Discriminating the Active Ru Species Towards the Selective Generation of Singlet Oxygen from Peroxymonosulfate: Nanoparticles Surpass Single‐Atom Catalysts

Singlet oxygen (1O2) is an exceptional reactive oxygen species in advanced oxidation processes for environmental remediation. Despite single‐atom catalysts (SACs) representing the promising candidate for the selective generation of 1O2 from peroxymonosulfate (PMS), the necessity to meticulously regu...

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Veröffentlicht in:	Angewandte Chemie 2024-04, Vol.136 (17), p.n/a
Hauptverfasser:	Bi, Guangyu, Ding, Rongrong, Song, Junsheng, Luo, Mengjie, Zhang, Haotian, Liu, Meng, Huang, Dahong, Mu, Yang
Format:	Artikel
Sprache:	eng
Schlagworte:	Catalysts Density functional theory Design optimization Dimerization Environmental cleanup Free energy Intermediates Nanoparticles Oxidation Oxygen PMS activation Pyrolysis Reactive oxygen species Ru nanoparticles Ruthenium selectivity single-atom catalysts Singlet oxygen
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