Polydopamine-modified cellulose nanofiber composite hydrogel with strong toughness and high adhesion for human motion detection and wireless sensing

The toughness and adhesiveness of composite hydrogels play an important role in the field of wearable sensors, where they are used due to their remarkable flexibility and diverse specialized properties. In this work, a composite hydrogel with strong toughness and high adhesion for human motion detec...

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Veröffentlicht in:Cellulose (London) 2024-07, Vol.31 (10), p.6421-6433
Hauptverfasser: Du, Hong, Cheng, Zhengbai, Liu, Yingying, Hu, Mengxin, Xia, Mingfeng, Sun, Xianhao, Lin, Zhaoyun, Liu, Hongbin
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container_end_page 6433
container_issue 10
container_start_page 6421
container_title Cellulose (London)
container_volume 31
creator Du, Hong
Cheng, Zhengbai
Liu, Yingying
Hu, Mengxin
Xia, Mingfeng
Sun, Xianhao
Lin, Zhaoyun
Liu, Hongbin
description The toughness and adhesiveness of composite hydrogels play an important role in the field of wearable sensors, where they are used due to their remarkable flexibility and diverse specialized properties. In this work, a composite hydrogel with strong toughness and high adhesion for human motion detection and wireless sensing was obtained. Polydopamine (PDA)-modified cellulose nanofibers (PCNFs) were introduced into a polyvinyl alcohol (PVA) and polyacrylamide (PAM) network, resulting in the fabrication of a PCNF/PVA-PAM composite hydrogel. Lithium chloride served as a crosslinking agent and provided conductive ions, and the PCNFs provided the composite hydrogel with strong toughness and adhesion abilities. The compression strength of the obtained PCNF/PVA-PAM composite hydrogel was 1.1 MPa, and its adhesion strength to glass was 63.8 kPa. Moreover, the composite hydrogel exhibited good anti-freezing properties. The compression sensitivity of the composite hydrogel was 1.29, and it still maintained stability even after 500 testing cycles. The strain-sensing abilities of the composite hydrogel were satisfactory for different human body parts. This composite material holds great promise in the fields of wearable devices and wireless signal transmission.
doi_str_mv 10.1007/s10570-024-05969-8
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subjects adhesion
Adhesive strength
Adhesive wear
Bioorganic Chemistry
Body parts
Cellulose
Cellulose fibers
cellulose nanofibers
Ceramics
Chemistry
Chemistry and Materials Science
Composite materials
Composites
compression strength
Compressive strength
cross-linking reagents
Crosslinking
Freezing
Glass
Human motion
Human performance
humans
Hydrogels
Lithium chloride
Motion perception
Nanofibers
Natural Materials
Organic Chemistry
Original Research
Physical Chemistry
Polyacrylamide
Polymer Sciences
Polyvinyl alcohol
Signal transmission
Sustainable Development
Toughness
Wearable technology
title Polydopamine-modified cellulose nanofiber composite hydrogel with strong toughness and high adhesion for human motion detection and wireless sensing
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