Inkjet Printing of Nanoporous Gold Electrode Arrays on Cellulose Membranes for High-Sensitive Paper-Like Electrochemical Oxygen Sensors Using Ionic Liquid Electrolytes
A simple approach to the mass production of nanoporous gold electrode arrays on cellulose membranes for electrochemical sensing of oxygen using ionic liquid (IL) electrolytes was established. The approach, combining the inkjet printing of gold nanoparticle (GNP) patterns with the self-catalytic grow...
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| Veröffentlicht in: | Analytical chemistry (Washington) 2012-04, Vol.84 (8), p.3745-3750 |
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| creator | Hu, Chengguo Bai, Xiaoyun Wang, Yingkai Jin, Wei Zhang, Xuan Hu, Shengshui |
| description | A simple approach to the mass production of nanoporous gold electrode arrays on cellulose membranes for electrochemical sensing of oxygen using ionic liquid (IL) electrolytes was established. The approach, combining the inkjet printing of gold nanoparticle (GNP) patterns with the self-catalytic growth of these patterns into conducting layers, can fabricate hundreds of self-designed gold arrays on cellulose membranes within several hours using an inexpensive inkjet printer. The resulting paper-based gold electrode arrays (PGEAs) had several unique properties as thin-film sensor platforms, including good conductivity, excellent flexibility, high integration, and low cost. The porous nature of PGEAs also allowed the addition of electrolytes from the back cellulose membrane side and controllably produced large three-phase electrolyte/electrode/gas interfaces at the front electrode side. A novel paper-based solid-state electrochemical oxygen (O2) sensor was therefore developed using an IL electrolyte, 1-butyl-3-methylimidazolium hexafluorophosphate (BMIMPF6). The sensor looked like a piece of paper but possessed high sensitivity for O2 in a linear range from 0.054 to 0.177 v/v %, along with a low detection limit of 0.0075% and a short response time of less than 10 s, foreseeing its promising applications in developing cost-effective and environment-friendly paper-based electrochemical gas sensors. |
| doi_str_mv | 10.1021/ac3003243 |
| format | Article |
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The approach, combining the inkjet printing of gold nanoparticle (GNP) patterns with the self-catalytic growth of these patterns into conducting layers, can fabricate hundreds of self-designed gold arrays on cellulose membranes within several hours using an inexpensive inkjet printer. The resulting paper-based gold electrode arrays (PGEAs) had several unique properties as thin-film sensor platforms, including good conductivity, excellent flexibility, high integration, and low cost. The porous nature of PGEAs also allowed the addition of electrolytes from the back cellulose membrane side and controllably produced large three-phase electrolyte/electrode/gas interfaces at the front electrode side. A novel paper-based solid-state electrochemical oxygen (O2) sensor was therefore developed using an IL electrolyte, 1-butyl-3-methylimidazolium hexafluorophosphate (BMIMPF6). The sensor looked like a piece of paper but possessed high sensitivity for O2 in a linear range from 0.054 to 0.177 v/v %, along with a low detection limit of 0.0075% and a short response time of less than 10 s, foreseeing its promising applications in developing cost-effective and environment-friendly paper-based electrochemical gas sensors.</description><identifier>ISSN: 0003-2700</identifier><identifier>EISSN: 1520-6882</identifier><identifier>DOI: 10.1021/ac3003243</identifier><identifier>PMID: 22424097</identifier><identifier>CODEN: ANCHAM</identifier><language>eng</language><publisher>Washington, DC: American Chemical Society</publisher><subject>Analytical chemistry ; Applied sciences ; Cellulose ; Cellulose - chemistry ; Chemistry ; Electrochemical methods ; Electrodes ; Electrolytes ; Exact sciences and technology ; General, instrumentation ; Global environmental pollution ; Gold - chemistry ; Imidazoles - chemistry ; Ionic Liquids - chemistry ; Limit of Detection ; Metal Nanoparticles - chemistry ; Microarray Analysis ; Microscopy, Electron, Scanning ; Nanoparticles ; Oxygen ; Oxygen - chemistry ; Pollution ; Porosity ; Printing</subject><ispartof>Analytical chemistry (Washington), 2012-04, Vol.84 (8), p.3745-3750</ispartof><rights>Copyright © 2012 American Chemical Society</rights><rights>2015 INIST-CNRS</rights><rights>Copyright American Chemical Society Apr 17, 2012</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a439t-ad667960f5a7a7edf2cb0fe507c9fb004b4ef451c04979e6f019c0138eb7131a3</citedby><cites>FETCH-LOGICAL-a439t-ad667960f5a7a7edf2cb0fe507c9fb004b4ef451c04979e6f019c0138eb7131a3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/ac3003243$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/ac3003243$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,776,780,2752,27053,27901,27902,56713,56763</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=25812024$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/22424097$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Hu, Chengguo</creatorcontrib><creatorcontrib>Bai, Xiaoyun</creatorcontrib><creatorcontrib>Wang, Yingkai</creatorcontrib><creatorcontrib>Jin, Wei</creatorcontrib><creatorcontrib>Zhang, Xuan</creatorcontrib><creatorcontrib>Hu, Shengshui</creatorcontrib><title>Inkjet Printing of Nanoporous Gold Electrode Arrays on Cellulose Membranes for High-Sensitive Paper-Like Electrochemical Oxygen Sensors Using Ionic Liquid Electrolytes</title><title>Analytical chemistry (Washington)</title><addtitle>Anal. Chem</addtitle><description>A simple approach to the mass production of nanoporous gold electrode arrays on cellulose membranes for electrochemical sensing of oxygen using ionic liquid (IL) electrolytes was established. The approach, combining the inkjet printing of gold nanoparticle (GNP) patterns with the self-catalytic growth of these patterns into conducting layers, can fabricate hundreds of self-designed gold arrays on cellulose membranes within several hours using an inexpensive inkjet printer. The resulting paper-based gold electrode arrays (PGEAs) had several unique properties as thin-film sensor platforms, including good conductivity, excellent flexibility, high integration, and low cost. The porous nature of PGEAs also allowed the addition of electrolytes from the back cellulose membrane side and controllably produced large three-phase electrolyte/electrode/gas interfaces at the front electrode side. A novel paper-based solid-state electrochemical oxygen (O2) sensor was therefore developed using an IL electrolyte, 1-butyl-3-methylimidazolium hexafluorophosphate (BMIMPF6). The sensor looked like a piece of paper but possessed high sensitivity for O2 in a linear range from 0.054 to 0.177 v/v %, along with a low detection limit of 0.0075% and a short response time of less than 10 s, foreseeing its promising applications in developing cost-effective and environment-friendly paper-based electrochemical gas sensors.</description><subject>Analytical chemistry</subject><subject>Applied sciences</subject><subject>Cellulose</subject><subject>Cellulose - chemistry</subject><subject>Chemistry</subject><subject>Electrochemical methods</subject><subject>Electrodes</subject><subject>Electrolytes</subject><subject>Exact sciences and technology</subject><subject>General, instrumentation</subject><subject>Global environmental pollution</subject><subject>Gold - chemistry</subject><subject>Imidazoles - chemistry</subject><subject>Ionic Liquids - chemistry</subject><subject>Limit of Detection</subject><subject>Metal Nanoparticles - chemistry</subject><subject>Microarray Analysis</subject><subject>Microscopy, Electron, Scanning</subject><subject>Nanoparticles</subject><subject>Oxygen</subject><subject>Oxygen - chemistry</subject><subject>Pollution</subject><subject>Porosity</subject><subject>Printing</subject><issn>0003-2700</issn><issn>1520-6882</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNpd0d1q2zAUB3AxNtas68VeYAjGYLvwdiTZln1ZQj8C2VpYe21k-ShVakupZI_mifaaU2iajV4JxI__-SLkA4NvDDj7rrQAEDwXr8iMFRyysqr4azKD9JtxCXBE3sW4BmAMWPmWHHGe8xxqOSN_Fu5-jSO9DtaN1q2oN_Sncn7jg58ivfB9R8961GPwHdLTENQ2Uu_oHPt-6n1E-gOHNiiHkRof6KVd3WW_0EU72t9Ir9UGQ7a09_icou9wsFr19Opxu0JHd9aHSG_jrvrCO6vp0j5M9lC3344Y35M3RvURT_bvMbk9P7uZX2bLq4vF_HSZqVzUY6a6spR1CaZQUknsDNctGCxA6tq0AHmbo8kLpiGvZY2lAVZrYKLCVjLBlDgmX55yN8E_TBjHZrBRp2HThGkhDQPgBfBKyEQ_vaBrPwWXukuKsbwUQtRJfX1SOvgYA5pmE-ygwjahZne95nC9ZD_uE6d2wO4gn8-VwOc9UDHt0KS9axv_uaJiHFLSwSkd_-_qZcG_MiCulQ</recordid><startdate>20120417</startdate><enddate>20120417</enddate><creator>Hu, Chengguo</creator><creator>Bai, Xiaoyun</creator><creator>Wang, Yingkai</creator><creator>Jin, Wei</creator><creator>Zhang, Xuan</creator><creator>Hu, Shengshui</creator><general>American Chemical Society</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QF</scope><scope>7QO</scope><scope>7QQ</scope><scope>7SC</scope><scope>7SE</scope><scope>7SP</scope><scope>7SR</scope><scope>7TA</scope><scope>7TB</scope><scope>7TM</scope><scope>7U5</scope><scope>7U7</scope><scope>7U9</scope><scope>8BQ</scope><scope>8FD</scope><scope>C1K</scope><scope>F28</scope><scope>FR3</scope><scope>H8D</scope><scope>H8G</scope><scope>H94</scope><scope>JG9</scope><scope>JQ2</scope><scope>KR7</scope><scope>L7M</scope><scope>L~C</scope><scope>L~D</scope><scope>P64</scope><scope>7X8</scope></search><sort><creationdate>20120417</creationdate><title>Inkjet Printing of Nanoporous Gold Electrode Arrays on Cellulose Membranes for High-Sensitive Paper-Like Electrochemical Oxygen Sensors Using Ionic Liquid Electrolytes</title><author>Hu, Chengguo ; Bai, Xiaoyun ; Wang, Yingkai ; Jin, Wei ; Zhang, Xuan ; Hu, Shengshui</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a439t-ad667960f5a7a7edf2cb0fe507c9fb004b4ef451c04979e6f019c0138eb7131a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2012</creationdate><topic>Analytical chemistry</topic><topic>Applied sciences</topic><topic>Cellulose</topic><topic>Cellulose - chemistry</topic><topic>Chemistry</topic><topic>Electrochemical methods</topic><topic>Electrodes</topic><topic>Electrolytes</topic><topic>Exact sciences and technology</topic><topic>General, instrumentation</topic><topic>Global environmental pollution</topic><topic>Gold - chemistry</topic><topic>Imidazoles - chemistry</topic><topic>Ionic Liquids - chemistry</topic><topic>Limit of Detection</topic><topic>Metal Nanoparticles - chemistry</topic><topic>Microarray Analysis</topic><topic>Microscopy, Electron, Scanning</topic><topic>Nanoparticles</topic><topic>Oxygen</topic><topic>Oxygen - chemistry</topic><topic>Pollution</topic><topic>Porosity</topic><topic>Printing</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Hu, Chengguo</creatorcontrib><creatorcontrib>Bai, Xiaoyun</creatorcontrib><creatorcontrib>Wang, Yingkai</creatorcontrib><creatorcontrib>Jin, Wei</creatorcontrib><creatorcontrib>Zhang, Xuan</creatorcontrib><creatorcontrib>Hu, Shengshui</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Aluminium Industry Abstracts</collection><collection>Biotechnology Research Abstracts</collection><collection>Ceramic Abstracts</collection><collection>Computer and Information Systems Abstracts</collection><collection>Corrosion Abstracts</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Materials Business File</collection><collection>Mechanical & Transportation Engineering Abstracts</collection><collection>Nucleic Acids Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Virology and AIDS Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>Aerospace Database</collection><collection>Copper Technical Reference Library</collection><collection>AIDS and Cancer Research Abstracts</collection><collection>Materials Research Database</collection><collection>ProQuest Computer Science Collection</collection><collection>Civil Engineering Abstracts</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Computer and Information Systems Abstracts Academic</collection><collection>Computer and Information Systems Abstracts Professional</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>MEDLINE - Academic</collection><jtitle>Analytical chemistry (Washington)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Hu, Chengguo</au><au>Bai, Xiaoyun</au><au>Wang, Yingkai</au><au>Jin, Wei</au><au>Zhang, Xuan</au><au>Hu, Shengshui</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Inkjet Printing of Nanoporous Gold Electrode Arrays on Cellulose Membranes for High-Sensitive Paper-Like Electrochemical Oxygen Sensors Using Ionic Liquid Electrolytes</atitle><jtitle>Analytical chemistry (Washington)</jtitle><addtitle>Anal. Chem</addtitle><date>2012-04-17</date><risdate>2012</risdate><volume>84</volume><issue>8</issue><spage>3745</spage><epage>3750</epage><pages>3745-3750</pages><issn>0003-2700</issn><eissn>1520-6882</eissn><coden>ANCHAM</coden><abstract>A simple approach to the mass production of nanoporous gold electrode arrays on cellulose membranes for electrochemical sensing of oxygen using ionic liquid (IL) electrolytes was established. The approach, combining the inkjet printing of gold nanoparticle (GNP) patterns with the self-catalytic growth of these patterns into conducting layers, can fabricate hundreds of self-designed gold arrays on cellulose membranes within several hours using an inexpensive inkjet printer. The resulting paper-based gold electrode arrays (PGEAs) had several unique properties as thin-film sensor platforms, including good conductivity, excellent flexibility, high integration, and low cost. The porous nature of PGEAs also allowed the addition of electrolytes from the back cellulose membrane side and controllably produced large three-phase electrolyte/electrode/gas interfaces at the front electrode side. A novel paper-based solid-state electrochemical oxygen (O2) sensor was therefore developed using an IL electrolyte, 1-butyl-3-methylimidazolium hexafluorophosphate (BMIMPF6). The sensor looked like a piece of paper but possessed high sensitivity for O2 in a linear range from 0.054 to 0.177 v/v %, along with a low detection limit of 0.0075% and a short response time of less than 10 s, foreseeing its promising applications in developing cost-effective and environment-friendly paper-based electrochemical gas sensors.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><pmid>22424097</pmid><doi>10.1021/ac3003243</doi><tpages>6</tpages></addata></record> |
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| ispartof | Analytical chemistry (Washington), 2012-04, Vol.84 (8), p.3745-3750 |
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| subjects | Analytical chemistry Applied sciences Cellulose Cellulose - chemistry Chemistry Electrochemical methods Electrodes Electrolytes Exact sciences and technology General, instrumentation Global environmental pollution Gold - chemistry Imidazoles - chemistry Ionic Liquids - chemistry Limit of Detection Metal Nanoparticles - chemistry Microarray Analysis Microscopy, Electron, Scanning Nanoparticles Oxygen Oxygen - chemistry Pollution Porosity Printing |
| title | Inkjet Printing of Nanoporous Gold Electrode Arrays on Cellulose Membranes for High-Sensitive Paper-Like Electrochemical Oxygen Sensors Using Ionic Liquid Electrolytes |
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