Spatial-spectral coupling in coherent anti-Stokes Raman scattering microscopy

Spatial-spectral coupling in coherent anti-Stokes Raman scattering microscopy

Coherent anti-Stokes Raman scattering (CARS) microscopy is a third-order nonlinear optical technique which permits label-free, molecule-specific hyperspectral imaging. The interference between coherent resonant and non-resonant terms leads to well known distortions in the vibrational spectrum, requi...

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Veröffentlicht in:Optics express 2013-07, Vol.21 (13), p.15298-15307
Hauptverfasser: Barlow, Aaron M, Popov, Konstantin, Andreana, Marco, Moffatt, Douglas J, Ridsdale, Andrew, Slepkov, Aaron D, Harden, James L, Ramunno, Lora, Stolow, Albert
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container_end_page 15307
container_issue 13
container_start_page 15298
container_title Optics express
container_volume 21
creator Barlow, Aaron M
Popov, Konstantin
Andreana, Marco
Moffatt, Douglas J
Ridsdale, Andrew
Slepkov, Aaron D
Harden, James L
Ramunno, Lora
Stolow, Albert
description Coherent anti-Stokes Raman scattering (CARS) microscopy is a third-order nonlinear optical technique which permits label-free, molecule-specific hyperspectral imaging. The interference between coherent resonant and non-resonant terms leads to well known distortions in the vibrational spectrum, requiring the use of retrieval algorithms. It also leads to spatial imaging distortions, largely due to the Gouy phase, when objects are smaller than the Rayleigh range. Here we consider that the focal position and spectral contributions to the nonlinear image formation are intrinsically coupled and cannot be corrected by conventional retrieval methods.
doi_str_mv 10.1364/OE.21.015298
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title Spatial-spectral coupling in coherent anti-Stokes Raman scattering microscopy
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