Effects of Antioxidant-Intercalated LDHs on Long-Term Thermal Oxidation Aging and Ultraviolet Aging Resistances of SBS-Modified Asphalt

AbstractThis research aimed to enhance the ultraviolet aging and long-term thermal oxidation aging resistances of styrene-butadiene-styrene (SBS)-modified asphalt simultaneously. For this purpose, antioxidant 1222–intercalated ultraviolet (UV) shielding material layered double hydroxides (LDHs) (LDH...

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Veröffentlicht in:Journal of materials in civil engineering 2024-08, Vol.36 (8)
Hauptverfasser: Chen, Shuaichao, Liu, Quantao, Wu, Hanjun, He, Liang, Wu, Shaopeng
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creator Chen, Shuaichao
Liu, Quantao
Wu, Hanjun
He, Liang
Wu, Shaopeng
description AbstractThis research aimed to enhance the ultraviolet aging and long-term thermal oxidation aging resistances of styrene-butadiene-styrene (SBS)-modified asphalt simultaneously. For this purpose, antioxidant 1222–intercalated ultraviolet (UV) shielding material layered double hydroxides (LDHs) (LDHs-1222) were prepared and added into SBS-modified asphalt as an antiaging agent. The effect of LDHs-1222 on the physical properties, high and low temperature rheology, and chemical composition of SBS-modified asphalt was investigated. Meanwhile, the aging properties of the asphalts after short-term or long-term thermo-oxidative aging and 7-day ultraviolet aging were investigated. The results showed that LDHs-1222 significantly improved the resistance of SBS-modified asphalt to short-term thermo-oxidative, long-term thermo-oxidative, and UV aging while having less impact on the physical and rheological properties than LDHs. Compared with SBS-modified asphalt, the softening point increment, aging indices of viscosity, complex modulus and carbonyl index, and SBS index decrement of the asphalt with LDHs-1222 were significantly reduced, and their growth rates were significantly slowed, indicating that the aging rate and degree of SBS-modified asphalt were reduced by the addition of LDHs-1222. SBS-modified asphalt with 4% LDHs-1222 exhibited superior resistance to long-term thermal oxidation and UV aging compared to asphalt with an equivalent amount of LDHs.
doi_str_mv 10.1061/JMCEE7.MTENG-17995
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For this purpose, antioxidant 1222–intercalated ultraviolet (UV) shielding material layered double hydroxides (LDHs) (LDHs-1222) were prepared and added into SBS-modified asphalt as an antiaging agent. The effect of LDHs-1222 on the physical properties, high and low temperature rheology, and chemical composition of SBS-modified asphalt was investigated. Meanwhile, the aging properties of the asphalts after short-term or long-term thermo-oxidative aging and 7-day ultraviolet aging were investigated. The results showed that LDHs-1222 significantly improved the resistance of SBS-modified asphalt to short-term thermo-oxidative, long-term thermo-oxidative, and UV aging while having less impact on the physical and rheological properties than LDHs. Compared with SBS-modified asphalt, the softening point increment, aging indices of viscosity, complex modulus and carbonyl index, and SBS index decrement of the asphalt with LDHs-1222 were significantly reduced, and their growth rates were significantly slowed, indicating that the aging rate and degree of SBS-modified asphalt were reduced by the addition of LDHs-1222. SBS-modified asphalt with 4% LDHs-1222 exhibited superior resistance to long-term thermal oxidation and UV aging compared to asphalt with an equivalent amount of LDHs.</description><identifier>ISSN: 0899-1561</identifier><identifier>EISSN: 1943-5533</identifier><identifier>DOI: 10.1061/JMCEE7.MTENG-17995</identifier><language>eng</language><publisher>New York: American Society of Civil Engineers</publisher><subject>Aging ; Antioxidants ; Asphalt ; Carbonyls ; Chemical composition ; Hydroxides ; Low temperature ; Oxidation ; Oxidation resistance ; Physical properties ; Rheological properties ; Rheology ; Softening points ; Styrenes ; Technical Papers ; Thermal resistance</subject><ispartof>Journal of materials in civil engineering, 2024-08, Vol.36 (8)</ispartof><rights>2024 American Society of Civil Engineers</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-a320t-f60ccd576b5e0382a88069c591b5d05eaa52c05937a98e2527572e82a4070cc13</cites><orcidid>0000-0003-1818-8702 ; 0000-0002-3682-3696</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttp://ascelibrary.org/doi/pdf/10.1061/JMCEE7.MTENG-17995$$EPDF$$P50$$Gasce$$H</linktopdf><linktohtml>$$Uhttp://ascelibrary.org/doi/abs/10.1061/JMCEE7.MTENG-17995$$EHTML$$P50$$Gasce$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,76193,76201</link.rule.ids></links><search><creatorcontrib>Chen, Shuaichao</creatorcontrib><creatorcontrib>Liu, Quantao</creatorcontrib><creatorcontrib>Wu, Hanjun</creatorcontrib><creatorcontrib>He, Liang</creatorcontrib><creatorcontrib>Wu, Shaopeng</creatorcontrib><title>Effects of Antioxidant-Intercalated LDHs on Long-Term Thermal Oxidation Aging and Ultraviolet Aging Resistances of SBS-Modified Asphalt</title><title>Journal of materials in civil engineering</title><description>AbstractThis research aimed to enhance the ultraviolet aging and long-term thermal oxidation aging resistances of styrene-butadiene-styrene (SBS)-modified asphalt simultaneously. For this purpose, antioxidant 1222–intercalated ultraviolet (UV) shielding material layered double hydroxides (LDHs) (LDHs-1222) were prepared and added into SBS-modified asphalt as an antiaging agent. The effect of LDHs-1222 on the physical properties, high and low temperature rheology, and chemical composition of SBS-modified asphalt was investigated. Meanwhile, the aging properties of the asphalts after short-term or long-term thermo-oxidative aging and 7-day ultraviolet aging were investigated. The results showed that LDHs-1222 significantly improved the resistance of SBS-modified asphalt to short-term thermo-oxidative, long-term thermo-oxidative, and UV aging while having less impact on the physical and rheological properties than LDHs. Compared with SBS-modified asphalt, the softening point increment, aging indices of viscosity, complex modulus and carbonyl index, and SBS index decrement of the asphalt with LDHs-1222 were significantly reduced, and their growth rates were significantly slowed, indicating that the aging rate and degree of SBS-modified asphalt were reduced by the addition of LDHs-1222. SBS-modified asphalt with 4% LDHs-1222 exhibited superior resistance to long-term thermal oxidation and UV aging compared to asphalt with an equivalent amount of LDHs.</description><subject>Aging</subject><subject>Antioxidants</subject><subject>Asphalt</subject><subject>Carbonyls</subject><subject>Chemical composition</subject><subject>Hydroxides</subject><subject>Low temperature</subject><subject>Oxidation</subject><subject>Oxidation resistance</subject><subject>Physical properties</subject><subject>Rheological properties</subject><subject>Rheology</subject><subject>Softening points</subject><subject>Styrenes</subject><subject>Technical Papers</subject><subject>Thermal resistance</subject><issn>0899-1561</issn><issn>1943-5533</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kMtOwzAQRS0EEuXxA6wssTaM4zqOl6EEWpRSiZZ1ZBynBAWn2C6CL-C3cR8SOzYz0uicO9JF6ILCFYWUXj9MR0UhrqaL4vGeUCElP0ADKoeMcM7YIRpAJiWhPKXH6MT7NwBgMIQB-imaxujgcd_g3Ia2_2prZQOZ2GCcVp0Kpsbl7TgCFpe9XZKFce948Rqn6vBsg0fL4nzZ2iVWtsbPXXDqs-07E_bXJ-NbH5TVZvtnfjMn075umzZm5371qrpwho4a1Xlzvt-n6PmuWIzGpJzdT0Z5SRRLIJAmBa1rLtIXboBlicoySKXmkr7wGrhRiicauGRCycwkPBFcJCZyQxDRpOwUXe5yV67_WBsfqrd-7Wx8WTHgPJNCUIhUsqO06713pqlWrn1X7ruiUG0Kr3aFV9vCq23hUbreScpr8xf7j_ELXz-DMQ</recordid><startdate>20240801</startdate><enddate>20240801</enddate><creator>Chen, Shuaichao</creator><creator>Liu, Quantao</creator><creator>Wu, Hanjun</creator><creator>He, Liang</creator><creator>Wu, Shaopeng</creator><general>American Society of Civil Engineers</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>FR3</scope><scope>KR7</scope><orcidid>https://orcid.org/0000-0003-1818-8702</orcidid><orcidid>https://orcid.org/0000-0002-3682-3696</orcidid></search><sort><creationdate>20240801</creationdate><title>Effects of Antioxidant-Intercalated LDHs on Long-Term Thermal Oxidation Aging and Ultraviolet Aging Resistances of SBS-Modified Asphalt</title><author>Chen, Shuaichao ; Liu, Quantao ; Wu, Hanjun ; He, Liang ; Wu, Shaopeng</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a320t-f60ccd576b5e0382a88069c591b5d05eaa52c05937a98e2527572e82a4070cc13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Aging</topic><topic>Antioxidants</topic><topic>Asphalt</topic><topic>Carbonyls</topic><topic>Chemical composition</topic><topic>Hydroxides</topic><topic>Low temperature</topic><topic>Oxidation</topic><topic>Oxidation resistance</topic><topic>Physical properties</topic><topic>Rheological properties</topic><topic>Rheology</topic><topic>Softening points</topic><topic>Styrenes</topic><topic>Technical Papers</topic><topic>Thermal resistance</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chen, Shuaichao</creatorcontrib><creatorcontrib>Liu, Quantao</creatorcontrib><creatorcontrib>Wu, Hanjun</creatorcontrib><creatorcontrib>He, Liang</creatorcontrib><creatorcontrib>Wu, Shaopeng</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><jtitle>Journal of materials in civil engineering</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chen, Shuaichao</au><au>Liu, Quantao</au><au>Wu, Hanjun</au><au>He, Liang</au><au>Wu, Shaopeng</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effects of Antioxidant-Intercalated LDHs on Long-Term Thermal Oxidation Aging and Ultraviolet Aging Resistances of SBS-Modified Asphalt</atitle><jtitle>Journal of materials in civil engineering</jtitle><date>2024-08-01</date><risdate>2024</risdate><volume>36</volume><issue>8</issue><issn>0899-1561</issn><eissn>1943-5533</eissn><abstract>AbstractThis research aimed to enhance the ultraviolet aging and long-term thermal oxidation aging resistances of styrene-butadiene-styrene (SBS)-modified asphalt simultaneously. For this purpose, antioxidant 1222–intercalated ultraviolet (UV) shielding material layered double hydroxides (LDHs) (LDHs-1222) were prepared and added into SBS-modified asphalt as an antiaging agent. The effect of LDHs-1222 on the physical properties, high and low temperature rheology, and chemical composition of SBS-modified asphalt was investigated. Meanwhile, the aging properties of the asphalts after short-term or long-term thermo-oxidative aging and 7-day ultraviolet aging were investigated. The results showed that LDHs-1222 significantly improved the resistance of SBS-modified asphalt to short-term thermo-oxidative, long-term thermo-oxidative, and UV aging while having less impact on the physical and rheological properties than LDHs. Compared with SBS-modified asphalt, the softening point increment, aging indices of viscosity, complex modulus and carbonyl index, and SBS index decrement of the asphalt with LDHs-1222 were significantly reduced, and their growth rates were significantly slowed, indicating that the aging rate and degree of SBS-modified asphalt were reduced by the addition of LDHs-1222. SBS-modified asphalt with 4% LDHs-1222 exhibited superior resistance to long-term thermal oxidation and UV aging compared to asphalt with an equivalent amount of LDHs.</abstract><cop>New York</cop><pub>American Society of Civil Engineers</pub><doi>10.1061/JMCEE7.MTENG-17995</doi><orcidid>https://orcid.org/0000-0003-1818-8702</orcidid><orcidid>https://orcid.org/0000-0002-3682-3696</orcidid></addata></record>
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source American Society of Civil Engineers:NESLI2:Journals:2014
subjects Aging
Antioxidants
Asphalt
Carbonyls
Chemical composition
Hydroxides
Low temperature
Oxidation
Oxidation resistance
Physical properties
Rheological properties
Rheology
Softening points
Styrenes
Technical Papers
Thermal resistance
title Effects of Antioxidant-Intercalated LDHs on Long-Term Thermal Oxidation Aging and Ultraviolet Aging Resistances of SBS-Modified Asphalt
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