Natural Isotopic Activity Ratios as Evidence of Migration and Leaching of Uranium in Egyptian Granitic Rocks

Gamma-spectrometry was utilized to analyse radionuclides in granitic rocks from the El Eridiya area through radiometric measurements. The activity concentration of 238 U ranges from 3493±83 to 5209±104 Bq kg −1 , while for 234 U and its isotope ( 235 U), it varies from 957±32 to 1012±34 Bq kg −1 and...

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Veröffentlicht in:Journal of physics. Conference series 2024-09, Vol.2830 (1), p.12022
Hauptverfasser: Ismaiel, Nahla A., Frag, Eman Y., Seif, W. M., Mira, Hamed I., Shabasy, Ahmed M., Khattab, Mahmoud R.
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container_start_page 12022
container_title Journal of physics. Conference series
container_volume 2830
creator Ismaiel, Nahla A.
Frag, Eman Y.
Seif, W. M.
Mira, Hamed I.
Shabasy, Ahmed M.
Khattab, Mahmoud R.
description Gamma-spectrometry was utilized to analyse radionuclides in granitic rocks from the El Eridiya area through radiometric measurements. The activity concentration of 238 U ranges from 3493±83 to 5209±104 Bq kg −1 , while for 234 U and its isotope ( 235 U), it varies from 957±32 to 1012±34 Bq kg −1 and 153.0±4.5 to 256.0±5.5 Bq kg −1 , respectively. However, for the isotopes 230 Th and 232 Th, the range is from 11217±254 to 16291±305 Bq kg −1 and 31.0±1.1 to 85.3±0.5 Bq kg −1 , respectively. The activity concentration of 40K ranged from 67.9±1.6 to 109.0±2.1 Bq kg −1 . The ratios of 234 U/ 238 U in the studied granitic rock samples vary from 0.21±0.01 to 0.54±0.03. Due to the current oxidising conditions, most of the rock samples show a higher presence of 234 U compared to 238 U, with 234 U/ 238 U activity ratios below one. Additionally, the activity ratios of 232 Th/ 238 U range from 0.006 to 0.019 in the granitic rock samples from the El Eridiya area. Figures 3 and 4 display uranium enrichment, with all samples showing 232 Th/ 238 U ratios below one for the earth’s crust. Additionally, all samples showed 230 Th/ 238 U and 230 Th/ 234 U activity levels above one, suggesting preferential leaching of uranium in an oxygen-rich setting. Similarly, the 234 U/ 238 U and 230 Th/2 38 U activity ratios are below and above one, indicating U-leaching and U-accumulation, respectively. Figure 3 and 4 show uranium enrichment, with all samples having 232 Th/ 238 U activity ratios below one for the earth’s crust. There were benefits to uranium leaching in an environment with oxidation in all samples, with 230 Th/ 238 U and 230 Th/ 234 U activity ratios exceeding one. If the 234 U/ 238 U activity ratio is lower than one but the 230 Th/ 238 U activity ratio is higher than 1, it suggests U-leaching; if the 234 U/ 238 U activity ratio is greater than one and the 230 Th/ 238 U activity ratio is less than 1, it suggests U-accumulation.
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M. ; Mira, Hamed I. ; Shabasy, Ahmed M. ; Khattab, Mahmoud R.</creator><creatorcontrib>Ismaiel, Nahla A. ; Frag, Eman Y. ; Seif, W. M. ; Mira, Hamed I. ; Shabasy, Ahmed M. ; Khattab, Mahmoud R.</creatorcontrib><description>Gamma-spectrometry was utilized to analyse radionuclides in granitic rocks from the El Eridiya area through radiometric measurements. The activity concentration of 238 U ranges from 3493±83 to 5209±104 Bq kg −1 , while for 234 U and its isotope ( 235 U), it varies from 957±32 to 1012±34 Bq kg −1 and 153.0±4.5 to 256.0±5.5 Bq kg −1 , respectively. However, for the isotopes 230 Th and 232 Th, the range is from 11217±254 to 16291±305 Bq kg −1 and 31.0±1.1 to 85.3±0.5 Bq kg −1 , respectively. The activity concentration of 40K ranged from 67.9±1.6 to 109.0±2.1 Bq kg −1 . The ratios of 234 U/ 238 U in the studied granitic rock samples vary from 0.21±0.01 to 0.54±0.03. Due to the current oxidising conditions, most of the rock samples show a higher presence of 234 U compared to 238 U, with 234 U/ 238 U activity ratios below one. Additionally, the activity ratios of 232 Th/ 238 U range from 0.006 to 0.019 in the granitic rock samples from the El Eridiya area. Figures 3 and 4 display uranium enrichment, with all samples showing 232 Th/ 238 U ratios below one for the earth’s crust. Additionally, all samples showed 230 Th/ 238 U and 230 Th/ 234 U activity levels above one, suggesting preferential leaching of uranium in an oxygen-rich setting. Similarly, the 234 U/ 238 U and 230 Th/2 38 U activity ratios are below and above one, indicating U-leaching and U-accumulation, respectively. Figure 3 and 4 show uranium enrichment, with all samples having 232 Th/ 238 U activity ratios below one for the earth’s crust. There were benefits to uranium leaching in an environment with oxidation in all samples, with 230 Th/ 238 U and 230 Th/ 234 U activity ratios exceeding one. If the 234 U/ 238 U activity ratio is lower than one but the 230 Th/ 238 U activity ratio is higher than 1, it suggests U-leaching; if the 234 U/ 238 U activity ratio is greater than one and the 230 Th/ 238 U activity ratio is less than 1, it suggests U-accumulation.</description><identifier>ISSN: 1742-6588</identifier><identifier>EISSN: 1742-6596</identifier><identifier>DOI: 10.1088/1742-6596/2830/1/012022</identifier><language>eng</language><publisher>Bristol: IOP Publishing</publisher><subject>Accumulation ; Earth ; Earth crust ; Granites ; Isotopes ; Leaching ; Migration ; Oxidation ; Radioactivity ; Radioisotopes ; Radionuclides ; Ratios ; Rocks ; Thorium isotopes ; Uranium ; Uranium 234 ; Uranium 238</subject><ispartof>Journal of physics. 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M.</creatorcontrib><creatorcontrib>Mira, Hamed I.</creatorcontrib><creatorcontrib>Shabasy, Ahmed M.</creatorcontrib><creatorcontrib>Khattab, Mahmoud R.</creatorcontrib><title>Natural Isotopic Activity Ratios as Evidence of Migration and Leaching of Uranium in Egyptian Granitic Rocks</title><title>Journal of physics. Conference series</title><addtitle>J. Phys.: Conf. Ser</addtitle><description>Gamma-spectrometry was utilized to analyse radionuclides in granitic rocks from the El Eridiya area through radiometric measurements. The activity concentration of 238 U ranges from 3493±83 to 5209±104 Bq kg −1 , while for 234 U and its isotope ( 235 U), it varies from 957±32 to 1012±34 Bq kg −1 and 153.0±4.5 to 256.0±5.5 Bq kg −1 , respectively. However, for the isotopes 230 Th and 232 Th, the range is from 11217±254 to 16291±305 Bq kg −1 and 31.0±1.1 to 85.3±0.5 Bq kg −1 , respectively. The activity concentration of 40K ranged from 67.9±1.6 to 109.0±2.1 Bq kg −1 . The ratios of 234 U/ 238 U in the studied granitic rock samples vary from 0.21±0.01 to 0.54±0.03. Due to the current oxidising conditions, most of the rock samples show a higher presence of 234 U compared to 238 U, with 234 U/ 238 U activity ratios below one. Additionally, the activity ratios of 232 Th/ 238 U range from 0.006 to 0.019 in the granitic rock samples from the El Eridiya area. Figures 3 and 4 display uranium enrichment, with all samples showing 232 Th/ 238 U ratios below one for the earth’s crust. Additionally, all samples showed 230 Th/ 238 U and 230 Th/ 234 U activity levels above one, suggesting preferential leaching of uranium in an oxygen-rich setting. Similarly, the 234 U/ 238 U and 230 Th/2 38 U activity ratios are below and above one, indicating U-leaching and U-accumulation, respectively. Figure 3 and 4 show uranium enrichment, with all samples having 232 Th/ 238 U activity ratios below one for the earth’s crust. 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The activity concentration of 238 U ranges from 3493±83 to 5209±104 Bq kg −1 , while for 234 U and its isotope ( 235 U), it varies from 957±32 to 1012±34 Bq kg −1 and 153.0±4.5 to 256.0±5.5 Bq kg −1 , respectively. However, for the isotopes 230 Th and 232 Th, the range is from 11217±254 to 16291±305 Bq kg −1 and 31.0±1.1 to 85.3±0.5 Bq kg −1 , respectively. The activity concentration of 40K ranged from 67.9±1.6 to 109.0±2.1 Bq kg −1 . The ratios of 234 U/ 238 U in the studied granitic rock samples vary from 0.21±0.01 to 0.54±0.03. Due to the current oxidising conditions, most of the rock samples show a higher presence of 234 U compared to 238 U, with 234 U/ 238 U activity ratios below one. Additionally, the activity ratios of 232 Th/ 238 U range from 0.006 to 0.019 in the granitic rock samples from the El Eridiya area. Figures 3 and 4 display uranium enrichment, with all samples showing 232 Th/ 238 U ratios below one for the earth’s crust. Additionally, all samples showed 230 Th/ 238 U and 230 Th/ 234 U activity levels above one, suggesting preferential leaching of uranium in an oxygen-rich setting. Similarly, the 234 U/ 238 U and 230 Th/2 38 U activity ratios are below and above one, indicating U-leaching and U-accumulation, respectively. Figure 3 and 4 show uranium enrichment, with all samples having 232 Th/ 238 U activity ratios below one for the earth’s crust. There were benefits to uranium leaching in an environment with oxidation in all samples, with 230 Th/ 238 U and 230 Th/ 234 U activity ratios exceeding one. If the 234 U/ 238 U activity ratio is lower than one but the 230 Th/ 238 U activity ratio is higher than 1, it suggests U-leaching; if the 234 U/ 238 U activity ratio is greater than one and the 230 Th/ 238 U activity ratio is less than 1, it suggests U-accumulation.</abstract><cop>Bristol</cop><pub>IOP Publishing</pub><doi>10.1088/1742-6596/2830/1/012022</doi><tpages>9</tpages><oa>free_for_read</oa></addata></record>
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subjects Accumulation
Earth
Earth crust
Granites
Isotopes
Leaching
Migration
Oxidation
Radioactivity
Radioisotopes
Radionuclides
Ratios
Rocks
Thorium isotopes
Uranium
Uranium 234
Uranium 238
title Natural Isotopic Activity Ratios as Evidence of Migration and Leaching of Uranium in Egyptian Granitic Rocks
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