AOX removal from industrial wastewaters using advanced oxidation processes: assessment of a combined chemical-biological oxidation
In this paper, the abatement of adsorbable halogenated organic compounds (AOX) from an industrial wastewater containing relatively high chloride concentrations by a combined chemical and biological oxidation is assessed. For chemical oxidation, the O(3)/UV, H(2)O(2)/UV and photo-Fenton processes are...
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| Veröffentlicht in: | Water science and technology 2013-01, Vol.68 (9), p.2048-2054 |
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| creator | LUYTEN, J SNIEGOWSKI, K VAN EYCK, K MAERTENS, D TIMMERMANS, S LIERS, Sven BRAEKEN, L |
| description | In this paper, the abatement of adsorbable halogenated organic compounds (AOX) from an industrial wastewater containing relatively high chloride concentrations by a combined chemical and biological oxidation is assessed. For chemical oxidation, the O(3)/UV, H(2)O(2)/UV and photo-Fenton processes are evaluated on pilot scale. Biological oxidation is simulated in a 4 h respirometry experiment with periodic aeration. The results show that a selective degradation of AOX with respect to the matrix compounds (expressed as chemical oxygen demand) could be achieved. For O(3)/UV, lowering the ratio of O(3) dosage to UV intensity leads to a better selectivity for AOX. During O(3)-based experiments, the AOX removal is generally less than during the H(2)O(2)-based experiments. However, after biological oxidation, the AOX levels are comparable. For H(2)O(2)/UV, optimal operating parameters for UV and H(2)O(2) dosage are next determined in a second run with another wastewater sample. |
| doi_str_mv | 10.2166/wst.2013.459 |
| format | Article |
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For chemical oxidation, the O(3)/UV, H(2)O(2)/UV and photo-Fenton processes are evaluated on pilot scale. Biological oxidation is simulated in a 4 h respirometry experiment with periodic aeration. The results show that a selective degradation of AOX with respect to the matrix compounds (expressed as chemical oxygen demand) could be achieved. For O(3)/UV, lowering the ratio of O(3) dosage to UV intensity leads to a better selectivity for AOX. During O(3)-based experiments, the AOX removal is generally less than during the H(2)O(2)-based experiments. However, after biological oxidation, the AOX levels are comparable. For H(2)O(2)/UV, optimal operating parameters for UV and H(2)O(2) dosage are next determined in a second run with another wastewater sample.</description><identifier>ISSN: 0273-1223</identifier><identifier>EISSN: 1996-9732</identifier><identifier>DOI: 10.2166/wst.2013.459</identifier><identifier>PMID: 24225107</identifier><identifier>CODEN: WSTED4</identifier><language>eng</language><publisher>London: International Water Association</publisher><subject>Aeration ; Analysis methods ; Applied sciences ; Biodegradation, Environmental ; Biological oxidation ; Biological Oxygen Demand Analysis ; Chemical compounds ; Chemical oxygen demand ; Dosage ; Exact sciences and technology ; General purification processes ; Halogenation ; Hydrogen peroxide ; Hydrogen Peroxide - chemistry ; Hydrogen-Ion Concentration ; Industrial wastes ; Industrial wastewater ; Iron - chemistry ; Natural water pollution ; Organic Chemicals - chemistry ; Organic compounds ; Oxidants - chemistry ; Oxidation ; Oxidation-Reduction ; Ozone - chemistry ; Pollution ; Pulp mill effluents ; Removal ; Respirometry ; Scale (corrosion) ; Selectivity ; Ultraviolet radiation ; Ultraviolet Rays ; Waste Disposal, Fluid - methods ; Wastewater ; Wastewaters ; Water Pollutants, Chemical - chemistry ; Water Pollution, Chemical - prevention & control ; Water treatment and pollution</subject><ispartof>Water science and technology, 2013-01, Vol.68 (9), p.2048-2054</ispartof><rights>2015 INIST-CNRS</rights><rights>Copyright IWA Publishing Nov 2013</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c387t-6cdb9b7cf504ad9c63842acc434232c98de810cd4a78c64f1265a1372c117bca3</citedby></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=28200222$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24225107$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>LUYTEN, J</creatorcontrib><creatorcontrib>SNIEGOWSKI, K</creatorcontrib><creatorcontrib>VAN EYCK, K</creatorcontrib><creatorcontrib>MAERTENS, D</creatorcontrib><creatorcontrib>TIMMERMANS, S</creatorcontrib><creatorcontrib>LIERS, Sven</creatorcontrib><creatorcontrib>BRAEKEN, L</creatorcontrib><title>AOX removal from industrial wastewaters using advanced oxidation processes: assessment of a combined chemical-biological oxidation</title><title>Water science and technology</title><addtitle>Water Sci Technol</addtitle><description>In this paper, the abatement of adsorbable halogenated organic compounds (AOX) from an industrial wastewater containing relatively high chloride concentrations by a combined chemical and biological oxidation is assessed. For chemical oxidation, the O(3)/UV, H(2)O(2)/UV and photo-Fenton processes are evaluated on pilot scale. Biological oxidation is simulated in a 4 h respirometry experiment with periodic aeration. The results show that a selective degradation of AOX with respect to the matrix compounds (expressed as chemical oxygen demand) could be achieved. For O(3)/UV, lowering the ratio of O(3) dosage to UV intensity leads to a better selectivity for AOX. During O(3)-based experiments, the AOX removal is generally less than during the H(2)O(2)-based experiments. However, after biological oxidation, the AOX levels are comparable. For H(2)O(2)/UV, optimal operating parameters for UV and H(2)O(2) dosage are next determined in a second run with another wastewater sample.</description><subject>Aeration</subject><subject>Analysis methods</subject><subject>Applied sciences</subject><subject>Biodegradation, Environmental</subject><subject>Biological oxidation</subject><subject>Biological Oxygen Demand Analysis</subject><subject>Chemical compounds</subject><subject>Chemical oxygen demand</subject><subject>Dosage</subject><subject>Exact sciences and technology</subject><subject>General purification processes</subject><subject>Halogenation</subject><subject>Hydrogen peroxide</subject><subject>Hydrogen Peroxide - chemistry</subject><subject>Hydrogen-Ion Concentration</subject><subject>Industrial wastes</subject><subject>Industrial wastewater</subject><subject>Iron - chemistry</subject><subject>Natural water pollution</subject><subject>Organic Chemicals - chemistry</subject><subject>Organic compounds</subject><subject>Oxidants - chemistry</subject><subject>Oxidation</subject><subject>Oxidation-Reduction</subject><subject>Ozone - chemistry</subject><subject>Pollution</subject><subject>Pulp mill effluents</subject><subject>Removal</subject><subject>Respirometry</subject><subject>Scale (corrosion)</subject><subject>Selectivity</subject><subject>Ultraviolet radiation</subject><subject>Ultraviolet Rays</subject><subject>Waste Disposal, Fluid - methods</subject><subject>Wastewater</subject><subject>Wastewaters</subject><subject>Water Pollutants, Chemical - chemistry</subject><subject>Water Pollution, Chemical - prevention & control</subject><subject>Water treatment and pollution</subject><issn>0273-1223</issn><issn>1996-9732</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2013</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNpdkU2LFDEQhoMo7rh68ywBETzYY74m6fa2LH7Bwl4UvIXqSnrN0t1ZU907evWXm2FHFzxVBR7eFO_D2HMptkpa-3ZPy1YJqbdm1z1gG9l1tumcVg_ZRiinG6mUPmFPiK6FEE4b8ZidKKPUTgq3Yb_PLr_xEqd8CyMfSp54msNKS0n1vQda4h6WWIivlOYrDuEWZoyB558pwJLyzG9KxkgU6R2Hw6ApzgvPAweOeerTXGn8HqeEMDZ9ymO-Oqz3CU_ZowFGis-O85R9_fD-y_mn5uLy4-fzs4sGdeuWxmLou97hsBMGQodWt0YBotFGaYVdG2IrBQYDrkVrBqnsDqR2CqV0PYI-Za_vcuvFP9ZIi58SYRxHmGNeyctaoLTCalvRl_-h13ktc73Oy87Uj61xulJv7igsmajEwd-UNEH55aXwBze-uvEHN75GV_zFMXTtpxj-wX9lVODVEQCqDQ2lVp3onmuVEKra_AO8NJlL</recordid><startdate>20130101</startdate><enddate>20130101</enddate><creator>LUYTEN, J</creator><creator>SNIEGOWSKI, K</creator><creator>VAN EYCK, K</creator><creator>MAERTENS, D</creator><creator>TIMMERMANS, S</creator><creator>LIERS, Sven</creator><creator>BRAEKEN, L</creator><general>International Water Association</general><general>IWA Publishing</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QH</scope><scope>7UA</scope><scope>7X7</scope><scope>7XB</scope><scope>88E</scope><scope>8FE</scope><scope>8FG</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>BHPHI</scope><scope>BKSAR</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>F1W</scope><scope>FYUFA</scope><scope>GHDGH</scope><scope>H96</scope><scope>H97</scope><scope>HCIFZ</scope><scope>K9.</scope><scope>L.G</scope><scope>L6V</scope><scope>M0S</scope><scope>M1P</scope><scope>M7S</scope><scope>PCBAR</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PTHSS</scope><scope>7X8</scope></search><sort><creationdate>20130101</creationdate><title>AOX removal from industrial wastewaters using advanced oxidation processes: assessment of a combined chemical-biological oxidation</title><author>LUYTEN, J ; SNIEGOWSKI, K ; VAN EYCK, K ; MAERTENS, D ; TIMMERMANS, S ; LIERS, Sven ; BRAEKEN, L</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c387t-6cdb9b7cf504ad9c63842acc434232c98de810cd4a78c64f1265a1372c117bca3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2013</creationdate><topic>Aeration</topic><topic>Analysis methods</topic><topic>Applied sciences</topic><topic>Biodegradation, Environmental</topic><topic>Biological oxidation</topic><topic>Biological Oxygen Demand Analysis</topic><topic>Chemical compounds</topic><topic>Chemical oxygen demand</topic><topic>Dosage</topic><topic>Exact sciences and technology</topic><topic>General purification processes</topic><topic>Halogenation</topic><topic>Hydrogen peroxide</topic><topic>Hydrogen Peroxide - chemistry</topic><topic>Hydrogen-Ion Concentration</topic><topic>Industrial wastes</topic><topic>Industrial wastewater</topic><topic>Iron - chemistry</topic><topic>Natural water pollution</topic><topic>Organic Chemicals - chemistry</topic><topic>Organic compounds</topic><topic>Oxidants - chemistry</topic><topic>Oxidation</topic><topic>Oxidation-Reduction</topic><topic>Ozone - chemistry</topic><topic>Pollution</topic><topic>Pulp mill effluents</topic><topic>Removal</topic><topic>Respirometry</topic><topic>Scale (corrosion)</topic><topic>Selectivity</topic><topic>Ultraviolet radiation</topic><topic>Ultraviolet Rays</topic><topic>Waste Disposal, Fluid - methods</topic><topic>Wastewater</topic><topic>Wastewaters</topic><topic>Water Pollutants, Chemical - chemistry</topic><topic>Water Pollution, Chemical - prevention & control</topic><topic>Water treatment and pollution</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>LUYTEN, J</creatorcontrib><creatorcontrib>SNIEGOWSKI, K</creatorcontrib><creatorcontrib>VAN EYCK, K</creatorcontrib><creatorcontrib>MAERTENS, D</creatorcontrib><creatorcontrib>TIMMERMANS, S</creatorcontrib><creatorcontrib>LIERS, Sven</creatorcontrib><creatorcontrib>BRAEKEN, L</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Aqualine</collection><collection>Water Resources Abstracts</collection><collection>Health & Medical Collection (Proquest)</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Medical Database (Alumni Edition)</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni)</collection><collection>ProQuest Central</collection><collection>AUTh Library subscriptions: ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest Natural Science Collection</collection><collection>Earth, Atmospheric & Aquatic Science Collection</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Health Research Premium Collection</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 3: Aquatic Pollution & Environmental Quality</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><collection>ProQuest Engineering Collection</collection><collection>Health & Medical Collection (Alumni Edition)</collection><collection>PML(ProQuest Medical Library)</collection><collection>Engineering Database</collection><collection>Earth, Atmospheric & Aquatic Science Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Engineering Collection</collection><collection>MEDLINE - Academic</collection><jtitle>Water science and technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>LUYTEN, J</au><au>SNIEGOWSKI, K</au><au>VAN EYCK, K</au><au>MAERTENS, D</au><au>TIMMERMANS, S</au><au>LIERS, Sven</au><au>BRAEKEN, L</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>AOX removal from industrial wastewaters using advanced oxidation processes: assessment of a combined chemical-biological oxidation</atitle><jtitle>Water science and technology</jtitle><addtitle>Water Sci Technol</addtitle><date>2013-01-01</date><risdate>2013</risdate><volume>68</volume><issue>9</issue><spage>2048</spage><epage>2054</epage><pages>2048-2054</pages><issn>0273-1223</issn><eissn>1996-9732</eissn><coden>WSTED4</coden><abstract>In this paper, the abatement of adsorbable halogenated organic compounds (AOX) from an industrial wastewater containing relatively high chloride concentrations by a combined chemical and biological oxidation is assessed. For chemical oxidation, the O(3)/UV, H(2)O(2)/UV and photo-Fenton processes are evaluated on pilot scale. Biological oxidation is simulated in a 4 h respirometry experiment with periodic aeration. The results show that a selective degradation of AOX with respect to the matrix compounds (expressed as chemical oxygen demand) could be achieved. For O(3)/UV, lowering the ratio of O(3) dosage to UV intensity leads to a better selectivity for AOX. During O(3)-based experiments, the AOX removal is generally less than during the H(2)O(2)-based experiments. However, after biological oxidation, the AOX levels are comparable. For H(2)O(2)/UV, optimal operating parameters for UV and H(2)O(2) dosage are next determined in a second run with another wastewater sample.</abstract><cop>London</cop><pub>International Water Association</pub><pmid>24225107</pmid><doi>10.2166/wst.2013.459</doi><tpages>7</tpages><oa>free_for_read</oa></addata></record> |
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| issn | 0273-1223 1996-9732 |
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| subjects | Aeration Analysis methods Applied sciences Biodegradation, Environmental Biological oxidation Biological Oxygen Demand Analysis Chemical compounds Chemical oxygen demand Dosage Exact sciences and technology General purification processes Halogenation Hydrogen peroxide Hydrogen Peroxide - chemistry Hydrogen-Ion Concentration Industrial wastes Industrial wastewater Iron - chemistry Natural water pollution Organic Chemicals - chemistry Organic compounds Oxidants - chemistry Oxidation Oxidation-Reduction Ozone - chemistry Pollution Pulp mill effluents Removal Respirometry Scale (corrosion) Selectivity Ultraviolet radiation Ultraviolet Rays Waste Disposal, Fluid - methods Wastewater Wastewaters Water Pollutants, Chemical - chemistry Water Pollution, Chemical - prevention & control Water treatment and pollution |
| title | AOX removal from industrial wastewaters using advanced oxidation processes: assessment of a combined chemical-biological oxidation |
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