Improving the luminescence intensity of Mn2+ doped B-P-Zn-K based glass–ceramics through tuning structure of Mn2
For photoluminescence (PL) properties of Mn 2+ in glass–ceramics are highly dependent on the concentration of Mn 2+ , we experimentally observed the change of Mn 2+ structures from isolated Mn 2+ ion as a tetrahedron, octahedron to Mn 2+ -Mn 2+ dimer in B-P-Zn-K based glass–ceramics with characteris...
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| Veröffentlicht in: | Applied physics. A, Materials science & processing Materials science & processing, 2024-04, Vol.130 (4), Article 247 |
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| creator | Song, Wenqiang Zhao, Fengjiao Xu, Changyuan Wang, Qun Yin, Hongming |
| description | For photoluminescence (PL) properties of Mn
2+
in glass–ceramics are highly dependent on the concentration of Mn
2+
, we experimentally observed the change of Mn
2+
structures from isolated Mn
2+
ion as a tetrahedron, octahedron to Mn
2+
-Mn
2+
dimer in B-P-Zn-K based glass–ceramics with characteristic PL peaks locating at 504 nm, 600 nm, and 660 nm, respectively. Spectral results reveal that condensed Mn
2+
would lead to redshift of PL emission and reduced Luminous intensity caused by concentration quenching, however, with increasing Mn
2+
content, shift of Mn
2+
structure is the determining factor for PL redshift. Moreover, compared with tetrahedral and octahedral Mn
2+
, Mn
2+
-Mn
2+
dimer exhibits highly enhanced PL emission and shortened life span which reveal that transitions of Mn
2+
-Mn
2+
dimer are far more efficient than those transitions in tetrahedral and octahedral Mn
2+
. This enables tuning of color and efficiency of PL emission for Mn-doped glass–ceramics via a simple method.
Graphical abstract |
| doi_str_mv | 10.1007/s00339-024-07404-y |
| format | Article |
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2+
in glass–ceramics are highly dependent on the concentration of Mn
2+
, we experimentally observed the change of Mn
2+
structures from isolated Mn
2+
ion as a tetrahedron, octahedron to Mn
2+
-Mn
2+
dimer in B-P-Zn-K based glass–ceramics with characteristic PL peaks locating at 504 nm, 600 nm, and 660 nm, respectively. Spectral results reveal that condensed Mn
2+
would lead to redshift of PL emission and reduced Luminous intensity caused by concentration quenching, however, with increasing Mn
2+
content, shift of Mn
2+
structure is the determining factor for PL redshift. Moreover, compared with tetrahedral and octahedral Mn
2+
, Mn
2+
-Mn
2+
dimer exhibits highly enhanced PL emission and shortened life span which reveal that transitions of Mn
2+
-Mn
2+
dimer are far more efficient than those transitions in tetrahedral and octahedral Mn
2+
. This enables tuning of color and efficiency of PL emission for Mn-doped glass–ceramics via a simple method.
Graphical abstract</description><identifier>ISSN: 0947-8396</identifier><identifier>EISSN: 1432-0630</identifier><identifier>DOI: 10.1007/s00339-024-07404-y</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Characterization and Evaluation of Materials ; Condensed Matter Physics ; Dimers ; Glass ceramics ; Luminous intensity ; Machines ; Manganese ions ; Manufacturing ; Nanotechnology ; Optical and Electronic Materials ; Photoluminescence ; Physics ; Physics and Astronomy ; Processes ; Red shift ; Surfaces and Interfaces ; Tetrahedra ; Thin Films ; Tuning</subject><ispartof>Applied physics. A, Materials science & processing, 2024-04, Vol.130 (4), Article 247</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH, DE part of Springer Nature 2024. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c200t-77eadb116f3d2b52675679a7e4090d3331915d031ffae9a219cacc0af87175bc3</cites><orcidid>0000-0002-4024-1330</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s00339-024-07404-y$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s00339-024-07404-y$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Song, Wenqiang</creatorcontrib><creatorcontrib>Zhao, Fengjiao</creatorcontrib><creatorcontrib>Xu, Changyuan</creatorcontrib><creatorcontrib>Wang, Qun</creatorcontrib><creatorcontrib>Yin, Hongming</creatorcontrib><title>Improving the luminescence intensity of Mn2+ doped B-P-Zn-K based glass–ceramics through tuning structure of Mn2</title><title>Applied physics. A, Materials science & processing</title><addtitle>Appl. Phys. A</addtitle><description>For photoluminescence (PL) properties of Mn
2+
in glass–ceramics are highly dependent on the concentration of Mn
2+
, we experimentally observed the change of Mn
2+
structures from isolated Mn
2+
ion as a tetrahedron, octahedron to Mn
2+
-Mn
2+
dimer in B-P-Zn-K based glass–ceramics with characteristic PL peaks locating at 504 nm, 600 nm, and 660 nm, respectively. Spectral results reveal that condensed Mn
2+
would lead to redshift of PL emission and reduced Luminous intensity caused by concentration quenching, however, with increasing Mn
2+
content, shift of Mn
2+
structure is the determining factor for PL redshift. Moreover, compared with tetrahedral and octahedral Mn
2+
, Mn
2+
-Mn
2+
dimer exhibits highly enhanced PL emission and shortened life span which reveal that transitions of Mn
2+
-Mn
2+
dimer are far more efficient than those transitions in tetrahedral and octahedral Mn
2+
. This enables tuning of color and efficiency of PL emission for Mn-doped glass–ceramics via a simple method.
Graphical abstract</description><subject>Characterization and Evaluation of Materials</subject><subject>Condensed Matter Physics</subject><subject>Dimers</subject><subject>Glass ceramics</subject><subject>Luminous intensity</subject><subject>Machines</subject><subject>Manganese ions</subject><subject>Manufacturing</subject><subject>Nanotechnology</subject><subject>Optical and Electronic Materials</subject><subject>Photoluminescence</subject><subject>Physics</subject><subject>Physics and Astronomy</subject><subject>Processes</subject><subject>Red shift</subject><subject>Surfaces and Interfaces</subject><subject>Tetrahedra</subject><subject>Thin Films</subject><subject>Tuning</subject><issn>0947-8396</issn><issn>1432-0630</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kL1OwzAURi0EEqXwAkyWGJHh2k7ieoSKn4oiGGBhsRzHSVM1TrETpGy8A2_Ik-DSSmx4ubL0fefqHoROKVxQAHEZADiXBFhCQCSQkGEPjWjCGYGMwz4agUwEmXCZHaKjEJYQX8LYCPlZs_btR-0q3C0sXvVN7Www1hmLa9dZF-puwG2JHx07x0W7tgW-Js_kzZEHnOsQv9VKh_D9-WWs101tQgT5tq8WuOvdhhs635uu93aHOUYHpV4Fe7KbY_R6e_MyvSfzp7vZ9GpODAPoiBBWFzmlWckLlqcsE2kmpBY2AQkF55xKmhbAaVlqKzWj0mhjQJcTQUWaGz5GZ1tuPPC9t6FTy7b3Lq5UTE5SmXBIZUyxbcr4NgRvS7X2daP9oCiojVu1dauiW_XrVg2xxLelEMOusv4P_U_rBwKwfiA</recordid><startdate>20240401</startdate><enddate>20240401</enddate><creator>Song, Wenqiang</creator><creator>Zhao, Fengjiao</creator><creator>Xu, Changyuan</creator><creator>Wang, Qun</creator><creator>Yin, Hongming</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-4024-1330</orcidid></search><sort><creationdate>20240401</creationdate><title>Improving the luminescence intensity of Mn2+ doped B-P-Zn-K based glass–ceramics through tuning structure of Mn2</title><author>Song, Wenqiang ; Zhao, Fengjiao ; Xu, Changyuan ; Wang, Qun ; Yin, Hongming</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c200t-77eadb116f3d2b52675679a7e4090d3331915d031ffae9a219cacc0af87175bc3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Characterization and Evaluation of Materials</topic><topic>Condensed Matter Physics</topic><topic>Dimers</topic><topic>Glass ceramics</topic><topic>Luminous intensity</topic><topic>Machines</topic><topic>Manganese ions</topic><topic>Manufacturing</topic><topic>Nanotechnology</topic><topic>Optical and Electronic Materials</topic><topic>Photoluminescence</topic><topic>Physics</topic><topic>Physics and Astronomy</topic><topic>Processes</topic><topic>Red shift</topic><topic>Surfaces and Interfaces</topic><topic>Tetrahedra</topic><topic>Thin Films</topic><topic>Tuning</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Song, Wenqiang</creatorcontrib><creatorcontrib>Zhao, Fengjiao</creatorcontrib><creatorcontrib>Xu, Changyuan</creatorcontrib><creatorcontrib>Wang, Qun</creatorcontrib><creatorcontrib>Yin, Hongming</creatorcontrib><collection>CrossRef</collection><jtitle>Applied physics. A, Materials science & processing</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Song, Wenqiang</au><au>Zhao, Fengjiao</au><au>Xu, Changyuan</au><au>Wang, Qun</au><au>Yin, Hongming</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Improving the luminescence intensity of Mn2+ doped B-P-Zn-K based glass–ceramics through tuning structure of Mn2</atitle><jtitle>Applied physics. A, Materials science & processing</jtitle><stitle>Appl. Phys. A</stitle><date>2024-04-01</date><risdate>2024</risdate><volume>130</volume><issue>4</issue><artnum>247</artnum><issn>0947-8396</issn><eissn>1432-0630</eissn><abstract>For photoluminescence (PL) properties of Mn
2+
in glass–ceramics are highly dependent on the concentration of Mn
2+
, we experimentally observed the change of Mn
2+
structures from isolated Mn
2+
ion as a tetrahedron, octahedron to Mn
2+
-Mn
2+
dimer in B-P-Zn-K based glass–ceramics with characteristic PL peaks locating at 504 nm, 600 nm, and 660 nm, respectively. Spectral results reveal that condensed Mn
2+
would lead to redshift of PL emission and reduced Luminous intensity caused by concentration quenching, however, with increasing Mn
2+
content, shift of Mn
2+
structure is the determining factor for PL redshift. Moreover, compared with tetrahedral and octahedral Mn
2+
, Mn
2+
-Mn
2+
dimer exhibits highly enhanced PL emission and shortened life span which reveal that transitions of Mn
2+
-Mn
2+
dimer are far more efficient than those transitions in tetrahedral and octahedral Mn
2+
. This enables tuning of color and efficiency of PL emission for Mn-doped glass–ceramics via a simple method.
Graphical abstract</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s00339-024-07404-y</doi><orcidid>https://orcid.org/0000-0002-4024-1330</orcidid></addata></record> |
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| ispartof | Applied physics. A, Materials science & processing, 2024-04, Vol.130 (4), Article 247 |
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| language | eng |
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| source | SpringerLink Journals - AutoHoldings |
| subjects | Characterization and Evaluation of Materials Condensed Matter Physics Dimers Glass ceramics Luminous intensity Machines Manganese ions Manufacturing Nanotechnology Optical and Electronic Materials Photoluminescence Physics Physics and Astronomy Processes Red shift Surfaces and Interfaces Tetrahedra Thin Films Tuning |
| title | Improving the luminescence intensity of Mn2+ doped B-P-Zn-K based glass–ceramics through tuning structure of Mn2 |
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