Scattering of Stark-decelerated OH radicals with rare-gas atoms
We present a combined experimental and theoretical study on the rotationally inelastic scattering of OH (X 2 Π 3/2 , J = 3/2 , f ) radicals with the collision partners He, Ne, Ar, Kr, Xe, and D 2 as a function of the collision energy between ∼70 cm −1 and 400 cm −1 . The OH radicals are state select...
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| Veröffentlicht in: | The European physical journal. D, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2011-11, Vol.65 (1-2), p.189-198 |
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| container_title | The European physical journal. D, Atomic, molecular, and optical physics |
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| creator | Scharfenberg, L. Gubbels, K. B. Kirste, M. Groenenboom, G. C. van der Avoird, A. Meijer, G. van de Meerakker, S. Y. T. |
| description | We present a combined experimental and theoretical study on the rotationally inelastic scattering of OH (X
2
Π
3/2
,
J
= 3/2
, f
) radicals with the collision partners He, Ne, Ar, Kr, Xe, and D
2
as a function of the collision energy between ∼70 cm
−1
and 400 cm
−1
. The OH radicals are state selected and velocity tuned prior to the collision using a Stark decelerator, and field-free parity-resolved state-to-state inelastic relative scattering cross sections are measured in a crossed molecular beam configuration. For all OH-rare gas atom systems excellent agreement is obtained with the cross sections predicted by coupled channel scattering calculations based on accurate ab initio potential energy surfaces. This series of experiments complements recent studies on the scattering of OH radicals with Xe [J.J. Gilijamse, S. Hoekstra, S.Y.T. van de Meerakker, G.C. Groenenboom, G. Meijer, Science
313
, 1617 (2006)], Ar [L. Scharfenberg, J. Kłos, P.J. Dagdigian, M.H. Alexander, G. Meijer, S.Y.T. van de Meerakker, Phys. Chem. Chem. Phys.
12
, 10660 (2010)], He, and D
2
[M. Kirste, L. Scharfenberg, J. Kłos, F. Lique, M.H. Alexander, G. Meijer, S.Y.T. van de Meerakker, Phys. Rev. A
82
, 042717 (2010)]. A comparison of the relative scattering cross sections for this set of collision partners reveals interesting trends in the scattering behavior. |
| doi_str_mv | 10.1140/epjd/e2011-20009-4 |
| format | Article |
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2
Π
3/2
,
J
= 3/2
, f
) radicals with the collision partners He, Ne, Ar, Kr, Xe, and D
2
as a function of the collision energy between ∼70 cm
−1
and 400 cm
−1
. The OH radicals are state selected and velocity tuned prior to the collision using a Stark decelerator, and field-free parity-resolved state-to-state inelastic relative scattering cross sections are measured in a crossed molecular beam configuration. For all OH-rare gas atom systems excellent agreement is obtained with the cross sections predicted by coupled channel scattering calculations based on accurate ab initio potential energy surfaces. This series of experiments complements recent studies on the scattering of OH radicals with Xe [J.J. Gilijamse, S. Hoekstra, S.Y.T. van de Meerakker, G.C. Groenenboom, G. Meijer, Science
313
, 1617 (2006)], Ar [L. Scharfenberg, J. Kłos, P.J. Dagdigian, M.H. Alexander, G. Meijer, S.Y.T. van de Meerakker, Phys. Chem. Chem. Phys.
12
, 10660 (2010)], He, and D
2
[M. Kirste, L. Scharfenberg, J. Kłos, F. Lique, M.H. Alexander, G. Meijer, S.Y.T. van de Meerakker, Phys. Rev. A
82
, 042717 (2010)]. A comparison of the relative scattering cross sections for this set of collision partners reveals interesting trends in the scattering behavior.</description><identifier>ISSN: 1434-6060</identifier><identifier>EISSN: 1434-6079</identifier><identifier>DOI: 10.1140/epjd/e2011-20009-4</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Applications of Nonlinear Dynamics and Chaos Theory ; Atomic ; Channels ; Collision dynamics ; Cross sections ; Mathematical analysis ; Molecular ; Molecular beams ; Optical and Plasma Physics ; Physical Chemistry ; Physics ; Physics and Astronomy ; Quantum Information Technology ; Quantum Physics ; Radicals ; Regular Article ; Scattering ; Scattering cross sections ; Spectroscopy/Spectrometry ; Spintronics</subject><ispartof>The European physical journal. D, Atomic, molecular, and optical physics, 2011-11, Vol.65 (1-2), p.189-198</ispartof><rights>EDP Sciences, SIF, Springer-Verlag Berlin Heidelberg 2011</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c324t-cbeecb4cdd5041a131c397b4f8779d80bfd881edddc9774d09a2766bcb029d4c3</citedby><cites>FETCH-LOGICAL-c324t-cbeecb4cdd5041a131c397b4f8779d80bfd881edddc9774d09a2766bcb029d4c3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1140/epjd/e2011-20009-4$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1140/epjd/e2011-20009-4$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Scharfenberg, L.</creatorcontrib><creatorcontrib>Gubbels, K. B.</creatorcontrib><creatorcontrib>Kirste, M.</creatorcontrib><creatorcontrib>Groenenboom, G. C.</creatorcontrib><creatorcontrib>van der Avoird, A.</creatorcontrib><creatorcontrib>Meijer, G.</creatorcontrib><creatorcontrib>van de Meerakker, S. Y. T.</creatorcontrib><title>Scattering of Stark-decelerated OH radicals with rare-gas atoms</title><title>The European physical journal. D, Atomic, molecular, and optical physics</title><addtitle>Eur. Phys. J. D</addtitle><description>We present a combined experimental and theoretical study on the rotationally inelastic scattering of OH (X
2
Π
3/2
,
J
= 3/2
, f
) radicals with the collision partners He, Ne, Ar, Kr, Xe, and D
2
as a function of the collision energy between ∼70 cm
−1
and 400 cm
−1
. The OH radicals are state selected and velocity tuned prior to the collision using a Stark decelerator, and field-free parity-resolved state-to-state inelastic relative scattering cross sections are measured in a crossed molecular beam configuration. For all OH-rare gas atom systems excellent agreement is obtained with the cross sections predicted by coupled channel scattering calculations based on accurate ab initio potential energy surfaces. This series of experiments complements recent studies on the scattering of OH radicals with Xe [J.J. Gilijamse, S. Hoekstra, S.Y.T. van de Meerakker, G.C. Groenenboom, G. Meijer, Science
313
, 1617 (2006)], Ar [L. Scharfenberg, J. Kłos, P.J. Dagdigian, M.H. Alexander, G. Meijer, S.Y.T. van de Meerakker, Phys. Chem. Chem. Phys.
12
, 10660 (2010)], He, and D
2
[M. Kirste, L. Scharfenberg, J. Kłos, F. Lique, M.H. Alexander, G. Meijer, S.Y.T. van de Meerakker, Phys. Rev. A
82
, 042717 (2010)]. A comparison of the relative scattering cross sections for this set of collision partners reveals interesting trends in the scattering behavior.</description><subject>Applications of Nonlinear Dynamics and Chaos Theory</subject><subject>Atomic</subject><subject>Channels</subject><subject>Collision dynamics</subject><subject>Cross sections</subject><subject>Mathematical analysis</subject><subject>Molecular</subject><subject>Molecular beams</subject><subject>Optical and Plasma Physics</subject><subject>Physical Chemistry</subject><subject>Physics</subject><subject>Physics and Astronomy</subject><subject>Quantum Information Technology</subject><subject>Quantum Physics</subject><subject>Radicals</subject><subject>Regular Article</subject><subject>Scattering</subject><subject>Scattering cross sections</subject><subject>Spectroscopy/Spectrometry</subject><subject>Spintronics</subject><issn>1434-6060</issn><issn>1434-6079</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2011</creationdate><recordtype>article</recordtype><recordid>eNp9kE1PAjEQhhujiYj-AU979FKZfrDdnowhKiYkHNBz021ncRHYtS0x_nsKGI-eOs0872TmIeSWwT1jEkbYr_wIOTBGOQBoKs_IgEkhaQlKn__VJVySqxhXmeFjWQ7Iw8LZlDC022XRNcUi2fBJPTpcY7AJfTGfFsH61tl1LL7b9JF_AenSxsKmbhOvyUWTW3jz-w7J-_PT22RKZ_OX18njjDrBZaKuRnS1dN6PQTLLBHNCq1o2lVLaV1A3vqoYeu-dVkp60JarsqxdDVx76cSQ3J3m9qH72mFMZtPGvOXabrHbRcOg4pyBGJcZ5SfUhS7GgI3pQ7ux4SdD5mDLHGyZoy1ztGVkDolTKPYHFxjMqtuFbT7pv9QeIEhvLQ</recordid><startdate>20111101</startdate><enddate>20111101</enddate><creator>Scharfenberg, L.</creator><creator>Gubbels, K. B.</creator><creator>Kirste, M.</creator><creator>Groenenboom, G. C.</creator><creator>van der Avoird, A.</creator><creator>Meijer, G.</creator><creator>van de Meerakker, S. Y. T.</creator><general>Springer Berlin Heidelberg</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7U5</scope><scope>8FD</scope><scope>L7M</scope></search><sort><creationdate>20111101</creationdate><title>Scattering of Stark-decelerated OH radicals with rare-gas atoms</title><author>Scharfenberg, L. ; Gubbels, K. B. ; Kirste, M. ; Groenenboom, G. C. ; van der Avoird, A. ; Meijer, G. ; van de Meerakker, S. Y. T.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c324t-cbeecb4cdd5041a131c397b4f8779d80bfd881edddc9774d09a2766bcb029d4c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2011</creationdate><topic>Applications of Nonlinear Dynamics and Chaos Theory</topic><topic>Atomic</topic><topic>Channels</topic><topic>Collision dynamics</topic><topic>Cross sections</topic><topic>Mathematical analysis</topic><topic>Molecular</topic><topic>Molecular beams</topic><topic>Optical and Plasma Physics</topic><topic>Physical Chemistry</topic><topic>Physics</topic><topic>Physics and Astronomy</topic><topic>Quantum Information Technology</topic><topic>Quantum Physics</topic><topic>Radicals</topic><topic>Regular Article</topic><topic>Scattering</topic><topic>Scattering cross sections</topic><topic>Spectroscopy/Spectrometry</topic><topic>Spintronics</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Scharfenberg, L.</creatorcontrib><creatorcontrib>Gubbels, K. B.</creatorcontrib><creatorcontrib>Kirste, M.</creatorcontrib><creatorcontrib>Groenenboom, G. C.</creatorcontrib><creatorcontrib>van der Avoird, A.</creatorcontrib><creatorcontrib>Meijer, G.</creatorcontrib><creatorcontrib>van de Meerakker, S. Y. T.</creatorcontrib><collection>CrossRef</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>The European physical journal. D, Atomic, molecular, and optical physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Scharfenberg, L.</au><au>Gubbels, K. B.</au><au>Kirste, M.</au><au>Groenenboom, G. C.</au><au>van der Avoird, A.</au><au>Meijer, G.</au><au>van de Meerakker, S. Y. T.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Scattering of Stark-decelerated OH radicals with rare-gas atoms</atitle><jtitle>The European physical journal. D, Atomic, molecular, and optical physics</jtitle><stitle>Eur. Phys. J. D</stitle><date>2011-11-01</date><risdate>2011</risdate><volume>65</volume><issue>1-2</issue><spage>189</spage><epage>198</epage><pages>189-198</pages><issn>1434-6060</issn><eissn>1434-6079</eissn><abstract>We present a combined experimental and theoretical study on the rotationally inelastic scattering of OH (X
2
Π
3/2
,
J
= 3/2
, f
) radicals with the collision partners He, Ne, Ar, Kr, Xe, and D
2
as a function of the collision energy between ∼70 cm
−1
and 400 cm
−1
. The OH radicals are state selected and velocity tuned prior to the collision using a Stark decelerator, and field-free parity-resolved state-to-state inelastic relative scattering cross sections are measured in a crossed molecular beam configuration. For all OH-rare gas atom systems excellent agreement is obtained with the cross sections predicted by coupled channel scattering calculations based on accurate ab initio potential energy surfaces. This series of experiments complements recent studies on the scattering of OH radicals with Xe [J.J. Gilijamse, S. Hoekstra, S.Y.T. van de Meerakker, G.C. Groenenboom, G. Meijer, Science
313
, 1617 (2006)], Ar [L. Scharfenberg, J. Kłos, P.J. Dagdigian, M.H. Alexander, G. Meijer, S.Y.T. van de Meerakker, Phys. Chem. Chem. Phys.
12
, 10660 (2010)], He, and D
2
[M. Kirste, L. Scharfenberg, J. Kłos, F. Lique, M.H. Alexander, G. Meijer, S.Y.T. van de Meerakker, Phys. Rev. A
82
, 042717 (2010)]. A comparison of the relative scattering cross sections for this set of collision partners reveals interesting trends in the scattering behavior.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1140/epjd/e2011-20009-4</doi><tpages>10</tpages></addata></record> |
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| issn | 1434-6060 1434-6079 |
| language | eng |
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| source | SpringerNature Journals |
| subjects | Applications of Nonlinear Dynamics and Chaos Theory Atomic Channels Collision dynamics Cross sections Mathematical analysis Molecular Molecular beams Optical and Plasma Physics Physical Chemistry Physics Physics and Astronomy Quantum Information Technology Quantum Physics Radicals Regular Article Scattering Scattering cross sections Spectroscopy/Spectrometry Spintronics |
| title | Scattering of Stark-decelerated OH radicals with rare-gas atoms |
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