Post-1990 Temporal Trends of PCBs and Organochlorine Pesticides in the Atmosphere and in Fish from Lakes Erie, Michigan, and Superior
We have analyzed concentration data sets covering the period 1992–2010 from the Great Lakes Integrated Atmospheric Deposition Network and from the Great Lakes Fish Monitoring and Surveillance Program to determine and compare pollutant time trends in the atmosphere and in fish. The analytes of intere...
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| Veröffentlicht in: | Environmental science & technology 2013-08, Vol.47 (16), p.9109-9114 |
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| creator | Salamova, Amina Pagano, James J Holsen, Thomas M Hites, Ronald A |
| description | We have analyzed concentration data sets covering the period 1992–2010 from the Great Lakes Integrated Atmospheric Deposition Network and from the Great Lakes Fish Monitoring and Surveillance Program to determine and compare pollutant time trends in the atmosphere and in fish. The analytes of interest were polychlorinated biphenyls, DDTs, chlordanes, dieldrin, and α- and γ-hexachlorocyclohexane (HCHs), and the sites of interest were Lakes Erie, Michigan, and Superior. Overall, we found no significant differences between the atmospheric and fish temporal trends for any of these compounds in any of the lakes. Polychlorinated biphenyl concentrations are decreasing in both the atmosphere and in the fish with halving times of 14 ± 2 years. The halving times for DDTs, chlordanes, and dieldrin are 8.7 ± 0.4 years for both the atmosphere and the fish. The most rapid temporal trend was observed for α- and γ-HCH concentrations, which are decreasing in both the atmosphere and in fish with halving times of 3.3 ± 0.4 years. The practical implications of these results are discussed. |
| doi_str_mv | 10.1021/es401895g |
| format | Article |
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The analytes of interest were polychlorinated biphenyls, DDTs, chlordanes, dieldrin, and α- and γ-hexachlorocyclohexane (HCHs), and the sites of interest were Lakes Erie, Michigan, and Superior. Overall, we found no significant differences between the atmospheric and fish temporal trends for any of these compounds in any of the lakes. Polychlorinated biphenyl concentrations are decreasing in both the atmosphere and in the fish with halving times of 14 ± 2 years. The halving times for DDTs, chlordanes, and dieldrin are 8.7 ± 0.4 years for both the atmosphere and the fish. The most rapid temporal trend was observed for α- and γ-HCH concentrations, which are decreasing in both the atmosphere and in fish with halving times of 3.3 ± 0.4 years. The practical implications of these results are discussed.</description><identifier>ISSN: 0013-936X</identifier><identifier>EISSN: 1520-5851</identifier><identifier>DOI: 10.1021/es401895g</identifier><identifier>PMID: 23905987</identifier><identifier>CODEN: ESTHAG</identifier><language>eng</language><publisher>Washington, DC: American Chemical Society</publisher><subject>Agnatha. Pisces ; Air Pollutants - analysis ; Animal, plant and microbial ecology ; Animals ; Applied ecology ; Applied sciences ; Aquatic ecology ; Atmospheric pollution ; Biological and medical sciences ; Comparative analysis ; Earth sciences ; Earth, ocean, space ; Ecotoxicology, biological effects of pollution ; Effects of pollution and side effects of pesticides on vertebrates ; Engineering and environment geology. Geothermics ; Environmental Monitoring ; Exact sciences and technology ; Fishes ; Fundamental and applied biological sciences. 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Sci. Technol</addtitle><description>We have analyzed concentration data sets covering the period 1992–2010 from the Great Lakes Integrated Atmospheric Deposition Network and from the Great Lakes Fish Monitoring and Surveillance Program to determine and compare pollutant time trends in the atmosphere and in fish. The analytes of interest were polychlorinated biphenyls, DDTs, chlordanes, dieldrin, and α- and γ-hexachlorocyclohexane (HCHs), and the sites of interest were Lakes Erie, Michigan, and Superior. Overall, we found no significant differences between the atmospheric and fish temporal trends for any of these compounds in any of the lakes. Polychlorinated biphenyl concentrations are decreasing in both the atmosphere and in the fish with halving times of 14 ± 2 years. The halving times for DDTs, chlordanes, and dieldrin are 8.7 ± 0.4 years for both the atmosphere and the fish. The most rapid temporal trend was observed for α- and γ-HCH concentrations, which are decreasing in both the atmosphere and in fish with halving times of 3.3 ± 0.4 years. The practical implications of these results are discussed.</description><subject>Agnatha. Pisces</subject><subject>Air Pollutants - analysis</subject><subject>Animal, plant and microbial ecology</subject><subject>Animals</subject><subject>Applied ecology</subject><subject>Applied sciences</subject><subject>Aquatic ecology</subject><subject>Atmospheric pollution</subject><subject>Biological and medical sciences</subject><subject>Comparative analysis</subject><subject>Earth sciences</subject><subject>Earth, ocean, space</subject><subject>Ecotoxicology, biological effects of pollution</subject><subject>Effects of pollution and side effects of pesticides on vertebrates</subject><subject>Engineering and environment geology. Geothermics</subject><subject>Environmental Monitoring</subject><subject>Exact sciences and technology</subject><subject>Fishes</subject><subject>Fundamental and applied biological sciences. Psychology</subject><subject>Great Lakes Region</subject><subject>Hydrocarbons, Chlorinated - analysis</subject><subject>Lakes</subject><subject>Organic chemistry</subject><subject>PCB</subject><subject>Pesticides</subject><subject>Pesticides - analysis</subject><subject>Pollutants</subject><subject>Pollutants physicochemistry study: properties, effects, reactions, transport and distribution</subject><subject>Pollution</subject><subject>Pollution, environment geology</subject><subject>Polychlorinated biphenyls</subject><subject>Polychlorinated Biphenyls - analysis</subject><subject>Regression Analysis</subject><subject>Trends</subject><issn>0013-936X</issn><issn>1520-5851</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2013</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqN0VFr1TAUB_Agiru7-uAXkIAICqs7aZKmfZyXTQdXdmFX8K2k6cma2TZd0j74Afa97d2u29AXnwLhxz8550_IGwafGKTsGKMAlhfy6hlZMJlCInPJnpMFAONJwbMfB-QwxmsASDnkL8lByguQRa4W5Hbj45iwogC6xW7wQbd0G7CvI_WWblafI9V9TS_Cle69aVofXI90g3F0xtUYqevp2CA9GTsfhwYD3vn59szFhtrgO7rWP2d4Ghwe0W_ONG7OOrpjl9OAwfnwirywuo34en8uyfez0-3qa7K--HK-OlknWkA2JopZy-salNCCGSOqAivLdGVlnokstQIx50pBUaO0TIDKlWIgpeAVs0JoviQf7nOH4G-meYiyc9Fg2-oe_RRLJriYF5qz7D9ominJ0jl8Sd79Ra_9FPp5kJ1SIuMp7AI_3isTfIwBbTkE1-nwq2RQ7mosH2qc7dt94lR1WD_IP73N4P0e6Gh0a4PujYuPTmVKpBIenTbxya_-efA3kp-uBw</recordid><startdate>20130820</startdate><enddate>20130820</enddate><creator>Salamova, Amina</creator><creator>Pagano, James J</creator><creator>Holsen, Thomas M</creator><creator>Hites, Ronald A</creator><general>American Chemical Society</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QO</scope><scope>7ST</scope><scope>7T7</scope><scope>7U7</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>P64</scope><scope>SOI</scope><scope>7X8</scope><scope>7QH</scope><scope>7TG</scope><scope>7TV</scope><scope>7UA</scope><scope>F1W</scope><scope>H97</scope><scope>KL.</scope><scope>L.G</scope></search><sort><creationdate>20130820</creationdate><title>Post-1990 Temporal Trends of PCBs and Organochlorine Pesticides in the Atmosphere and in Fish from Lakes Erie, Michigan, and Superior</title><author>Salamova, Amina ; Pagano, James J ; Holsen, Thomas M ; Hites, Ronald A</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a406t-71ff3dd074a41cc4b9ebf1abf586462f4ee837709de5f1407877105543b1f44a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2013</creationdate><topic>Agnatha. Pisces</topic><topic>Air Pollutants - analysis</topic><topic>Animal, plant and microbial ecology</topic><topic>Animals</topic><topic>Applied ecology</topic><topic>Applied sciences</topic><topic>Aquatic ecology</topic><topic>Atmospheric pollution</topic><topic>Biological and medical sciences</topic><topic>Comparative analysis</topic><topic>Earth sciences</topic><topic>Earth, ocean, space</topic><topic>Ecotoxicology, biological effects of pollution</topic><topic>Effects of pollution and side effects of pesticides on vertebrates</topic><topic>Engineering and environment geology. Geothermics</topic><topic>Environmental Monitoring</topic><topic>Exact sciences and technology</topic><topic>Fishes</topic><topic>Fundamental and applied biological sciences. Psychology</topic><topic>Great Lakes Region</topic><topic>Hydrocarbons, Chlorinated - analysis</topic><topic>Lakes</topic><topic>Organic chemistry</topic><topic>PCB</topic><topic>Pesticides</topic><topic>Pesticides - analysis</topic><topic>Pollutants</topic><topic>Pollutants physicochemistry study: properties, effects, reactions, transport and distribution</topic><topic>Pollution</topic><topic>Pollution, environment geology</topic><topic>Polychlorinated biphenyls</topic><topic>Polychlorinated Biphenyls - analysis</topic><topic>Regression Analysis</topic><topic>Trends</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Salamova, Amina</creatorcontrib><creatorcontrib>Pagano, James J</creatorcontrib><creatorcontrib>Holsen, Thomas M</creatorcontrib><creatorcontrib>Hites, Ronald A</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Biotechnology Research Abstracts</collection><collection>Environment Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Toxicology Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environment Abstracts</collection><collection>MEDLINE - Academic</collection><collection>Aqualine</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Pollution Abstracts</collection><collection>Water Resources Abstracts</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 3: Aquatic Pollution & Environmental Quality</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><jtitle>Environmental science & technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Salamova, Amina</au><au>Pagano, James J</au><au>Holsen, Thomas M</au><au>Hites, Ronald A</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Post-1990 Temporal Trends of PCBs and Organochlorine Pesticides in the Atmosphere and in Fish from Lakes Erie, Michigan, and Superior</atitle><jtitle>Environmental science & technology</jtitle><addtitle>Environ. Sci. Technol</addtitle><date>2013-08-20</date><risdate>2013</risdate><volume>47</volume><issue>16</issue><spage>9109</spage><epage>9114</epage><pages>9109-9114</pages><issn>0013-936X</issn><eissn>1520-5851</eissn><coden>ESTHAG</coden><abstract>We have analyzed concentration data sets covering the period 1992–2010 from the Great Lakes Integrated Atmospheric Deposition Network and from the Great Lakes Fish Monitoring and Surveillance Program to determine and compare pollutant time trends in the atmosphere and in fish. The analytes of interest were polychlorinated biphenyls, DDTs, chlordanes, dieldrin, and α- and γ-hexachlorocyclohexane (HCHs), and the sites of interest were Lakes Erie, Michigan, and Superior. Overall, we found no significant differences between the atmospheric and fish temporal trends for any of these compounds in any of the lakes. Polychlorinated biphenyl concentrations are decreasing in both the atmosphere and in the fish with halving times of 14 ± 2 years. The halving times for DDTs, chlordanes, and dieldrin are 8.7 ± 0.4 years for both the atmosphere and the fish. The most rapid temporal trend was observed for α- and γ-HCH concentrations, which are decreasing in both the atmosphere and in fish with halving times of 3.3 ± 0.4 years. The practical implications of these results are discussed.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><pmid>23905987</pmid><doi>10.1021/es401895g</doi><tpages>6</tpages></addata></record> |
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| subjects | Agnatha. Pisces Air Pollutants - analysis Animal, plant and microbial ecology Animals Applied ecology Applied sciences Aquatic ecology Atmospheric pollution Biological and medical sciences Comparative analysis Earth sciences Earth, ocean, space Ecotoxicology, biological effects of pollution Effects of pollution and side effects of pesticides on vertebrates Engineering and environment geology. Geothermics Environmental Monitoring Exact sciences and technology Fishes Fundamental and applied biological sciences. Psychology Great Lakes Region Hydrocarbons, Chlorinated - analysis Lakes Organic chemistry PCB Pesticides Pesticides - analysis Pollutants Pollutants physicochemistry study: properties, effects, reactions, transport and distribution Pollution Pollution, environment geology Polychlorinated biphenyls Polychlorinated Biphenyls - analysis Regression Analysis Trends |
| title | Post-1990 Temporal Trends of PCBs and Organochlorine Pesticides in the Atmosphere and in Fish from Lakes Erie, Michigan, and Superior |
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