Review of iodine behavior from nuclear fuel dissolution to environmental release

During nuclear fuel reprocessing, radioiodine, can be released. The speciation of iodine drives its volatility, and partitioning processes are highly variable because they depend on facility operating conditions. Starting from iodine behavior in the fuel and progressing to its behavior in the enviro...

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Veröffentlicht in:RSC advances 2024-11, Vol.14 (48), p.35255-35274
Hauptverfasser: Beck, Chelsie L, Cervantes, Juan, Chiswell, Steven, Greaney, Allison T, Johnson, Katherine R, Levitskaia, Tatiana G, Martin, Leigh R, McDaniel, Gavin, Noble, Stephen, Rakos, Jason M, Riley, Brian J, Ritzmann, Andrew, Tingey, Joel M
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container_end_page 35274
container_issue 48
container_start_page 35255
container_title RSC advances
container_volume 14
creator Beck, Chelsie L
Cervantes, Juan
Chiswell, Steven
Greaney, Allison T
Johnson, Katherine R
Levitskaia, Tatiana G
Martin, Leigh R
McDaniel, Gavin
Noble, Stephen
Rakos, Jason M
Riley, Brian J
Ritzmann, Andrew
Tingey, Joel M
description During nuclear fuel reprocessing, radioiodine, can be released. The speciation of iodine drives its volatility, and partitioning processes are highly variable because they depend on facility operating conditions. Starting from iodine behavior in the fuel and progressing to its behavior in the environment, this review article describes the current understanding of iodine partitioning during aqueous fuel reprocessing. This review outlines knowledge gaps and describes the effects of state-of-the-art reprocessing techniques on iodine speciation and volatility. Whereas many review articles have described iodine behavior during specific reprocessing steps, this review provides a holistic overview of radioiodine, from the forms of iodine in different types of irradiated fuel to the forms of iodine released into the environment. The resultant behavior of radioiodine compared with stable iodine in the environment is also described. During nuclear fuel reprocessing, radioiodine, can be released.
doi_str_mv 10.1039/d4ra06494a
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subjects Iodine 131
NUCLEAR FUEL CYCLE AND FUEL MATERIALS
Nuclear fuel reprocessing
Partitioning
Speciation
State-of-the-art reviews
Volatility
title Review of iodine behavior from nuclear fuel dissolution to environmental release
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