Pendant Proton‐Relays Systematically Tune the Rate and Selectivity of Electrocatalytic Ammonia Generation in a Fe‐Porphyrin Based Metal–Organic Framework

Electrocatalytic nitrite reduction (eNO2RR) is a promising alternative route to produce ammonia (NH3). Until now, several molecular catalysts have shown capability to homogeneously reduce nitrite to NH3, while taking advantage of added secondary‐sphere functionalities to direct catalytic performance...

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Veröffentlicht in:	Angewandte Chemie 2024-09, Vol.136 (37), p.n/a
Hauptverfasser:	Ghatak, Arnab, Shanker, G. Shiva, Sappati, Subrahmanyam, Liberman, Itamar, Shimoni, Ran, Hod, Idan
Format:	Artikel
Sprache:	eng
Schlagworte:	Ammonia Catalysts Catalytic activity Electrocatalytic nitrite reduction (eNO2RR) Electrochemistry Fe-porphyrin Iron Metal-organic frameworks Metal–Organic Framework (MOF) Porphyrins Proton relay Protons Relaying Second sphere
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