Perylene with peripherally fused pyrrole and pyridine: columnar packing, anti-Kasha dual emission and reactive oxygen species generation
Simultaneously fusing pyrrole and pyridine at perylene's opposite edges is facilely achieved in this work, yielding PerNN and its various derivatives. All targets demonstrate global diamagnetic ring current. Benefiting from a spatially separated donor-acceptor group within one planar skeleton,...
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| Veröffentlicht in: | New journal of chemistry 2024-05, Vol.48 (2), p.914-919 |
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| container_issue | 2 |
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| container_title | New journal of chemistry |
| container_volume | 48 |
| creator | Cao, Jing Zhang, Wenhao Ding, Yeda Zhang, Xuejin Zhang, Yuanyuan Qiao, Dan Biao, Shumin Dong, Xuefei Song, Jiayi Dai, Gaole Zhao, Ruiguo Wang, Qing |
| description | Simultaneously fusing pyrrole and pyridine at perylene's opposite edges is facilely achieved in this work, yielding
PerNN
and its various derivatives. All targets demonstrate global diamagnetic ring current. Benefiting from a spatially separated donor-acceptor group within one planar skeleton,
PerNN
exhibits efficient narrow blue emission and columnar stacking. More importantly, its alkylated derivatives
PerNN-MeCl
and
PerNN-MeI
display anti-Kasha dual emission responsive to solvent polarity and reveal highly efficient ROS generation, paving the way to great potential applications.
With a spatially separated donor-acceptor group within a plane,
PerNN
and its derivatives demonstrate properties such as columnar stacking, anti-Kasha dual emission responsive to solvent polarity and efficient ROS generation. |
| doi_str_mv | 10.1039/d4nj01177e |
| format | Article |
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PerNN
and its various derivatives. All targets demonstrate global diamagnetic ring current. Benefiting from a spatially separated donor-acceptor group within one planar skeleton,
PerNN
exhibits efficient narrow blue emission and columnar stacking. More importantly, its alkylated derivatives
PerNN-MeCl
and
PerNN-MeI
display anti-Kasha dual emission responsive to solvent polarity and reveal highly efficient ROS generation, paving the way to great potential applications.
With a spatially separated donor-acceptor group within a plane,
PerNN
and its derivatives demonstrate properties such as columnar stacking, anti-Kasha dual emission responsive to solvent polarity and efficient ROS generation.</description><identifier>ISSN: 1144-0546</identifier><identifier>EISSN: 1369-9261</identifier><identifier>DOI: 10.1039/d4nj01177e</identifier><language>eng</language><publisher>Cambridge: Royal Society of Chemistry</publisher><subject>Alkylation ; Diamagnetism ; Pyridines ; Ring currents</subject><ispartof>New journal of chemistry, 2024-05, Vol.48 (2), p.914-919</ispartof><rights>Copyright Royal Society of Chemistry 2024</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c240t-a3acf6a30f314ef9e0e62d948507d8f1c3ef61ad54e9b6c533fc32f97f6e19783</cites><orcidid>0000-0003-4270-3604 ; 0000-0002-5339-941X</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27922,27923</link.rule.ids></links><search><creatorcontrib>Cao, Jing</creatorcontrib><creatorcontrib>Zhang, Wenhao</creatorcontrib><creatorcontrib>Ding, Yeda</creatorcontrib><creatorcontrib>Zhang, Xuejin</creatorcontrib><creatorcontrib>Zhang, Yuanyuan</creatorcontrib><creatorcontrib>Qiao, Dan</creatorcontrib><creatorcontrib>Biao, Shumin</creatorcontrib><creatorcontrib>Dong, Xuefei</creatorcontrib><creatorcontrib>Song, Jiayi</creatorcontrib><creatorcontrib>Dai, Gaole</creatorcontrib><creatorcontrib>Zhao, Ruiguo</creatorcontrib><creatorcontrib>Wang, Qing</creatorcontrib><title>Perylene with peripherally fused pyrrole and pyridine: columnar packing, anti-Kasha dual emission and reactive oxygen species generation</title><title>New journal of chemistry</title><description>Simultaneously fusing pyrrole and pyridine at perylene's opposite edges is facilely achieved in this work, yielding
PerNN
and its various derivatives. All targets demonstrate global diamagnetic ring current. Benefiting from a spatially separated donor-acceptor group within one planar skeleton,
PerNN
exhibits efficient narrow blue emission and columnar stacking. More importantly, its alkylated derivatives
PerNN-MeCl
and
PerNN-MeI
display anti-Kasha dual emission responsive to solvent polarity and reveal highly efficient ROS generation, paving the way to great potential applications.
With a spatially separated donor-acceptor group within a plane,
PerNN
and its derivatives demonstrate properties such as columnar stacking, anti-Kasha dual emission responsive to solvent polarity and efficient ROS generation.</description><subject>Alkylation</subject><subject>Diamagnetism</subject><subject>Pyridines</subject><subject>Ring currents</subject><issn>1144-0546</issn><issn>1369-9261</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNpFkc1OwzAQhC0EEqVw4Y5kiRsiYMeOU3NDpfxWwAHOkXHW1CV1gp0AeQMeG7dFcNqR9tsdaQahfUpOKGHytORuTijNc9hAA8qETGQq6GbUlPOEZFxso50Q5mQJCTpA34_g-woc4E_bznAD3jYz8Kqqemy6ACVueu_rCrByK21L6-AM67rqFk553Cj9Zt3rcdy3NrlTYaZw2akKw8KGYGu3OvSgdGs_ANdf_Ss4HBrQFgKOOpq1EdtFW0ZVAfZ-5xA9X06extfJ9OHqZnw-TXTKSZsoprQRihHDKAcjgYBIS8lHGcnLkaGagRFUlRkH-SJ0xpjRLDUyNwKozEdsiA7Xfxtfv3cQ2mJed95Fy4KRTOQsG2UiUkdrSvs6BA-maLxdKN8XlBTLpIsLfn-7SnoS4YM17IP-4_6bYD9SpX3-</recordid><startdate>20240520</startdate><enddate>20240520</enddate><creator>Cao, Jing</creator><creator>Zhang, Wenhao</creator><creator>Ding, Yeda</creator><creator>Zhang, Xuejin</creator><creator>Zhang, Yuanyuan</creator><creator>Qiao, Dan</creator><creator>Biao, Shumin</creator><creator>Dong, Xuefei</creator><creator>Song, Jiayi</creator><creator>Dai, Gaole</creator><creator>Zhao, Ruiguo</creator><creator>Wang, Qing</creator><general>Royal Society of Chemistry</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>H9R</scope><scope>JG9</scope><scope>KA0</scope><orcidid>https://orcid.org/0000-0003-4270-3604</orcidid><orcidid>https://orcid.org/0000-0002-5339-941X</orcidid></search><sort><creationdate>20240520</creationdate><title>Perylene with peripherally fused pyrrole and pyridine: columnar packing, anti-Kasha dual emission and reactive oxygen species generation</title><author>Cao, Jing ; Zhang, Wenhao ; Ding, Yeda ; Zhang, Xuejin ; Zhang, Yuanyuan ; Qiao, Dan ; Biao, Shumin ; Dong, Xuefei ; Song, Jiayi ; Dai, Gaole ; Zhao, Ruiguo ; Wang, Qing</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c240t-a3acf6a30f314ef9e0e62d948507d8f1c3ef61ad54e9b6c533fc32f97f6e19783</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Alkylation</topic><topic>Diamagnetism</topic><topic>Pyridines</topic><topic>Ring currents</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Cao, Jing</creatorcontrib><creatorcontrib>Zhang, Wenhao</creatorcontrib><creatorcontrib>Ding, Yeda</creatorcontrib><creatorcontrib>Zhang, Xuejin</creatorcontrib><creatorcontrib>Zhang, Yuanyuan</creatorcontrib><creatorcontrib>Qiao, Dan</creatorcontrib><creatorcontrib>Biao, Shumin</creatorcontrib><creatorcontrib>Dong, Xuefei</creatorcontrib><creatorcontrib>Song, Jiayi</creatorcontrib><creatorcontrib>Dai, Gaole</creatorcontrib><creatorcontrib>Zhao, Ruiguo</creatorcontrib><creatorcontrib>Wang, Qing</creatorcontrib><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Illustrata: Natural Sciences</collection><collection>Materials Research Database</collection><collection>ProQuest Illustrata: Technology Collection</collection><jtitle>New journal of chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Cao, Jing</au><au>Zhang, Wenhao</au><au>Ding, Yeda</au><au>Zhang, Xuejin</au><au>Zhang, Yuanyuan</au><au>Qiao, Dan</au><au>Biao, Shumin</au><au>Dong, Xuefei</au><au>Song, Jiayi</au><au>Dai, Gaole</au><au>Zhao, Ruiguo</au><au>Wang, Qing</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Perylene with peripherally fused pyrrole and pyridine: columnar packing, anti-Kasha dual emission and reactive oxygen species generation</atitle><jtitle>New journal of chemistry</jtitle><date>2024-05-20</date><risdate>2024</risdate><volume>48</volume><issue>2</issue><spage>914</spage><epage>919</epage><pages>914-919</pages><issn>1144-0546</issn><eissn>1369-9261</eissn><abstract>Simultaneously fusing pyrrole and pyridine at perylene's opposite edges is facilely achieved in this work, yielding
PerNN
and its various derivatives. All targets demonstrate global diamagnetic ring current. Benefiting from a spatially separated donor-acceptor group within one planar skeleton,
PerNN
exhibits efficient narrow blue emission and columnar stacking. More importantly, its alkylated derivatives
PerNN-MeCl
and
PerNN-MeI
display anti-Kasha dual emission responsive to solvent polarity and reveal highly efficient ROS generation, paving the way to great potential applications.
With a spatially separated donor-acceptor group within a plane,
PerNN
and its derivatives demonstrate properties such as columnar stacking, anti-Kasha dual emission responsive to solvent polarity and efficient ROS generation.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/d4nj01177e</doi><tpages>6</tpages><orcidid>https://orcid.org/0000-0003-4270-3604</orcidid><orcidid>https://orcid.org/0000-0002-5339-941X</orcidid></addata></record> |
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| issn | 1144-0546 1369-9261 |
| language | eng |
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| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Alkylation Diamagnetism Pyridines Ring currents |
| title | Perylene with peripherally fused pyrrole and pyridine: columnar packing, anti-Kasha dual emission and reactive oxygen species generation |
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