Biaxial texture development in the ion beam assisted deposition of magnesium oxide
Low-energy ion-beam irradiation (
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Veröffentlicht in: | Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms Beam interactions with materials and atoms, 2012-02, Vol.272, p.28-32 |
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container_title | Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms |
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creator | Groves, James R. Hammond, Robert H. Matias, Vladimir DePaula, Raymond F. Stan, Liliana Clemens, Bruce M. |
description | Low-energy ion-beam irradiation ( |
doi_str_mv | 10.1016/j.nimb.2011.01.026 |
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keV) during the concurrent deposition of cubic oxide materials results in the growth of crystallographically textured thin films. A model system, magnesium oxide (MgO), has been successfully used as a biaxially textured template film for the heteroepitaxial deposition of many materials with texture dependent properties like high temperature superconductors, tunable microwave materials, and ferroelectrics. Here, we present data on the initial nucleation of biaxial crystallographic texture in this model system using an
in situ quartz crystal microbalance (QCM) substrate combined with
in situ reflected high-energy electron diffraction (RHEED). Correlation of mass uptake with the RHEED images of the growing surface shows that the development of crystallographic biaxial texture in this material system occurs suddenly as the initially polycrystalline MgO films reaches a critical film thickness of 2
nm. This texture continues to improve during subsequent growth. A simple model shows that the effect is not due simply to coverage effects. We use a combination of
in situ RHEED and
ex situ transmission electron microscopy to further elucidate the mechanism of this sudden texture formation. We present a physical model to describe this behavior and explain the role of ion-to-atom arrival ratio and underlying nucleation surface on texture development.</description><identifier>ISSN: 0168-583X</identifier><identifier>EISSN: 1872-9584</identifier><identifier>DOI: 10.1016/j.nimb.2011.01.026</identifier><language>eng</language><publisher>Elsevier B.V</publisher><subject>Biaxial texture ; Crystallography ; Deposition ; Ion beam assisted deposition ; Magnesium oxide ; Mathematical models ; Microorganisms ; Nucleation ; Nucleation and growth ; RHEED ; Surface layer ; Texture</subject><ispartof>Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms, 2012-02, Vol.272, p.28-32</ispartof><rights>2011 Elsevier B.V.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c333t-2dcab1ff07393118077df9b95ce6ebd6fb2b8e17135464dfad401efdc1a4410e3</citedby><cites>FETCH-LOGICAL-c333t-2dcab1ff07393118077df9b95ce6ebd6fb2b8e17135464dfad401efdc1a4410e3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0168583X11000450$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,27901,27902,65306</link.rule.ids></links><search><creatorcontrib>Groves, James R.</creatorcontrib><creatorcontrib>Hammond, Robert H.</creatorcontrib><creatorcontrib>Matias, Vladimir</creatorcontrib><creatorcontrib>DePaula, Raymond F.</creatorcontrib><creatorcontrib>Stan, Liliana</creatorcontrib><creatorcontrib>Clemens, Bruce M.</creatorcontrib><title>Biaxial texture development in the ion beam assisted deposition of magnesium oxide</title><title>Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms</title><description>Low-energy ion-beam irradiation (<1
keV) during the concurrent deposition of cubic oxide materials results in the growth of crystallographically textured thin films. A model system, magnesium oxide (MgO), has been successfully used as a biaxially textured template film for the heteroepitaxial deposition of many materials with texture dependent properties like high temperature superconductors, tunable microwave materials, and ferroelectrics. Here, we present data on the initial nucleation of biaxial crystallographic texture in this model system using an
in situ quartz crystal microbalance (QCM) substrate combined with
in situ reflected high-energy electron diffraction (RHEED). Correlation of mass uptake with the RHEED images of the growing surface shows that the development of crystallographic biaxial texture in this material system occurs suddenly as the initially polycrystalline MgO films reaches a critical film thickness of 2
nm. This texture continues to improve during subsequent growth. A simple model shows that the effect is not due simply to coverage effects. We use a combination of
in situ RHEED and
ex situ transmission electron microscopy to further elucidate the mechanism of this sudden texture formation. We present a physical model to describe this behavior and explain the role of ion-to-atom arrival ratio and underlying nucleation surface on texture development.</description><subject>Biaxial texture</subject><subject>Crystallography</subject><subject>Deposition</subject><subject>Ion beam assisted deposition</subject><subject>Magnesium oxide</subject><subject>Mathematical models</subject><subject>Microorganisms</subject><subject>Nucleation</subject><subject>Nucleation and growth</subject><subject>RHEED</subject><subject>Surface layer</subject><subject>Texture</subject><issn>0168-583X</issn><issn>1872-9584</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><recordid>eNp9kE1LxDAQhoMouK7-AU85emlNmn6CF138ggVBFLyFNJlolrapSbrUf2_KenYYmMM878A8CF1SklJCy-tdOpi-TTNCaUpiZ-URWtG6ypKmqPNjtIpQnRQ1-zhFZ97vSKyCFSv0emfEbESHA8xhcoAV7KGzYw9DwGbA4QuwsQNuQfRYeG98ABWh0XoTloXVuBefA3gz9djORsE5OtGi83DxN9fo_eH-bfOUbF8enze320QyxkKSKSlaqjWpWMMorUlVKd20TSGhhFaVus3aGmhFWZGXudJC5YSCVpKKPKcE2BpdHe6Ozn5P4APvjZfQdWIAO3kexZA6KmjKiGYHVDrrvQPNR2d64X4itHAl3_FFIF8EchI7W0I3hxDEJ_YGHPfSwCBBGQcycGXNf_Ffm8d7AQ</recordid><startdate>20120201</startdate><enddate>20120201</enddate><creator>Groves, James R.</creator><creator>Hammond, Robert H.</creator><creator>Matias, Vladimir</creator><creator>DePaula, Raymond F.</creator><creator>Stan, Liliana</creator><creator>Clemens, Bruce M.</creator><general>Elsevier B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7U5</scope><scope>8FD</scope><scope>L7M</scope></search><sort><creationdate>20120201</creationdate><title>Biaxial texture development in the ion beam assisted deposition of magnesium oxide</title><author>Groves, James R. ; Hammond, Robert H. ; Matias, Vladimir ; DePaula, Raymond F. ; Stan, Liliana ; Clemens, Bruce M.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c333t-2dcab1ff07393118077df9b95ce6ebd6fb2b8e17135464dfad401efdc1a4410e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2012</creationdate><topic>Biaxial texture</topic><topic>Crystallography</topic><topic>Deposition</topic><topic>Ion beam assisted deposition</topic><topic>Magnesium oxide</topic><topic>Mathematical models</topic><topic>Microorganisms</topic><topic>Nucleation</topic><topic>Nucleation and growth</topic><topic>RHEED</topic><topic>Surface layer</topic><topic>Texture</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Groves, James R.</creatorcontrib><creatorcontrib>Hammond, Robert H.</creatorcontrib><creatorcontrib>Matias, Vladimir</creatorcontrib><creatorcontrib>DePaula, Raymond F.</creatorcontrib><creatorcontrib>Stan, Liliana</creatorcontrib><creatorcontrib>Clemens, Bruce M.</creatorcontrib><collection>CrossRef</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Groves, James R.</au><au>Hammond, Robert H.</au><au>Matias, Vladimir</au><au>DePaula, Raymond F.</au><au>Stan, Liliana</au><au>Clemens, Bruce M.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Biaxial texture development in the ion beam assisted deposition of magnesium oxide</atitle><jtitle>Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms</jtitle><date>2012-02-01</date><risdate>2012</risdate><volume>272</volume><spage>28</spage><epage>32</epage><pages>28-32</pages><issn>0168-583X</issn><eissn>1872-9584</eissn><abstract>Low-energy ion-beam irradiation (<1
keV) during the concurrent deposition of cubic oxide materials results in the growth of crystallographically textured thin films. A model system, magnesium oxide (MgO), has been successfully used as a biaxially textured template film for the heteroepitaxial deposition of many materials with texture dependent properties like high temperature superconductors, tunable microwave materials, and ferroelectrics. Here, we present data on the initial nucleation of biaxial crystallographic texture in this model system using an
in situ quartz crystal microbalance (QCM) substrate combined with
in situ reflected high-energy electron diffraction (RHEED). Correlation of mass uptake with the RHEED images of the growing surface shows that the development of crystallographic biaxial texture in this material system occurs suddenly as the initially polycrystalline MgO films reaches a critical film thickness of 2
nm. This texture continues to improve during subsequent growth. A simple model shows that the effect is not due simply to coverage effects. We use a combination of
in situ RHEED and
ex situ transmission electron microscopy to further elucidate the mechanism of this sudden texture formation. We present a physical model to describe this behavior and explain the role of ion-to-atom arrival ratio and underlying nucleation surface on texture development.</abstract><pub>Elsevier B.V</pub><doi>10.1016/j.nimb.2011.01.026</doi><tpages>5</tpages></addata></record> |
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subjects | Biaxial texture Crystallography Deposition Ion beam assisted deposition Magnesium oxide Mathematical models Microorganisms Nucleation Nucleation and growth RHEED Surface layer Texture |
title | Biaxial texture development in the ion beam assisted deposition of magnesium oxide |
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