Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau
The physicochemical properties and origins of atmospheric aerosols in the Tibetan Plateau (TP) region are a research topic of great interest, but an in‐depth understanding of this topic is challenging, partially due to a lack of intensive in situ observations. Thus, a field campaign was conducted ov...
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creator | Yu, Zeren Tian, Pengfei Kang, Chenliang Song, Xin Huang, Jianping Guo, Yumin Shi, Jinsen Tang, Chenguang Zhang, Haotian Zhang, Zhida Cao, Xianjie Liang, Jiening Zhang, Lei |
description | The physicochemical properties and origins of atmospheric aerosols in the Tibetan Plateau (TP) region are a research topic of great interest, but an in‐depth understanding of this topic is challenging, partially due to a lack of intensive in situ observations. Thus, a field campaign was conducted over Yadong, a remote area on the south slope of the TP from June 11 to 31 August 2021. The aerosol loading was low, with a black carbon mass concentration of 147.4 ± 98.4 ng·m−3. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and increased from 450 to 700 nm wavelength. Organic matter (OM) accounting for 69.6% of the total aerosol mass and relatively high secondary organic carbon ratios, highlighting the importance of secondary formation. An interesting phenomenon observed was that the evolution of aerosols was mainly characterized by diurnal variation, which could not be explained by large‐scale atmospheric processes such as Indian summer monsoon. Instead, it was found that regional mountain‐valley winds between the Himalayas and South Asia transported polluted air masses toward the TP, especially in the afternoon when regional valley wind are expected to be the strongest and the boundary layer in South Asia is deepest. Additionally, daytime local valley wind further elevated these aerosols to higher altitudes on the TP. This paper provides insights into the transport mechanisms of aerosols from South Asia to the TP. These findings are of great importance since aerosols exhibit significant diurnal variations in the TP region.
Plain Language Summary
Previous studies focused on the analysis of the physical or chemical properties of aerosols on the Tibetan Plateau, but this study provides a comprehensive examination of both. The findings reveal that aerosols on the southern slope of the Tibetan Plateau exhibit strong absorption efficiency. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm), which may be attributed to aerosol secondary generation and coating. Finally, the mechanism of pollutant transport from South Asia to the Tibetan Plateau was analyzed relies on site observations, satellite, and reanalysis data to highlight the link between diurnal variations of pollutants and transport mechanism. The specific transport mechanism be understood uniformly across different scales, including Indian summer monsoon, regional mountain‐valley winds between the Himalayas and South Asia, and local mountain‐valley winds circulation.
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doi_str_mv | 10.1029/2023JD040193 |
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Plain Language Summary
Previous studies focused on the analysis of the physical or chemical properties of aerosols on the Tibetan Plateau, but this study provides a comprehensive examination of both. The findings reveal that aerosols on the southern slope of the Tibetan Plateau exhibit strong absorption efficiency. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm), which may be attributed to aerosol secondary generation and coating. Finally, the mechanism of pollutant transport from South Asia to the Tibetan Plateau was analyzed relies on site observations, satellite, and reanalysis data to highlight the link between diurnal variations of pollutants and transport mechanism. The specific transport mechanism be understood uniformly across different scales, including Indian summer monsoon, regional mountain‐valley winds between the Himalayas and South Asia, and local mountain‐valley winds circulation.
Key Points
Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and secondary organic matter was the major aerosol component
The evolution of aerosols was mainly characterized by diurnal variation that was related to transport mechanism over Yadong
The Himalayas‐South Asia regional mountain‐valley winds combined with local mountain‐valley winds transport aerosols to the Tibetan Plateau</description><identifier>ISSN: 2169-897X</identifier><identifier>EISSN: 2169-8996</identifier><identifier>DOI: 10.1029/2023JD040193</identifier><language>eng</language><publisher>Washington: Blackwell Publishing Ltd</publisher><subject>Aerosol absorption ; Aerosols ; Air masses ; Air pollution ; Albedo ; Atmospheric aerosols ; Atmospheric processes ; Black carbon ; Boundary layers ; Chemical properties ; Chemicophysical properties ; Diurnal variations ; Himalayas‐South Asia regional mountain‐valley winds ; in situ observations ; local mountain‐valley winds ; Monsoons ; Mountains ; Organic carbon ; Organic matter ; Physical properties ; Physicochemical processes ; Physicochemical properties ; Plateaus ; Pollutants ; Pollution dispersion ; Pollution transport ; Remote regions ; Satellite observation ; Scattering ; Secondary aerosols ; Slopes ; Summer ; Summer monsoon ; Valley winds ; Valleys ; Wavelength ; Wind ; Winds</subject><ispartof>Journal of geophysical research. Atmospheres, 2024-02, Vol.129 (4), p.n/a</ispartof><rights>2024. American Geophysical Union. All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c2640-fbfa5b723c106bcb924645c74bd6281a794841fdd180f3529e90ed9a14d765c43</cites><orcidid>0000-0002-9934-895X ; 0000-0003-2845-797X ; 0000-0002-4342-4159 ; 0000-0001-8140-4928</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1029%2F2023JD040193$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1029%2F2023JD040193$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,27903,27904,45553,45554</link.rule.ids></links><search><creatorcontrib>Yu, Zeren</creatorcontrib><creatorcontrib>Tian, Pengfei</creatorcontrib><creatorcontrib>Kang, Chenliang</creatorcontrib><creatorcontrib>Song, Xin</creatorcontrib><creatorcontrib>Huang, Jianping</creatorcontrib><creatorcontrib>Guo, Yumin</creatorcontrib><creatorcontrib>Shi, Jinsen</creatorcontrib><creatorcontrib>Tang, Chenguang</creatorcontrib><creatorcontrib>Zhang, Haotian</creatorcontrib><creatorcontrib>Zhang, Zhida</creatorcontrib><creatorcontrib>Cao, Xianjie</creatorcontrib><creatorcontrib>Liang, Jiening</creatorcontrib><creatorcontrib>Zhang, Lei</creatorcontrib><title>Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau</title><title>Journal of geophysical research. Atmospheres</title><description>The physicochemical properties and origins of atmospheric aerosols in the Tibetan Plateau (TP) region are a research topic of great interest, but an in‐depth understanding of this topic is challenging, partially due to a lack of intensive in situ observations. Thus, a field campaign was conducted over Yadong, a remote area on the south slope of the TP from June 11 to 31 August 2021. The aerosol loading was low, with a black carbon mass concentration of 147.4 ± 98.4 ng·m−3. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and increased from 450 to 700 nm wavelength. Organic matter (OM) accounting for 69.6% of the total aerosol mass and relatively high secondary organic carbon ratios, highlighting the importance of secondary formation. An interesting phenomenon observed was that the evolution of aerosols was mainly characterized by diurnal variation, which could not be explained by large‐scale atmospheric processes such as Indian summer monsoon. Instead, it was found that regional mountain‐valley winds between the Himalayas and South Asia transported polluted air masses toward the TP, especially in the afternoon when regional valley wind are expected to be the strongest and the boundary layer in South Asia is deepest. Additionally, daytime local valley wind further elevated these aerosols to higher altitudes on the TP. This paper provides insights into the transport mechanisms of aerosols from South Asia to the TP. These findings are of great importance since aerosols exhibit significant diurnal variations in the TP region.
Plain Language Summary
Previous studies focused on the analysis of the physical or chemical properties of aerosols on the Tibetan Plateau, but this study provides a comprehensive examination of both. The findings reveal that aerosols on the southern slope of the Tibetan Plateau exhibit strong absorption efficiency. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm), which may be attributed to aerosol secondary generation and coating. Finally, the mechanism of pollutant transport from South Asia to the Tibetan Plateau was analyzed relies on site observations, satellite, and reanalysis data to highlight the link between diurnal variations of pollutants and transport mechanism. The specific transport mechanism be understood uniformly across different scales, including Indian summer monsoon, regional mountain‐valley winds between the Himalayas and South Asia, and local mountain‐valley winds circulation.
Key Points
Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and secondary organic matter was the major aerosol component
The evolution of aerosols was mainly characterized by diurnal variation that was related to transport mechanism over Yadong
The Himalayas‐South Asia regional mountain‐valley winds combined with local mountain‐valley winds transport aerosols to the Tibetan Plateau</description><subject>Aerosol absorption</subject><subject>Aerosols</subject><subject>Air masses</subject><subject>Air pollution</subject><subject>Albedo</subject><subject>Atmospheric aerosols</subject><subject>Atmospheric processes</subject><subject>Black carbon</subject><subject>Boundary layers</subject><subject>Chemical properties</subject><subject>Chemicophysical properties</subject><subject>Diurnal variations</subject><subject>Himalayas‐South Asia regional mountain‐valley winds</subject><subject>in situ observations</subject><subject>local mountain‐valley winds</subject><subject>Monsoons</subject><subject>Mountains</subject><subject>Organic carbon</subject><subject>Organic matter</subject><subject>Physical properties</subject><subject>Physicochemical processes</subject><subject>Physicochemical properties</subject><subject>Plateaus</subject><subject>Pollutants</subject><subject>Pollution dispersion</subject><subject>Pollution transport</subject><subject>Remote regions</subject><subject>Satellite observation</subject><subject>Scattering</subject><subject>Secondary aerosols</subject><subject>Slopes</subject><subject>Summer</subject><subject>Summer monsoon</subject><subject>Valley winds</subject><subject>Valleys</subject><subject>Wavelength</subject><subject>Wind</subject><subject>Winds</subject><issn>2169-897X</issn><issn>2169-8996</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kN1Kw0AQhYMoWGrvfIAFb1vdv_zsZUi1WiotbQXvwmYzISlJNu5ulT6Jr2tqRbxybmY4fDOHOZ53TfAtwVTcUUzZfIo5JoKdeQNKAjGJhAjOf-fw9dIbWbvDfUWYcZ8PvM9VebCVkjVaGd2BcRXYMUpKaL7FRDedbqF1vSjbHG2NbG2njUPPoErZVraxSBcodo22XQmmUigGo62uLVq-g0ESraHRDlBsQCLdIlcC2ui9K9Gm7h2P20dpW2XgZItWtXQg91feRSFrC6OfPvReHu63yeNksZw9JfFiomjA8aTICulnIWWK4CBTmaA84L4KeZYHNCIyFDzipMhzEuGC-VSAwJALSXgeBr7ibOjdnO52Rr_twbp0p_em7S1TKhgJSMQo6anxiVL9a9ZAkXamaqQ5pASnx_TTv-n3ODvhH1UNh3_ZdD5bT_3eCbMvkK6Gjg</recordid><startdate>20240228</startdate><enddate>20240228</enddate><creator>Yu, Zeren</creator><creator>Tian, Pengfei</creator><creator>Kang, Chenliang</creator><creator>Song, Xin</creator><creator>Huang, Jianping</creator><creator>Guo, Yumin</creator><creator>Shi, Jinsen</creator><creator>Tang, Chenguang</creator><creator>Zhang, Haotian</creator><creator>Zhang, Zhida</creator><creator>Cao, Xianjie</creator><creator>Liang, Jiening</creator><creator>Zhang, Lei</creator><general>Blackwell Publishing Ltd</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7TG</scope><scope>7UA</scope><scope>8FD</scope><scope>C1K</scope><scope>F1W</scope><scope>FR3</scope><scope>H8D</scope><scope>H96</scope><scope>KL.</scope><scope>KR7</scope><scope>L.G</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0002-9934-895X</orcidid><orcidid>https://orcid.org/0000-0003-2845-797X</orcidid><orcidid>https://orcid.org/0000-0002-4342-4159</orcidid><orcidid>https://orcid.org/0000-0001-8140-4928</orcidid></search><sort><creationdate>20240228</creationdate><title>Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau</title><author>Yu, Zeren ; Tian, Pengfei ; Kang, Chenliang ; Song, Xin ; Huang, Jianping ; Guo, Yumin ; Shi, Jinsen ; Tang, Chenguang ; Zhang, Haotian ; Zhang, Zhida ; Cao, Xianjie ; Liang, Jiening ; Zhang, Lei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c2640-fbfa5b723c106bcb924645c74bd6281a794841fdd180f3529e90ed9a14d765c43</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Aerosol absorption</topic><topic>Aerosols</topic><topic>Air masses</topic><topic>Air pollution</topic><topic>Albedo</topic><topic>Atmospheric aerosols</topic><topic>Atmospheric processes</topic><topic>Black carbon</topic><topic>Boundary layers</topic><topic>Chemical properties</topic><topic>Chemicophysical properties</topic><topic>Diurnal variations</topic><topic>Himalayas‐South Asia regional mountain‐valley winds</topic><topic>in situ observations</topic><topic>local mountain‐valley winds</topic><topic>Monsoons</topic><topic>Mountains</topic><topic>Organic carbon</topic><topic>Organic matter</topic><topic>Physical properties</topic><topic>Physicochemical processes</topic><topic>Physicochemical properties</topic><topic>Plateaus</topic><topic>Pollutants</topic><topic>Pollution dispersion</topic><topic>Pollution transport</topic><topic>Remote regions</topic><topic>Satellite observation</topic><topic>Scattering</topic><topic>Secondary aerosols</topic><topic>Slopes</topic><topic>Summer</topic><topic>Summer monsoon</topic><topic>Valley winds</topic><topic>Valleys</topic><topic>Wavelength</topic><topic>Wind</topic><topic>Winds</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yu, Zeren</creatorcontrib><creatorcontrib>Tian, Pengfei</creatorcontrib><creatorcontrib>Kang, Chenliang</creatorcontrib><creatorcontrib>Song, Xin</creatorcontrib><creatorcontrib>Huang, Jianping</creatorcontrib><creatorcontrib>Guo, Yumin</creatorcontrib><creatorcontrib>Shi, Jinsen</creatorcontrib><creatorcontrib>Tang, Chenguang</creatorcontrib><creatorcontrib>Zhang, Haotian</creatorcontrib><creatorcontrib>Zhang, Zhida</creatorcontrib><creatorcontrib>Cao, Xianjie</creatorcontrib><creatorcontrib>Liang, Jiening</creatorcontrib><creatorcontrib>Zhang, Lei</creatorcontrib><collection>CrossRef</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Water Resources Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Engineering Research Database</collection><collection>Aerospace Database</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Civil Engineering Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Journal of geophysical research. Atmospheres</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yu, Zeren</au><au>Tian, Pengfei</au><au>Kang, Chenliang</au><au>Song, Xin</au><au>Huang, Jianping</au><au>Guo, Yumin</au><au>Shi, Jinsen</au><au>Tang, Chenguang</au><au>Zhang, Haotian</au><au>Zhang, Zhida</au><au>Cao, Xianjie</au><au>Liang, Jiening</au><au>Zhang, Lei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau</atitle><jtitle>Journal of geophysical research. Atmospheres</jtitle><date>2024-02-28</date><risdate>2024</risdate><volume>129</volume><issue>4</issue><epage>n/a</epage><issn>2169-897X</issn><eissn>2169-8996</eissn><abstract>The physicochemical properties and origins of atmospheric aerosols in the Tibetan Plateau (TP) region are a research topic of great interest, but an in‐depth understanding of this topic is challenging, partially due to a lack of intensive in situ observations. Thus, a field campaign was conducted over Yadong, a remote area on the south slope of the TP from June 11 to 31 August 2021. The aerosol loading was low, with a black carbon mass concentration of 147.4 ± 98.4 ng·m−3. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and increased from 450 to 700 nm wavelength. Organic matter (OM) accounting for 69.6% of the total aerosol mass and relatively high secondary organic carbon ratios, highlighting the importance of secondary formation. An interesting phenomenon observed was that the evolution of aerosols was mainly characterized by diurnal variation, which could not be explained by large‐scale atmospheric processes such as Indian summer monsoon. Instead, it was found that regional mountain‐valley winds between the Himalayas and South Asia transported polluted air masses toward the TP, especially in the afternoon when regional valley wind are expected to be the strongest and the boundary layer in South Asia is deepest. Additionally, daytime local valley wind further elevated these aerosols to higher altitudes on the TP. This paper provides insights into the transport mechanisms of aerosols from South Asia to the TP. These findings are of great importance since aerosols exhibit significant diurnal variations in the TP region.
Plain Language Summary
Previous studies focused on the analysis of the physical or chemical properties of aerosols on the Tibetan Plateau, but this study provides a comprehensive examination of both. The findings reveal that aerosols on the southern slope of the Tibetan Plateau exhibit strong absorption efficiency. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm), which may be attributed to aerosol secondary generation and coating. Finally, the mechanism of pollutant transport from South Asia to the Tibetan Plateau was analyzed relies on site observations, satellite, and reanalysis data to highlight the link between diurnal variations of pollutants and transport mechanism. The specific transport mechanism be understood uniformly across different scales, including Indian summer monsoon, regional mountain‐valley winds between the Himalayas and South Asia, and local mountain‐valley winds circulation.
Key Points
Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and secondary organic matter was the major aerosol component
The evolution of aerosols was mainly characterized by diurnal variation that was related to transport mechanism over Yadong
The Himalayas‐South Asia regional mountain‐valley winds combined with local mountain‐valley winds transport aerosols to the Tibetan Plateau</abstract><cop>Washington</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1029/2023JD040193</doi><tpages>19</tpages><orcidid>https://orcid.org/0000-0002-9934-895X</orcidid><orcidid>https://orcid.org/0000-0003-2845-797X</orcidid><orcidid>https://orcid.org/0000-0002-4342-4159</orcidid><orcidid>https://orcid.org/0000-0001-8140-4928</orcidid></addata></record> |
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subjects | Aerosol absorption Aerosols Air masses Air pollution Albedo Atmospheric aerosols Atmospheric processes Black carbon Boundary layers Chemical properties Chemicophysical properties Diurnal variations Himalayas‐South Asia regional mountain‐valley winds in situ observations local mountain‐valley winds Monsoons Mountains Organic carbon Organic matter Physical properties Physicochemical processes Physicochemical properties Plateaus Pollutants Pollution dispersion Pollution transport Remote regions Satellite observation Scattering Secondary aerosols Slopes Summer Summer monsoon Valley winds Valleys Wavelength Wind Winds |
title | Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau |
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