Three-photon near-infrared quantum cutting in Tm3+-doped transparent oxyfluoride glass ceramics
Efficient three-step sequential three-photon near-infrared (NIR) quantum cutting in Tm3+-doped transparent oxyfluoride glass ceramics has been demonstrated, where an absorbed blue photon could be cut into three NIR photons at 1190, 1460, and 1800 nm with quantum yield greater than unity. On the basi...
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Veröffentlicht in: | Applied physics letters 2012-10, Vol.101 (17) |
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creator | Yu, D. C. Zhang, J. P. Chen, Q. J. Zhang, W. J. Yang, Z. M. Zhang, Q. Y. |
description | Efficient three-step sequential three-photon near-infrared (NIR) quantum cutting in Tm3+-doped transparent oxyfluoride glass ceramics has been demonstrated, where an absorbed blue photon could be cut into three NIR photons at 1190, 1460, and 1800 nm with quantum yield greater than unity. On the basis of static and dynamic photoemission, monitored excitation, and time-resolved fluorescence spectra, we investigate in detail the underlying optoelectronic mechanism. Further development of an efficient triply-cutting material might open up a path towards ultra-efficient photonic devices, which enables more photons emitted than absorbed in the excitation process. |
doi_str_mv | 10.1063/1.4764005 |
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C. ; Zhang, J. P. ; Chen, Q. J. ; Zhang, W. J. ; Yang, Z. M. ; Zhang, Q. Y.</creator><creatorcontrib>Yu, D. C. ; Zhang, J. P. ; Chen, Q. J. ; Zhang, W. J. ; Yang, Z. M. ; Zhang, Q. Y.</creatorcontrib><description>Efficient three-step sequential three-photon near-infrared (NIR) quantum cutting in Tm3+-doped transparent oxyfluoride glass ceramics has been demonstrated, where an absorbed blue photon could be cut into three NIR photons at 1190, 1460, and 1800 nm with quantum yield greater than unity. On the basis of static and dynamic photoemission, monitored excitation, and time-resolved fluorescence spectra, we investigate in detail the underlying optoelectronic mechanism. 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Further development of an efficient triply-cutting material might open up a path towards ultra-efficient photonic devices, which enables more photons emitted than absorbed in the excitation process.</description><subject>Cutting</subject><subject>Dynamic tests</subject><subject>Excitation</subject><subject>Glass ceramics</subject><subject>Oxyfluorides</subject><subject>Photons</subject><subject>Spectra</subject><subject>Unity</subject><issn>0003-6951</issn><issn>1077-3118</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><recordid>eNotkM9LwzAcxYMoOKcH_4McFclMmrRJjzL8BQMv8xy-TZOt0iZdkoL7761sp_ce78M7PITuGV0xWvFnthKyEpSWF2jBqJSEM6Yu0YJSyklVl-wa3aT0M8ey4HyB9HYfrSXjPuTgsbcQSeddhGhbfJjA52nAZsq58zvcebwd-BNpwzi3OYJP4wz6jMPv0fVTiF1r8a6HlLCxEYbOpFt05aBP9u6sS_T99rpdf5DN1_vn-mVDDKuLTKQBUUkluWS1kqpRrhZtUxtVza5WjRMSrFWKNUI5A8wZxQGqtpkrBa7gS_Rw2h1jOEw2ZT10ydi-B2_DlDTjBS-YLCsxo48n1MSQUrROj7EbIB41o_r_RM30-UT-BxYoZW8</recordid><startdate>20121022</startdate><enddate>20121022</enddate><creator>Yu, D. 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Y.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Three-photon near-infrared quantum cutting in Tm3+-doped transparent oxyfluoride glass ceramics</atitle><jtitle>Applied physics letters</jtitle><date>2012-10-22</date><risdate>2012</risdate><volume>101</volume><issue>17</issue><issn>0003-6951</issn><eissn>1077-3118</eissn><abstract>Efficient three-step sequential three-photon near-infrared (NIR) quantum cutting in Tm3+-doped transparent oxyfluoride glass ceramics has been demonstrated, where an absorbed blue photon could be cut into three NIR photons at 1190, 1460, and 1800 nm with quantum yield greater than unity. On the basis of static and dynamic photoemission, monitored excitation, and time-resolved fluorescence spectra, we investigate in detail the underlying optoelectronic mechanism. Further development of an efficient triply-cutting material might open up a path towards ultra-efficient photonic devices, which enables more photons emitted than absorbed in the excitation process.</abstract><doi>10.1063/1.4764005</doi></addata></record> |
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source | American Institute of Physics (AIP) Journals; AIP Digital Archive; Alma/SFX Local Collection |
subjects | Cutting Dynamic tests Excitation Glass ceramics Oxyfluorides Photons Spectra Unity |
title | Three-photon near-infrared quantum cutting in Tm3+-doped transparent oxyfluoride glass ceramics |
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