subject>Applied sciences</subject><subject>Atmosphere - chemistry</subject><subject>Atmospheric pollution</subject><subject>China</subject><subject>Dioxins</subject><subject>Dispersed sources and other</subject><subject>Electronic Waste</subject><subject>Exact sciences and technology</subject><subject>Halogenated Diphenyl Ethers - analysis</subject><subject>Particulate Matter - analysis</subject><subject>PBDEs</subject><subject>Pollution</subject><subject>Pollution sources. Measurement results</subject><subject>POPs</subject><subject>Printed circuit boards</subject><subject>Recycling</subject><subject>Waste Management</subject><issn>0045-6535</issn><issn>1879-1298</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqNkc-O0zAQhyMEYsvCKyBzQOKSMo4TJz6iCliklTgAZ2vWmbQuiR1sh1VfhmfFoeXPkYttab7P9syvKF5w2HLg8vVxaw40-TgfKNC2Ai62oLYgmwfFhnetKnmluofFBqBuStmI5qp4EuMRIMuNelxcVbWQbVeJTfHjBke_J4eJeubDHp01bPbjuCR0KTLr2IwhWbOMGWETpkQhMppsWo1-CdbtWSBzMuN68gO7x5jJORdWwthgFpvYncfQ_7oPWTrN1uDIqDyz9z58jQc_r_Ynv6TclmO7g3X4tHg04Bjp2WW_Lr68e_t5d1Pefnz_YffmtjQ1tKmsDJLolDIDVIIjVG0jgYQkUYmWEHIJZI8Gm5pqkJWC1sjBAMIgRJ2X6-LV-d45-G8LxaQnGw2NIzryS9S8zoqQqmszqs6oCT7GQIPOrU4YTpqDXuPRR_1PPHqNR4PSOZ7sPr88s9xN1P8xf-eRgZcXAGOe0BDQGRv_ch20isPK7c4c5aF8txR0NJacod7mLJLuvf2P7_wExKu3ug</recordid><startdate>201401</startdate><enddate>201401</enddate><creator>Ren, Zhaofang</creator><creator>Xiao, Xiao</creator><creator>Chen, Deyi</creator><creator>Bi, Xinhui</creator><creator>Huang, Bo</creator><creator>Liu, Ming</creator><creator>Hu, Jianfang</creator><creator>Peng, Ping’an</creator><creator>Sheng, Guoying</creator><creator>Fu, Jiamo</creator><general>Elsevier Ltd</general><general>Elsevier</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope></search><sort><creationdate>201401</creationdate><title>Halogenated organic pollutants in particulate matters emitted during recycling of waste printed circuit boards in a typical e-waste workshop of Southern China</title><author>Ren, Zhaofang ; Xiao, Xiao ; Chen, Deyi ; Bi, Xinhui ; Huang, Bo ; Liu, Ming ; Hu, Jianfang ; Peng, Ping’an ; Sheng, Guoying ; Fu, Jiamo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c407t-2cae3899cf0231a027560e36e3237ea089906daca54e4062907c6fc0a0f3340f3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Air Pollutants - analysis</topic><topic>Air Pollutants, Occupational - analysis</topic><topic>Applied sciences</topic><topic>Atmosphere - chemistry</topic><topic>Atmospheric pollution</topic><topic>China</topic><topic>Dioxins</topic><topic>Dispersed sources and other</topic><topic>Electronic Waste</topic><topic>Exact sciences and technology</topic><topic>Halogenated Diphenyl Ethers - analysis</topic><topic>Particulate Matter - analysis</topic><topic>PBDEs</topic><topic>Pollution</topic><topic>Pollution sources. Measurement results</topic><topic>POPs</topic><topic>Printed circuit boards</topic><topic>Recycling</topic><topic>Waste Management</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ren, Zhaofang</creatorcontrib><creatorcontrib>Xiao, Xiao</creatorcontrib><creatorcontrib>Chen, Deyi</creatorcontrib><creatorcontrib>Bi, Xinhui</creatorcontrib><creatorcontrib>Huang, Bo</creatorcontrib><creatorcontrib>Liu, Ming</creatorcontrib><creatorcontrib>Hu, Jianfang</creatorcontrib><creatorcontrib>Peng, Ping’an</creatorcontrib><creatorcontrib>Sheng, Guoying</creatorcontrib><creatorcontrib>Fu, Jiamo</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>Chemosphere (Oxford)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ren, Zhaofang</au><au>Xiao, Xiao</au><au>Chen, Deyi</au><au>Bi, Xinhui</au><au>Huang, Bo</au><au>Liu, Ming</au><au>Hu, Jianfang</au><au>Peng, Ping’an</au><au>Sheng, Guoying</au><au>Fu, Jiamo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Halogenated organic pollutants in particulate matters emitted during recycling of waste printed circuit boards in a typical e-waste workshop of Southern China</atitle><jtitle>Chemosphere (Oxford)</jtitle><addtitle>Chemosphere</addtitle><date>2014-01</date><risdate>2014</risdate><volume>94</volume><spage>143</spage><epage>150</epage><pages>143-150</pages><issn>0045-6535</issn><eissn>1879-1298</eissn><coden>CMSHAF</coden><abstract>•Levels and patterns of PBDEs, PCDD/Fs and PBDD/Fs associated with PM were presented.•BDE-47, -99, and -209 were the dominant PBDE congeners.•Concentrations of PBDD/Fs were higher than PCDD/Fs.•E-waste recycling represents a strong source of PBDEs and dioxins.
Air particle samples collected from a typical workshop of Southern China engaged in recycling waste printed circuit boards were analyzed for PBDEs, PCDD/Fs, and PBDD/Fs. The concentrations and profiles of these compounds were presented. Concentrations of ∑PBDEs, ∑PCDD/Fs and ∑PBDD/Fs in this workshop were 948ngm−3, 317pgm−3 (14.5pg WHO-TEQm−3) and 481pgm−3 (91.3pg I-TEQm−3), respectively. BDEs-47, -99, and -209 were the dominant PBDE congeners, and the relatively high levels of octa- and nona-BDEs might be generated from the degradation of BDE-209. The levels of 2,3,7,8-PCDD/Fs and 2,3,7,8-PBDD/Fs were much higher than those in the atmospheric environment, and concentrations of PBDD/Fs were higher than those of PCDD/Fs. These findings suggest that the primitive recycling method represents a strong source of halogenated organic pollutants to the ambient atmosphere of an e-waste recycling locale.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><pmid>24367823</pmid><doi>10.1016/j.chemosphere.2013.09.065</doi><tpages>8</tpages></addata></record> |
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| ispartof | Chemosphere (Oxford), 2014-01, Vol.94, p.143-150 |
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| subjects | Air Pollutants - analysis Air Pollutants, Occupational - analysis Applied sciences Atmosphere - chemistry Atmospheric pollution China Dioxins Dispersed sources and other Electronic Waste Exact sciences and technology Halogenated Diphenyl Ethers - analysis Particulate Matter - analysis PBDEs Pollution Pollution sources. Measurement results POPs Printed circuit boards Recycling Waste Management |
| title | Halogenated organic pollutants in particulate matters emitted during recycling of waste printed circuit boards in a typical e-waste workshop of Southern China |
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