Photoluminescence and Raman Spectroscopy of Polycrystalline ZnO Nanofibers Deposited by Electrospinning

The technique of electrospinning offers the advantage of growing nanowires in bulk quantities in comparison with traditional methods. We report optical studies of polycrystalline zinc oxide (ZnO) nanofibers (∼100 nm thick and 5  μ m long) deposited by electrospinning. Photoluminescence from the nano...

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Veröffentlicht in:Journal of electronic materials 2011-09, Vol.40 (9), p.2015-2019
Hauptverfasser: Sen, Banani, Stroscio, Michael, Dutta, Mitra
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creator Sen, Banani
Stroscio, Michael
Dutta, Mitra
description The technique of electrospinning offers the advantage of growing nanowires in bulk quantities in comparison with traditional methods. We report optical studies of polycrystalline zinc oxide (ZnO) nanofibers (∼100 nm thick and 5  μ m long) deposited by electrospinning. Photoluminescence from the nanofibers shows a near-ultraviolet (near-UV) peak corresponding to near-band-edge emission and a strong broad peak in the visible region from oxygen antisite and interstitial defects. Temperature-dependent photoluminescence spectroscopy reveals that different carrier recombination mechanisms are dominant at low temperature. Our Raman spectroscopy results demonstrate that characterization of the quasimodes of longitudinal optical (LO) and transverse optical (TO) phonons present in an ensemble of polycrystalline nanofibers tilted at various angles in addition to the dominant E 2 (high) mode provides a promising technique for assessing the quality of such randomly oriented nanowires.
doi_str_mv 10.1007/s11664-011-1688-8
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source Springer Nature - Complete Springer Journals
subjects Carrier recombination
Characterization and Evaluation of Materials
Chemistry and Materials Science
Condensed matter: electronic structure, electrical, magnetic, and optical properties
Cross-disciplinary physics: materials science
rheology
Deposition
Electrical engineering
Electronics and Microelectronics
Electrospinning
Exact sciences and technology
Instrumentation
Materials Science
Methods of nanofabrication
Nanocrystals and nanoparticles
Nanofibers
Nanomaterials
Nanoscale materials and structures: fabrication and characterization
Nanowires
Optical and Electronic Materials
Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation
Optical properties of low-dimensional, mesoscopic, and nanoscale materials and structures
Photoluminescence
Physics
Quantum wires
Raman spectroscopy
Solid State Physics
Spectrum analysis
Zinc oxide
Zinc oxides
title Photoluminescence and Raman Spectroscopy of Polycrystalline ZnO Nanofibers Deposited by Electrospinning
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