Li4SnS4 Sulfide Composite Electrolyte for Improved Solid-State Lithium Batteries
In all-solid lithium metal batteries, sulfide electrolytes offer superior ion conductivity. Nevertheless, they also confront significant challenges, such as the formation of internal dendrites and instability in lithium and humid air. In order to overcome these issues, a sulfide composite electrolyt...
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| Veröffentlicht in: | Journal of electronic materials 2024-12, Vol.53 (12), p.7400-7408 |
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| creator | Zheng, Lihao Ren, Gaoya Wang, Shuai Yang, Yefeng |
| description | In all-solid lithium metal batteries, sulfide electrolytes offer superior ion conductivity. Nevertheless, they also confront significant challenges, such as the formation of internal dendrites and instability in lithium and humid air. In order to overcome these issues, a sulfide composite electrolyte has been prepared by mixing polyethylene oxide polymers with air-stable inorganic sulfide, Li
4
SnS
4
, which can achieve good chemical and electrochemical stability. Meanwhile, the introduced Li
4
SnS
4
can facilitate the movement of Li
+
ions in the composite electrolyte, which exhibits an elevated ion conductivity up to 2.55 × 10
−5
S cm
−1
.
Graphical Abstract |
| doi_str_mv | 10.1007/s11664-024-11467-1 |
| format | Article |
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4
SnS
4
, which can achieve good chemical and electrochemical stability. Meanwhile, the introduced Li
4
SnS
4
can facilitate the movement of Li
+
ions in the composite electrolyte, which exhibits an elevated ion conductivity up to 2.55 × 10
−5
S cm
−1
.
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4
SnS
4
, which can achieve good chemical and electrochemical stability. Meanwhile, the introduced Li
4
SnS
4
can facilitate the movement of Li
+
ions in the composite electrolyte, which exhibits an elevated ion conductivity up to 2.55 × 10
−5
S cm
−1
.
Graphical Abstract</description><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Electrodes</subject><subject>Electrolytes</subject><subject>Electronics and Microelectronics</subject><subject>Energy</subject><subject>Flexibility</subject><subject>High-Energy Battery Materials</subject><subject>Instrumentation</subject><subject>Lithium</subject><subject>Lithium batteries</subject><subject>Lithium ions</subject><subject>Materials Science</subject><subject>Membranes</subject><subject>Molten salt electrolytes</subject><subject>Optical and Electronic Materials</subject><subject>Polyethylene oxide</subject><subject>Polymers</subject><subject>Solid electrolytes</subject><subject>Solid State Physics</subject><subject>Temperature</subject><subject>Topical Collection: High-Energy Battery Materials</subject><issn>0361-5235</issn><issn>1543-186X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kE9LxDAQxYMouK5-AU8Fz9FM86fpUZdVFwoK3YO3kG0TzdJu1yQV9tubtYI3LzMD896b4YfQNZBbIKS4CwBCMExyhgGYKDCcoBlwRjFI8XaKZoQKwDyn_BxdhLAlBDhImKHXyrF6V7OsHjvrWpMthn4_BBdNtuxME_3QHdJsB5-t-r0fvkyb1UPnWlxHnRaVix9u7LMHHaPxzoRLdGZ1F8zVb5-j9eNyvXjG1cvTanFf4SYnJGLZ6pYTbWVRyFRkWQhJNbCNKZmwZVG2tJSc51rn1gpjG8vNRtLSaKZ5saFzdDPFpp8-RxOi2g6j36WLigKFBKLIIanySdX4IQRvrNp712t_UEDUEZyawKmkVz_g1NFEJ1NI4t278X_R_7i-AUvacJQ</recordid><startdate>20241201</startdate><enddate>20241201</enddate><creator>Zheng, Lihao</creator><creator>Ren, Gaoya</creator><creator>Wang, Shuai</creator><creator>Yang, Yefeng</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-1438-9307</orcidid></search><sort><creationdate>20241201</creationdate><title>Li4SnS4 Sulfide Composite Electrolyte for Improved Solid-State Lithium Batteries</title><author>Zheng, Lihao ; Ren, Gaoya ; Wang, Shuai ; Yang, Yefeng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c200t-8dad50af8778f87897683a14be946f979d398552aa2ff6efcf5eb839ea4a57b3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Electrodes</topic><topic>Electrolytes</topic><topic>Electronics and Microelectronics</topic><topic>Energy</topic><topic>Flexibility</topic><topic>High-Energy Battery Materials</topic><topic>Instrumentation</topic><topic>Lithium</topic><topic>Lithium batteries</topic><topic>Lithium ions</topic><topic>Materials Science</topic><topic>Membranes</topic><topic>Molten salt electrolytes</topic><topic>Optical and Electronic Materials</topic><topic>Polyethylene oxide</topic><topic>Polymers</topic><topic>Solid electrolytes</topic><topic>Solid State Physics</topic><topic>Temperature</topic><topic>Topical Collection: High-Energy Battery Materials</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zheng, Lihao</creatorcontrib><creatorcontrib>Ren, Gaoya</creatorcontrib><creatorcontrib>Wang, Shuai</creatorcontrib><creatorcontrib>Yang, Yefeng</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of electronic materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zheng, Lihao</au><au>Ren, Gaoya</au><au>Wang, Shuai</au><au>Yang, Yefeng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Li4SnS4 Sulfide Composite Electrolyte for Improved Solid-State Lithium Batteries</atitle><jtitle>Journal of electronic materials</jtitle><stitle>J. Electron. Mater</stitle><date>2024-12-01</date><risdate>2024</risdate><volume>53</volume><issue>12</issue><spage>7400</spage><epage>7408</epage><pages>7400-7408</pages><issn>0361-5235</issn><eissn>1543-186X</eissn><abstract>In all-solid lithium metal batteries, sulfide electrolytes offer superior ion conductivity. Nevertheless, they also confront significant challenges, such as the formation of internal dendrites and instability in lithium and humid air. In order to overcome these issues, a sulfide composite electrolyte has been prepared by mixing polyethylene oxide polymers with air-stable inorganic sulfide, Li
4
SnS
4
, which can achieve good chemical and electrochemical stability. Meanwhile, the introduced Li
4
SnS
4
can facilitate the movement of Li
+
ions in the composite electrolyte, which exhibits an elevated ion conductivity up to 2.55 × 10
−5
S cm
−1
.
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| subjects | Characterization and Evaluation of Materials Chemistry and Materials Science Electrodes Electrolytes Electronics and Microelectronics Energy Flexibility High-Energy Battery Materials Instrumentation Lithium Lithium batteries Lithium ions Materials Science Membranes Molten salt electrolytes Optical and Electronic Materials Polyethylene oxide Polymers Solid electrolytes Solid State Physics Temperature Topical Collection: High-Energy Battery Materials |
| title | Li4SnS4 Sulfide Composite Electrolyte for Improved Solid-State Lithium Batteries |
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