Multiscale non-adiabatic dynamics with radiative decay, case study on the post-ionization fragmentation of rare-gas tetramers

A novel multiscale method introducing radiative decay in realistic simulations of complex systems involving metastable states is proposed in order to address the competition between non-radiative and radiative processes. Specific implementation of the proposed method is used in a case study of the p...

Ausführliche Beschreibung

Gespeichert in:

Bibliographische Detailangaben
Veröffentlicht in:	Europhysics letters 2012-05, Vol.98 (3), p.1-1
Hauptverfasser:	Janecek, I, Janca, T, Naar, P, Renard, F, Kalus, R, Gadea, F X
Format:	Artikel
Sprache:	eng
Schlagworte:	Complex systems Decay Dynamic tests Dynamics Fragmentation Monomers Multiscale methods Simulation
Online-Zugang:	Volltext
Tags:	Tag hinzufügen Keine Tags, Fügen Sie den ersten Tag hinzu!

container_end_page	1
container_issue	3
container_start_page	1
container_title	Europhysics letters
container_volume	98
creator	Janecek, I Janca, T Naar, P Renard, F Kalus, R Gadea, F X
description	A novel multiscale method introducing radiative decay in realistic simulations of complex systems involving metastable states is proposed in order to address the competition between non-radiative and radiative processes. Specific implementation of the proposed method is used in a case study of the post-ionization fragmentation of heavier rare-gas tetramers considered for very long times. The present multiscale approach allows to take into account the non-adiabatic dynamics typically in tens of picoseconds as well as radiative decay typically in the microsecond regime. Agreement with experimental findings that mainly monomer ion fragments are produced is found here for the first time for Kr... and to some extent also for Xe... (ProQuest: ... denotes formulae/symbols omitted.)
format	Article
fullrecord	<record><control><sourceid>proquest</sourceid><recordid>TN_cdi_proquest_miscellaneous_1372623387</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1372623387</sourcerecordid><originalsourceid>FETCH-proquest_miscellaneous_13726233873</originalsourceid><addsrcrecordid>eNqVjs1OwzAQhC0EEuHnHfbYQy3FSfPDGVH1wo17tXU2rZFjF--mKJX67g2CF-A0mplPo7lRmSnaWq_aanWrsrx4qXSVN9W9emD-zHNjWlNn6vI-enFs0ROEGDR2DncozkI3BRycZfh2coD0U4g7EXRkcVqCRSZgGbsJYgA5EBwji3YxuPMMzlmfcD9QkF8X-3kjkd4jg5AkHCjxk7rr0TM9_-mjWqzfPl43-pji10gs22H-Rt5joDjy1pRNURdl2TblP9ArVlZV5w</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1372623387</pqid></control><display><type>article</type><title>Multiscale non-adiabatic dynamics with radiative decay, case study on the post-ionization fragmentation of rare-gas tetramers</title><source>IOP Publishing Journals</source><creator>Janecek, I ; Janca, T ; Naar, P ; Renard, F ; Kalus, R ; Gadea, F X</creator><creatorcontrib>Janecek, I ; Janca, T ; Naar, P ; Renard, F ; Kalus, R ; Gadea, F X</creatorcontrib><description>A novel multiscale method introducing radiative decay in realistic simulations of complex systems involving metastable states is proposed in order to address the competition between non-radiative and radiative processes. Specific implementation of the proposed method is used in a case study of the post-ionization fragmentation of heavier rare-gas tetramers considered for very long times. The present multiscale approach allows to take into account the non-adiabatic dynamics typically in tens of picoseconds as well as radiative decay typically in the microsecond regime. Agreement with experimental findings that mainly monomer ion fragments are produced is found here for the first time for Kr... and to some extent also for Xe... (ProQuest: ... denotes formulae/symbols omitted.)</description><identifier>ISSN: 0295-5075</identifier><identifier>EISSN: 1286-4854</identifier><language>eng</language><subject>Complex systems ; Decay ; Dynamic tests ; Dynamics ; Fragmentation ; Monomers ; Multiscale methods ; Simulation</subject><ispartof>Europhysics letters, 2012-05, Vol.98 (3), p.1-1</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780</link.rule.ids></links><search><creatorcontrib>Janecek, I</creatorcontrib><creatorcontrib>Janca, T</creatorcontrib><creatorcontrib>Naar, P</creatorcontrib><creatorcontrib>Renard, F</creatorcontrib><creatorcontrib>Kalus, R</creatorcontrib><creatorcontrib>Gadea, F X</creatorcontrib><title>Multiscale non-adiabatic dynamics with radiative decay, case study on the post-ionization fragmentation of rare-gas tetramers</title><title>Europhysics letters</title><description>A novel multiscale method introducing radiative decay in realistic simulations of complex systems involving metastable states is proposed in order to address the competition between non-radiative and radiative processes. Specific implementation of the proposed method is used in a case study of the post-ionization fragmentation of heavier rare-gas tetramers considered for very long times. The present multiscale approach allows to take into account the non-adiabatic dynamics typically in tens of picoseconds as well as radiative decay typically in the microsecond regime. Agreement with experimental findings that mainly monomer ion fragments are produced is found here for the first time for Kr... and to some extent also for Xe... (ProQuest: ... denotes formulae/symbols omitted.)</description><subject>Complex systems</subject><subject>Decay</subject><subject>Dynamic tests</subject><subject>Dynamics</subject><subject>Fragmentation</subject><subject>Monomers</subject><subject>Multiscale methods</subject><subject>Simulation</subject><issn>0295-5075</issn><issn>1286-4854</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><recordid>eNqVjs1OwzAQhC0EEuHnHfbYQy3FSfPDGVH1wo17tXU2rZFjF--mKJX67g2CF-A0mplPo7lRmSnaWq_aanWrsrx4qXSVN9W9emD-zHNjWlNn6vI-enFs0ROEGDR2DncozkI3BRycZfh2coD0U4g7EXRkcVqCRSZgGbsJYgA5EBwji3YxuPMMzlmfcD9QkF8X-3kjkd4jg5AkHCjxk7rr0TM9_-mjWqzfPl43-pji10gs22H-Rt5joDjy1pRNURdl2TblP9ArVlZV5w</recordid><startdate>20120501</startdate><enddate>20120501</enddate><creator>Janecek, I</creator><creator>Janca, T</creator><creator>Naar, P</creator><creator>Renard, F</creator><creator>Kalus, R</creator><creator>Gadea, F X</creator><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>20120501</creationdate><title>Multiscale non-adiabatic dynamics with radiative decay, case study on the post-ionization fragmentation of rare-gas tetramers</title><author>Janecek, I ; Janca, T ; Naar, P ; Renard, F ; Kalus, R ; Gadea, F X</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-proquest_miscellaneous_13726233873</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2012</creationdate><topic>Complex systems</topic><topic>Decay</topic><topic>Dynamic tests</topic><topic>Dynamics</topic><topic>Fragmentation</topic><topic>Monomers</topic><topic>Multiscale methods</topic><topic>Simulation</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Janecek, I</creatorcontrib><creatorcontrib>Janca, T</creatorcontrib><creatorcontrib>Naar, P</creatorcontrib><creatorcontrib>Renard, F</creatorcontrib><creatorcontrib>Kalus, R</creatorcontrib><creatorcontrib>Gadea, F X</creatorcontrib><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Europhysics letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Janecek, I</au><au>Janca, T</au><au>Naar, P</au><au>Renard, F</au><au>Kalus, R</au><au>Gadea, F X</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Multiscale non-adiabatic dynamics with radiative decay, case study on the post-ionization fragmentation of rare-gas tetramers</atitle><jtitle>Europhysics letters</jtitle><date>2012-05-01</date><risdate>2012</risdate><volume>98</volume><issue>3</issue><spage>1</spage><epage>1</epage><pages>1-1</pages><issn>0295-5075</issn><eissn>1286-4854</eissn><abstract>A novel multiscale method introducing radiative decay in realistic simulations of complex systems involving metastable states is proposed in order to address the competition between non-radiative and radiative processes. Specific implementation of the proposed method is used in a case study of the post-ionization fragmentation of heavier rare-gas tetramers considered for very long times. The present multiscale approach allows to take into account the non-adiabatic dynamics typically in tens of picoseconds as well as radiative decay typically in the microsecond regime. Agreement with experimental findings that mainly monomer ion fragments are produced is found here for the first time for Kr... and to some extent also for Xe... (ProQuest: ... denotes formulae/symbols omitted.)</abstract></addata></record>
fulltext	fulltext
identifier	ISSN: 0295-5075
ispartof	Europhysics letters, 2012-05, Vol.98 (3), p.1-1
issn	0295-5075 1286-4854
language	eng
recordid	cdi_proquest_miscellaneous_1372623387
source	IOP Publishing Journals
subjects	Complex systems Decay Dynamic tests Dynamics Fragmentation Monomers Multiscale methods Simulation
title	Multiscale non-adiabatic dynamics with radiative decay, case study on the post-ionization fragmentation of rare-gas tetramers
url	https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-06T08%3A48%3A24IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Multiscale%20non-adiabatic%20dynamics%20with%20radiative%20decay,%20case%20study%20on%20the%20post-ionization%20fragmentation%20of%20rare-gas%20tetramers&rft.jtitle=Europhysics%20letters&rft.au=Janecek,%20I&rft.date=2012-05-01&rft.volume=98&rft.issue=3&rft.spage=1&rft.epage=1&rft.pages=1-1&rft.issn=0295-5075&rft.eissn=1286-4854&rft_id=info:doi/&rft_dat=%3Cproquest%3E1372623387%3C/proquest%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1372623387&rft_id=info:pmid/&rfr_iscdi=true