Collective Asymmetric Synthesis of Thiosilvatins

Thiosilvatins are a family of biologically active sulfenylated diketopiperazine natural products. The first members were reported over 40 years ago, but total synthesis of a thiosilvatin has remained elusive. Here, we describe the first, collective, synthesis of the parent epidithiodiketopiperazine...

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Veröffentlicht in:	Angewandte Chemie 2024-12, Vol.136 (51), p.n/a
Hauptverfasser:	Liu, Jian, Ekberg, Robin, Koning, Nicolas R., Strand, Daniel
Format:	Artikel
Sprache:	eng
Schlagworte:	Absolute configuration Asymmetric synthesis Asymmetry Biological activity Chemical synthesis diastereoconvergent synthesis epidithiodiketopiperazines Natural products organocatalysis Sulfur total synthesis
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