Light‐Driven C−C Coupling for Targeted Synthesis of CH3COOH with Nearly 100 % Selectivity from CO2

Targeted synthesis of acetic acid (CH3COOH) from CO2 photoreduction under mild conditions mainly limits by the kinetic challenge of the C−C coupling. Herein, we utilized doping engineering to build charge‐asymmetrical metal pair sites for boosted C−C coupling, enhancing the activity and selectivity...

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Veröffentlicht in:	Angewandte Chemie International Edition 2024-03, Vol.63 (13), p.n/a
Hauptverfasser:	Ding, Jinyu, Du, Peijin, Zhu, Juncheng, Hu, Qing, He, Dongpo, Wu, Yang, Liu, Wenxiu, Zhu, Shan, Yan, Wensheng, Hu, Jun, Zhu, Junfa, Chen, Qingxia, Jiao, Xingchen, Xie, Yi
Format:	Artikel
Sprache:	eng
Schlagworte:	Acetic acid Asymmetry Carbon dioxide CH3COOH synthesis CO2 photoreduction Cobalt Cobalt oxides Coupling C−C coupling Doping Free energy Heat of formation Heavy metals Intermediates nearly 100 % selectivity Palladium Photoelectron spectroscopy Photoelectrons Photoreduction Protonation Spectroscopy Spectrum analysis Synthesis
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