Amidourea-Based Hydrogen-Bonded Heteroduplexes: Structure and Assembling Selectivity
A new class of multiply hydrogen-bonded heteroduplexes from readily available amidourea derivatives was designed, and their structures and selective assembling behaviors were investigated. Amidourea derivative 3 could selectively assemble with 1 to form a stable heteroduplex via eight intermolecular...
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| Veröffentlicht in: | Journal of organic chemistry 2012-09, Vol.77 (18), p.7815-7822 |
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| container_end_page | 7822 |
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| container_issue | 18 |
| container_start_page | 7815 |
| container_title | Journal of organic chemistry |
| container_volume | 77 |
| creator | Chu, Wei-Jun Chen, Jianming Chen, Chuan-Feng Yang, Yong Shuai, Zhigang |
| description | A new class of multiply hydrogen-bonded heteroduplexes from readily available amidourea derivatives was designed, and their structures and selective assembling behaviors were investigated. Amidourea derivative 3 could selectively assemble with 1 to form a stable heteroduplex via eight intermolecular bifurcated hydrogen bonds, but could not assemble with 2 at all, because of their unique structures and the spacing effect, although 1 and 2 possessed the same hydrogen-bonding sequence. The high stability and selectivity will make the amidourea-based hydrogen-bonded heteroduplexes be potentially applicable in the design of well-defined supramolecular architectures and novel functional materials. |
| doi_str_mv | 10.1021/jo301434a |
| format | Article |
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Amidourea derivative 3 could selectively assemble with 1 to form a stable heteroduplex via eight intermolecular bifurcated hydrogen bonds, but could not assemble with 2 at all, because of their unique structures and the spacing effect, although 1 and 2 possessed the same hydrogen-bonding sequence. 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Org. Chem</addtitle><date>2012-09-21</date><risdate>2012</risdate><volume>77</volume><issue>18</issue><spage>7815</spage><epage>7822</epage><pages>7815-7822</pages><issn>0022-3263</issn><eissn>1520-6904</eissn><coden>JOCEAH</coden><abstract>A new class of multiply hydrogen-bonded heteroduplexes from readily available amidourea derivatives was designed, and their structures and selective assembling behaviors were investigated. Amidourea derivative 3 could selectively assemble with 1 to form a stable heteroduplex via eight intermolecular bifurcated hydrogen bonds, but could not assemble with 2 at all, because of their unique structures and the spacing effect, although 1 and 2 possessed the same hydrogen-bonding sequence. The high stability and selectivity will make the amidourea-based hydrogen-bonded heteroduplexes be potentially applicable in the design of well-defined supramolecular architectures and novel functional materials.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><pmid>22924633</pmid><doi>10.1021/jo301434a</doi><tpages>8</tpages></addata></record> |
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| source | ACS Publications; MEDLINE |
| subjects | Chemistry Condensed benzenic and aromatic compounds Crystallography, X-Ray Exact sciences and technology Hydrogen Bonding Macromolecular Substances - chemical synthesis Macromolecular Substances - chemistry Models, Molecular Noncondensed benzenic compounds Organic chemistry Preparations and properties Urea - analogs & derivatives Urea - chemistry |
| title | Amidourea-Based Hydrogen-Bonded Heteroduplexes: Structure and Assembling Selectivity |
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