Quantum coherence effects in hybrid nanoparticle molecules in the presence of ultra-short dephasing times

We study quantum coherence effects in single nanoparticle systems consisting of a semiconductor quantum dot and a metallic nanoparticle in the presence of the ultra-short dephasing times of the quantum dots. The results suggest that coherent exciton-plasmon coupling can sustain the collective molecu...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Applied physics letters 2012-11, Vol.101 (21)
1. Verfasser: Sadeghi, S M
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:We study quantum coherence effects in single nanoparticle systems consisting of a semiconductor quantum dot and a metallic nanoparticle in the presence of the ultra-short dephasing times of the quantum dots. The results suggest that coherent exciton-plasmon coupling can sustain the collective molecular resonances (plasmonic meta-resonances) of these systems at about room temperature. We investigate quantum optical properties of the quantum dots under this condition, demonstrating formation of ultranarrow gain and absorption spectral lines. These results are discussed in terms of plasmonic normalization of coherent population oscillation and the collective states of the nanoparticle systems.
ISSN:0003-6951
1077-3118
DOI:10.1063/1.4767653