Mechanisms of two-color laser-induced field-free molecular orientation

Two mechanisms of two-color (ω+2ω) laser-induced field-free molecular orientation, based on the hyperpolarizability and ionization depletion, are explored and compared. The CO molecule is used as a computational example. While the hyperpolarizability mechanism generates small amounts of orientation...

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Veröffentlicht in:Physical review letters 2012-09, Vol.109 (11), p.113001-113001, Article 113001
Hauptverfasser: Spanner, Michael, Patchkovskii, Serguei, Frumker, Eugene, Corkum, Paul
Format: Artikel
Sprache:eng
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