Corrosion and Cavitation Erosion Behaviours of Cast Nickel Aluminium Bronze in 3.5% NaCl Solution with Different Sulphide Concentrations
The effect of sulphide (Na 2 S) concentration (SC) on the corrosion and cavitation erosion behaviours of a cast nickel aluminium bronze (NAB) in 3.5% NaCl solution is investigated in this study. The results show that when the SC exceeds 50 ppm, the hydrogen evolution reaction dominates the cathodic...
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| Veröffentlicht in: | Acta metallurgica sinica : English letters 2019-12, Vol.32 (12), p.1470-1482 |
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| creator | Song, Qi-Ning Xu, Nan Tong, Yao Huang, Chen-Ming Sun, Shou-Yu Xu, Chen-Bo Bao, Ye-Feng Jiang, Yong-Feng Qiao, Yan-Xin Zhu, Zhi-Yuan Wang, Zheng-Bin |
| description | The effect of sulphide (Na
2
S) concentration (SC) on the corrosion and cavitation erosion behaviours of a cast nickel aluminium bronze (NAB) in 3.5% NaCl solution is investigated in this study. The results show that when the SC exceeds 50 ppm, the hydrogen evolution reaction dominates the cathodic process, and a limiting current region appears in the anodic branch of the polarisation curve due to the formation of a copper sulphide film, which is a diffusion-controlled process. After long-term immersion, the increased mass loss rate of NAB with the sulphide additions of 20 and 50 ppm is attributed to the less protective films, which contains a mixture of copper oxides and sulphides. Moreover, NAB undergoes severe localised corrosion (selective phase corrosion, SPC) at the
β
′ phases and eutectoid microstructure
α
+
κ
III
. By comparison, NAB undergoes general corrosion and a copper sulphide film is formed in 100 and 200 ppm sulphide solutions. Cavitation erosion greatly increases the corrosion rate of NAB in all solutions and causes a negative potential shift in 3.5% NaCl solution due to the film destruction. However, a positive potential shift occurs in the solutions with SC higher than 50 ppm due to the accelerated mass transfer of the cathodic process. The cavitation erosion mass loss rate of NAB increases with the increase of SC. The occurrence of severe SPC decreases the phase boundary cohesion and causes brittle fracture under the cavitation impact. The corrosion–enhanced erosion is the most predominant factor for the cavitation erosion damage when the SC exceeds 50 ppm. |
| doi_str_mv | 10.1007/s40195-019-00963-7 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2933747121</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2933747121</sourcerecordid><originalsourceid>FETCH-LOGICAL-c363t-8fcc33aa415d059796e2adf44177b7e06b516552c993eedae3ee8c22c5250f503</originalsourceid><addsrcrecordid>eNp9UMtOwzAQtBBIlMIPcLKEOKb4Ecf1sQ3lIVXlUDhbruNQl9QudgKCL-CzcR8SNy6z2tHMrHYAuMRogBHiNzFHWLAsQYaQKGjGj0CPYJFnmAzFMeglVZFxLPApOItxlTaSM94DP6UPwUfrHVSugqX6sK1qt-vkQI_NMpG-CxH6OgliC2dWv5kGjppubZ3t1nAcvPs20DpIB-wazlTZwLlvul3Qp22X8NbWtQnGtXDeNZulrQwsvdOJCLtz8Ryc1KqJ5uIw--DlbvJcPmTTp_vHcjTNNC1omw1rrSlVKsesQkxwURiiqjrPMecLblCxYLhgjGghqDGVMgmHmhDNCEM1Q7QPrva5m-DfOxNbuUq_uXRSEkEpzzkmOKnIXqVTCzGYWm6CXavwJTGS28blvnGZQO4alzyZ6N4Uk9i9mvAX_Y_rF7yyhNw</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2933747121</pqid></control><display><type>article</type><title>Corrosion and Cavitation Erosion Behaviours of Cast Nickel Aluminium Bronze in 3.5% NaCl Solution with Different Sulphide Concentrations</title><source>SpringerNature Journals</source><source>ProQuest Central UK/Ireland</source><source>Alma/SFX Local Collection</source><source>ProQuest Central</source><creator>Song, Qi-Ning ; Xu, Nan ; Tong, Yao ; Huang, Chen-Ming ; Sun, Shou-Yu ; Xu, Chen-Bo ; Bao, Ye-Feng ; Jiang, Yong-Feng ; Qiao, Yan-Xin ; Zhu, Zhi-Yuan ; Wang, Zheng-Bin</creator><creatorcontrib>Song, Qi-Ning ; Xu, Nan ; Tong, Yao ; Huang, Chen-Ming ; Sun, Shou-Yu ; Xu, Chen-Bo ; Bao, Ye-Feng ; Jiang, Yong-Feng ; Qiao, Yan-Xin ; Zhu, Zhi-Yuan ; Wang, Zheng-Bin</creatorcontrib><description>The effect of sulphide (Na
2
S) concentration (SC) on the corrosion and cavitation erosion behaviours of a cast nickel aluminium bronze (NAB) in 3.5% NaCl solution is investigated in this study. The results show that when the SC exceeds 50 ppm, the hydrogen evolution reaction dominates the cathodic process, and a limiting current region appears in the anodic branch of the polarisation curve due to the formation of a copper sulphide film, which is a diffusion-controlled process. After long-term immersion, the increased mass loss rate of NAB with the sulphide additions of 20 and 50 ppm is attributed to the less protective films, which contains a mixture of copper oxides and sulphides. Moreover, NAB undergoes severe localised corrosion (selective phase corrosion, SPC) at the
β
′ phases and eutectoid microstructure
α
+
κ
III
. By comparison, NAB undergoes general corrosion and a copper sulphide film is formed in 100 and 200 ppm sulphide solutions. Cavitation erosion greatly increases the corrosion rate of NAB in all solutions and causes a negative potential shift in 3.5% NaCl solution due to the film destruction. However, a positive potential shift occurs in the solutions with SC higher than 50 ppm due to the accelerated mass transfer of the cathodic process. The cavitation erosion mass loss rate of NAB increases with the increase of SC. The occurrence of severe SPC decreases the phase boundary cohesion and causes brittle fracture under the cavitation impact. The corrosion–enhanced erosion is the most predominant factor for the cavitation erosion damage when the SC exceeds 50 ppm.</description><identifier>ISSN: 1006-7191</identifier><identifier>EISSN: 2194-1289</identifier><identifier>DOI: 10.1007/s40195-019-00963-7</identifier><language>eng</language><publisher>Beijing: The Chinese Society for Metals</publisher><subject>Alloys ; Aluminum bronzes ; Behavior ; Bronze ; Cavitation ; Cavitation erosion ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Copper ; Copper oxides ; Copper sulfides ; Corrosion and Coatings ; Corrosion effects ; Corrosion rate ; Corrosion resistance ; Corrosion tests ; Diffusion rate ; Electrode polarization ; Electrodes ; Eutectoids ; Hydrogen embrittlement ; Hydrogen evolution reactions ; Intermetallic compounds ; Localized corrosion ; Mass transfer ; Materials Science ; Metallic Materials ; Nanotechnology ; Nickel ; Organometallic Chemistry ; Seawater ; Sodium chloride ; Sodium sulfide ; Spectroscopy/Spectrometry ; Stainless steel ; Tribology ; Uniform attack (corrosion)</subject><ispartof>Acta metallurgica sinica : English letters, 2019-12, Vol.32 (12), p.1470-1482</ispartof><rights>The Chinese Society for Metals (CSM) and Springer-Verlag GmbH Germany, part of Springer Nature 2019</rights><rights>The Chinese Society for Metals (CSM) and Springer-Verlag GmbH Germany, part of Springer Nature 2019.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c363t-8fcc33aa415d059796e2adf44177b7e06b516552c993eedae3ee8c22c5250f503</citedby><cites>FETCH-LOGICAL-c363t-8fcc33aa415d059796e2adf44177b7e06b516552c993eedae3ee8c22c5250f503</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s40195-019-00963-7$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2933747121?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>315,781,785,21393,27929,27930,33749,41493,42562,43810,51324,64390,64394,72474</link.rule.ids></links><search><creatorcontrib>Song, Qi-Ning</creatorcontrib><creatorcontrib>Xu, Nan</creatorcontrib><creatorcontrib>Tong, Yao</creatorcontrib><creatorcontrib>Huang, Chen-Ming</creatorcontrib><creatorcontrib>Sun, Shou-Yu</creatorcontrib><creatorcontrib>Xu, Chen-Bo</creatorcontrib><creatorcontrib>Bao, Ye-Feng</creatorcontrib><creatorcontrib>Jiang, Yong-Feng</creatorcontrib><creatorcontrib>Qiao, Yan-Xin</creatorcontrib><creatorcontrib>Zhu, Zhi-Yuan</creatorcontrib><creatorcontrib>Wang, Zheng-Bin</creatorcontrib><title>Corrosion and Cavitation Erosion Behaviours of Cast Nickel Aluminium Bronze in 3.5% NaCl Solution with Different Sulphide Concentrations</title><title>Acta metallurgica sinica : English letters</title><addtitle>Acta Metall. Sin. (Engl. Lett.)</addtitle><description>The effect of sulphide (Na
2
S) concentration (SC) on the corrosion and cavitation erosion behaviours of a cast nickel aluminium bronze (NAB) in 3.5% NaCl solution is investigated in this study. The results show that when the SC exceeds 50 ppm, the hydrogen evolution reaction dominates the cathodic process, and a limiting current region appears in the anodic branch of the polarisation curve due to the formation of a copper sulphide film, which is a diffusion-controlled process. After long-term immersion, the increased mass loss rate of NAB with the sulphide additions of 20 and 50 ppm is attributed to the less protective films, which contains a mixture of copper oxides and sulphides. Moreover, NAB undergoes severe localised corrosion (selective phase corrosion, SPC) at the
β
′ phases and eutectoid microstructure
α
+
κ
III
. By comparison, NAB undergoes general corrosion and a copper sulphide film is formed in 100 and 200 ppm sulphide solutions. Cavitation erosion greatly increases the corrosion rate of NAB in all solutions and causes a negative potential shift in 3.5% NaCl solution due to the film destruction. However, a positive potential shift occurs in the solutions with SC higher than 50 ppm due to the accelerated mass transfer of the cathodic process. The cavitation erosion mass loss rate of NAB increases with the increase of SC. The occurrence of severe SPC decreases the phase boundary cohesion and causes brittle fracture under the cavitation impact. The corrosion–enhanced erosion is the most predominant factor for the cavitation erosion damage when the SC exceeds 50 ppm.</description><subject>Alloys</subject><subject>Aluminum bronzes</subject><subject>Behavior</subject><subject>Bronze</subject><subject>Cavitation</subject><subject>Cavitation erosion</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Copper</subject><subject>Copper oxides</subject><subject>Copper sulfides</subject><subject>Corrosion and Coatings</subject><subject>Corrosion effects</subject><subject>Corrosion rate</subject><subject>Corrosion resistance</subject><subject>Corrosion tests</subject><subject>Diffusion rate</subject><subject>Electrode polarization</subject><subject>Electrodes</subject><subject>Eutectoids</subject><subject>Hydrogen embrittlement</subject><subject>Hydrogen evolution reactions</subject><subject>Intermetallic compounds</subject><subject>Localized corrosion</subject><subject>Mass transfer</subject><subject>Materials Science</subject><subject>Metallic Materials</subject><subject>Nanotechnology</subject><subject>Nickel</subject><subject>Organometallic Chemistry</subject><subject>Seawater</subject><subject>Sodium chloride</subject><subject>Sodium sulfide</subject><subject>Spectroscopy/Spectrometry</subject><subject>Stainless steel</subject><subject>Tribology</subject><subject>Uniform attack (corrosion)</subject><issn>1006-7191</issn><issn>2194-1289</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9UMtOwzAQtBBIlMIPcLKEOKb4Ecf1sQ3lIVXlUDhbruNQl9QudgKCL-CzcR8SNy6z2tHMrHYAuMRogBHiNzFHWLAsQYaQKGjGj0CPYJFnmAzFMeglVZFxLPApOItxlTaSM94DP6UPwUfrHVSugqX6sK1qt-vkQI_NMpG-CxH6OgliC2dWv5kGjppubZ3t1nAcvPs20DpIB-wazlTZwLlvul3Qp22X8NbWtQnGtXDeNZulrQwsvdOJCLtz8Ryc1KqJ5uIw--DlbvJcPmTTp_vHcjTNNC1omw1rrSlVKsesQkxwURiiqjrPMecLblCxYLhgjGghqDGVMgmHmhDNCEM1Q7QPrva5m-DfOxNbuUq_uXRSEkEpzzkmOKnIXqVTCzGYWm6CXavwJTGS28blvnGZQO4alzyZ6N4Uk9i9mvAX_Y_rF7yyhNw</recordid><startdate>20191201</startdate><enddate>20191201</enddate><creator>Song, Qi-Ning</creator><creator>Xu, Nan</creator><creator>Tong, Yao</creator><creator>Huang, Chen-Ming</creator><creator>Sun, Shou-Yu</creator><creator>Xu, Chen-Bo</creator><creator>Bao, Ye-Feng</creator><creator>Jiang, Yong-Feng</creator><creator>Qiao, Yan-Xin</creator><creator>Zhu, Zhi-Yuan</creator><creator>Wang, Zheng-Bin</creator><general>The Chinese Society for Metals</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope></search><sort><creationdate>20191201</creationdate><title>Corrosion and Cavitation Erosion Behaviours of Cast Nickel Aluminium Bronze in 3.5% NaCl Solution with Different Sulphide Concentrations</title><author>Song, Qi-Ning ; Xu, Nan ; Tong, Yao ; Huang, Chen-Ming ; Sun, Shou-Yu ; Xu, Chen-Bo ; Bao, Ye-Feng ; Jiang, Yong-Feng ; Qiao, Yan-Xin ; Zhu, Zhi-Yuan ; Wang, Zheng-Bin</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c363t-8fcc33aa415d059796e2adf44177b7e06b516552c993eedae3ee8c22c5250f503</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><topic>Alloys</topic><topic>Aluminum bronzes</topic><topic>Behavior</topic><topic>Bronze</topic><topic>Cavitation</topic><topic>Cavitation erosion</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Copper</topic><topic>Copper oxides</topic><topic>Copper sulfides</topic><topic>Corrosion and Coatings</topic><topic>Corrosion effects</topic><topic>Corrosion rate</topic><topic>Corrosion resistance</topic><topic>Corrosion tests</topic><topic>Diffusion rate</topic><topic>Electrode polarization</topic><topic>Electrodes</topic><topic>Eutectoids</topic><topic>Hydrogen embrittlement</topic><topic>Hydrogen evolution reactions</topic><topic>Intermetallic compounds</topic><topic>Localized corrosion</topic><topic>Mass transfer</topic><topic>Materials Science</topic><topic>Metallic Materials</topic><topic>Nanotechnology</topic><topic>Nickel</topic><topic>Organometallic Chemistry</topic><topic>Seawater</topic><topic>Sodium chloride</topic><topic>Sodium sulfide</topic><topic>Spectroscopy/Spectrometry</topic><topic>Stainless steel</topic><topic>Tribology</topic><topic>Uniform attack (corrosion)</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Song, Qi-Ning</creatorcontrib><creatorcontrib>Xu, Nan</creatorcontrib><creatorcontrib>Tong, Yao</creatorcontrib><creatorcontrib>Huang, Chen-Ming</creatorcontrib><creatorcontrib>Sun, Shou-Yu</creatorcontrib><creatorcontrib>Xu, Chen-Bo</creatorcontrib><creatorcontrib>Bao, Ye-Feng</creatorcontrib><creatorcontrib>Jiang, Yong-Feng</creatorcontrib><creatorcontrib>Qiao, Yan-Xin</creatorcontrib><creatorcontrib>Zhu, Zhi-Yuan</creatorcontrib><creatorcontrib>Wang, Zheng-Bin</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><jtitle>Acta metallurgica sinica : English letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Song, Qi-Ning</au><au>Xu, Nan</au><au>Tong, Yao</au><au>Huang, Chen-Ming</au><au>Sun, Shou-Yu</au><au>Xu, Chen-Bo</au><au>Bao, Ye-Feng</au><au>Jiang, Yong-Feng</au><au>Qiao, Yan-Xin</au><au>Zhu, Zhi-Yuan</au><au>Wang, Zheng-Bin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Corrosion and Cavitation Erosion Behaviours of Cast Nickel Aluminium Bronze in 3.5% NaCl Solution with Different Sulphide Concentrations</atitle><jtitle>Acta metallurgica sinica : English letters</jtitle><stitle>Acta Metall. Sin. (Engl. Lett.)</stitle><date>2019-12-01</date><risdate>2019</risdate><volume>32</volume><issue>12</issue><spage>1470</spage><epage>1482</epage><pages>1470-1482</pages><issn>1006-7191</issn><eissn>2194-1289</eissn><abstract>The effect of sulphide (Na
2
S) concentration (SC) on the corrosion and cavitation erosion behaviours of a cast nickel aluminium bronze (NAB) in 3.5% NaCl solution is investigated in this study. The results show that when the SC exceeds 50 ppm, the hydrogen evolution reaction dominates the cathodic process, and a limiting current region appears in the anodic branch of the polarisation curve due to the formation of a copper sulphide film, which is a diffusion-controlled process. After long-term immersion, the increased mass loss rate of NAB with the sulphide additions of 20 and 50 ppm is attributed to the less protective films, which contains a mixture of copper oxides and sulphides. Moreover, NAB undergoes severe localised corrosion (selective phase corrosion, SPC) at the
β
′ phases and eutectoid microstructure
α
+
κ
III
. By comparison, NAB undergoes general corrosion and a copper sulphide film is formed in 100 and 200 ppm sulphide solutions. Cavitation erosion greatly increases the corrosion rate of NAB in all solutions and causes a negative potential shift in 3.5% NaCl solution due to the film destruction. However, a positive potential shift occurs in the solutions with SC higher than 50 ppm due to the accelerated mass transfer of the cathodic process. The cavitation erosion mass loss rate of NAB increases with the increase of SC. The occurrence of severe SPC decreases the phase boundary cohesion and causes brittle fracture under the cavitation impact. The corrosion–enhanced erosion is the most predominant factor for the cavitation erosion damage when the SC exceeds 50 ppm.</abstract><cop>Beijing</cop><pub>The Chinese Society for Metals</pub><doi>10.1007/s40195-019-00963-7</doi><tpages>13</tpages><oa>free_for_read</oa></addata></record> |
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| subjects | Alloys Aluminum bronzes Behavior Bronze Cavitation Cavitation erosion Characterization and Evaluation of Materials Chemistry and Materials Science Copper Copper oxides Copper sulfides Corrosion and Coatings Corrosion effects Corrosion rate Corrosion resistance Corrosion tests Diffusion rate Electrode polarization Electrodes Eutectoids Hydrogen embrittlement Hydrogen evolution reactions Intermetallic compounds Localized corrosion Mass transfer Materials Science Metallic Materials Nanotechnology Nickel Organometallic Chemistry Seawater Sodium chloride Sodium sulfide Spectroscopy/Spectrometry Stainless steel Tribology Uniform attack (corrosion) |
| title | Corrosion and Cavitation Erosion Behaviours of Cast Nickel Aluminium Bronze in 3.5% NaCl Solution with Different Sulphide Concentrations |
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