Investigation of radiation effects on structural, morphological, and compositional properties of WO3 nanostructures for water splitting applications
Gamma radiation can cause structural defects in metal oxide thin films, affecting their conversion efficiency. This study focuses on synthesizing and characterizing Tungsten oxide (WO 3 ) films for photo-electrochemical (PEC) water-splitting applications. The pristine WO 3 film was irradiated with a...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2024, Vol.333 (8), p.4421-4432 |
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| container_title | Journal of radioanalytical and nuclear chemistry |
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| creator | Pande, Sukhada S. Kakade, Prashant M. Kachere, Avinash R. Shinde, Pratibha S. Kolhe, Pankaj S. Sonawane, Kishor M. Ruz, Priyanka Sudarshan, V. Dhole, Sanjay D. Jadkar, Sandesh R. Sharma, Rajendrakumar Mandlik, Nandkumar T. |
| description | Gamma radiation can cause structural defects in metal oxide thin films, affecting their conversion efficiency. This study focuses on synthesizing and characterizing Tungsten oxide (WO
3
) films for photo-electrochemical (PEC) water-splitting applications. The pristine WO
3
film was irradiated with a Co-60 gamma source to improve its photocatalytic activity and was named G-WO
3
. The resulting G-WO
3
thin films showed a decrease in the optical direct band gap and showed higher photocurrent density and lower charge transfer resistance for PEC applications. The carrier charge density (
N
d
) values were found to be increased after γ-radiation. The synthesized G-WO
3
thin films possess good stability and reusability for photo-electrochemical water-splitting applications. |
| doi_str_mv | 10.1007/s10967-024-09520-8 |
| format | Article |
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3
) films for photo-electrochemical (PEC) water-splitting applications. The pristine WO
3
film was irradiated with a Co-60 gamma source to improve its photocatalytic activity and was named G-WO
3
. The resulting G-WO
3
thin films showed a decrease in the optical direct band gap and showed higher photocurrent density and lower charge transfer resistance for PEC applications. The carrier charge density (
N
d
) values were found to be increased after γ-radiation. The synthesized G-WO
3
thin films possess good stability and reusability for photo-electrochemical water-splitting applications.</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-024-09520-8</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Carrier density ; Catalytic activity ; Charge density ; Charge transfer ; Chemistry ; Chemistry and Materials Science ; Current carriers ; Diagnostic Radiology ; Gamma rays ; Hadrons ; Heavy Ions ; Inorganic Chemistry ; Metal oxides ; Nuclear Chemistry ; Nuclear Physics ; Photocatalysis ; Photoelectric effect ; Physical Chemistry ; Radiation effects ; Synthesis ; Thin films ; Tungsten oxides ; Water splitting</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2024, Vol.333 (8), p.4421-4432</ispartof><rights>Akadémiai Kiadó, Budapest, Hungary 2024. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c270t-801daf375025ac053a33bdef0c57dc17b52bbd5cdda22ce2b7278c425302c2cc3</cites><orcidid>0000-0002-1678-2620</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-024-09520-8$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-024-09520-8$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27903,27904,41467,42536,51298</link.rule.ids></links><search><creatorcontrib>Pande, Sukhada S.</creatorcontrib><creatorcontrib>Kakade, Prashant M.</creatorcontrib><creatorcontrib>Kachere, Avinash R.</creatorcontrib><creatorcontrib>Shinde, Pratibha S.</creatorcontrib><creatorcontrib>Kolhe, Pankaj S.</creatorcontrib><creatorcontrib>Sonawane, Kishor M.</creatorcontrib><creatorcontrib>Ruz, Priyanka</creatorcontrib><creatorcontrib>Sudarshan, V.</creatorcontrib><creatorcontrib>Dhole, Sanjay D.</creatorcontrib><creatorcontrib>Jadkar, Sandesh R.</creatorcontrib><creatorcontrib>Sharma, Rajendrakumar</creatorcontrib><creatorcontrib>Mandlik, Nandkumar T.</creatorcontrib><title>Investigation of radiation effects on structural, morphological, and compositional properties of WO3 nanostructures for water splitting applications</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>Gamma radiation can cause structural defects in metal oxide thin films, affecting their conversion efficiency. This study focuses on synthesizing and characterizing Tungsten oxide (WO
3
) films for photo-electrochemical (PEC) water-splitting applications. The pristine WO
3
film was irradiated with a Co-60 gamma source to improve its photocatalytic activity and was named G-WO
3
. The resulting G-WO
3
thin films showed a decrease in the optical direct band gap and showed higher photocurrent density and lower charge transfer resistance for PEC applications. The carrier charge density (
N
d
) values were found to be increased after γ-radiation. The synthesized G-WO
3
thin films possess good stability and reusability for photo-electrochemical water-splitting applications.</description><subject>Carrier density</subject><subject>Catalytic activity</subject><subject>Charge density</subject><subject>Charge transfer</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Current carriers</subject><subject>Diagnostic Radiology</subject><subject>Gamma rays</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>Inorganic Chemistry</subject><subject>Metal oxides</subject><subject>Nuclear Chemistry</subject><subject>Nuclear Physics</subject><subject>Photocatalysis</subject><subject>Photoelectric effect</subject><subject>Physical Chemistry</subject><subject>Radiation effects</subject><subject>Synthesis</subject><subject>Thin films</subject><subject>Tungsten oxides</subject><subject>Water splitting</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kM9OxCAQxonRxHX1BTyReLU6wFK6R7PxzyYme9F4JJTSyqZbKlCN7-EDS7cab55mhnzfN8wPoXMCVwRAXAcCy1xkQBcZLDmFrDhAM8KLIqOigEM0A8ryjAtGjtFJCFsAWBYFm6GvdfduQrSNitZ12NXYq8pOg6lro2PAqQ3RDzoOXrWXeOd8_-pa11g9jqqrsHa73gU7ulSLe-9646M1Ycx72TDcqc79RqTX2nn8oaLxOPStjdF2DVZ9avV-cThFR7Vqgzn7qXP0fHf7tHrIHjf369XNY6apgJgVQCpVM8GBcqWBM8VYWZkaNBeVJqLktCwrrqtKUaoNLUWCoReUM6Caas3m6GLKTT9-GxIGuXWDTycEyRLPPAdgJKnopNLeheBNLXtvd8p_SgJypC8n-jLRl3v6skgmNplCEneN8X_R_7i-ARtBjLo</recordid><startdate>2024</startdate><enddate>2024</enddate><creator>Pande, Sukhada S.</creator><creator>Kakade, Prashant M.</creator><creator>Kachere, Avinash R.</creator><creator>Shinde, Pratibha S.</creator><creator>Kolhe, Pankaj S.</creator><creator>Sonawane, Kishor M.</creator><creator>Ruz, Priyanka</creator><creator>Sudarshan, V.</creator><creator>Dhole, Sanjay D.</creator><creator>Jadkar, Sandesh R.</creator><creator>Sharma, Rajendrakumar</creator><creator>Mandlik, Nandkumar T.</creator><general>Springer International Publishing</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-1678-2620</orcidid></search><sort><creationdate>2024</creationdate><title>Investigation of radiation effects on structural, morphological, and compositional properties of WO3 nanostructures for water splitting applications</title><author>Pande, Sukhada S. ; Kakade, Prashant M. ; Kachere, Avinash R. ; Shinde, Pratibha S. ; Kolhe, Pankaj S. ; Sonawane, Kishor M. ; Ruz, Priyanka ; Sudarshan, V. ; Dhole, Sanjay D. ; Jadkar, Sandesh R. ; Sharma, Rajendrakumar ; Mandlik, Nandkumar T.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c270t-801daf375025ac053a33bdef0c57dc17b52bbd5cdda22ce2b7278c425302c2cc3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Carrier density</topic><topic>Catalytic activity</topic><topic>Charge density</topic><topic>Charge transfer</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Current carriers</topic><topic>Diagnostic Radiology</topic><topic>Gamma rays</topic><topic>Hadrons</topic><topic>Heavy Ions</topic><topic>Inorganic Chemistry</topic><topic>Metal oxides</topic><topic>Nuclear Chemistry</topic><topic>Nuclear Physics</topic><topic>Photocatalysis</topic><topic>Photoelectric effect</topic><topic>Physical Chemistry</topic><topic>Radiation effects</topic><topic>Synthesis</topic><topic>Thin films</topic><topic>Tungsten oxides</topic><topic>Water splitting</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Pande, Sukhada S.</creatorcontrib><creatorcontrib>Kakade, Prashant M.</creatorcontrib><creatorcontrib>Kachere, Avinash R.</creatorcontrib><creatorcontrib>Shinde, Pratibha S.</creatorcontrib><creatorcontrib>Kolhe, Pankaj S.</creatorcontrib><creatorcontrib>Sonawane, Kishor M.</creatorcontrib><creatorcontrib>Ruz, Priyanka</creatorcontrib><creatorcontrib>Sudarshan, V.</creatorcontrib><creatorcontrib>Dhole, Sanjay D.</creatorcontrib><creatorcontrib>Jadkar, Sandesh R.</creatorcontrib><creatorcontrib>Sharma, Rajendrakumar</creatorcontrib><creatorcontrib>Mandlik, Nandkumar T.</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Pande, Sukhada S.</au><au>Kakade, Prashant M.</au><au>Kachere, Avinash R.</au><au>Shinde, Pratibha S.</au><au>Kolhe, Pankaj S.</au><au>Sonawane, Kishor M.</au><au>Ruz, Priyanka</au><au>Sudarshan, V.</au><au>Dhole, Sanjay D.</au><au>Jadkar, Sandesh R.</au><au>Sharma, Rajendrakumar</au><au>Mandlik, Nandkumar T.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Investigation of radiation effects on structural, morphological, and compositional properties of WO3 nanostructures for water splitting applications</atitle><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle><stitle>J Radioanal Nucl Chem</stitle><date>2024</date><risdate>2024</risdate><volume>333</volume><issue>8</issue><spage>4421</spage><epage>4432</epage><pages>4421-4432</pages><issn>0236-5731</issn><eissn>1588-2780</eissn><abstract>Gamma radiation can cause structural defects in metal oxide thin films, affecting their conversion efficiency. This study focuses on synthesizing and characterizing Tungsten oxide (WO
3
) films for photo-electrochemical (PEC) water-splitting applications. The pristine WO
3
film was irradiated with a Co-60 gamma source to improve its photocatalytic activity and was named G-WO
3
. The resulting G-WO
3
thin films showed a decrease in the optical direct band gap and showed higher photocurrent density and lower charge transfer resistance for PEC applications. The carrier charge density (
N
d
) values were found to be increased after γ-radiation. The synthesized G-WO
3
thin films possess good stability and reusability for photo-electrochemical water-splitting applications.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s10967-024-09520-8</doi><tpages>12</tpages><orcidid>https://orcid.org/0000-0002-1678-2620</orcidid></addata></record> |
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| subjects | Carrier density Catalytic activity Charge density Charge transfer Chemistry Chemistry and Materials Science Current carriers Diagnostic Radiology Gamma rays Hadrons Heavy Ions Inorganic Chemistry Metal oxides Nuclear Chemistry Nuclear Physics Photocatalysis Photoelectric effect Physical Chemistry Radiation effects Synthesis Thin films Tungsten oxides Water splitting |
| title | Investigation of radiation effects on structural, morphological, and compositional properties of WO3 nanostructures for water splitting applications |
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