Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau

The physicochemical properties and origins of atmospheric aerosols in the Tibetan Plateau (TP) region are a research topic of great interest, but an in‐depth understanding of this topic is challenging, partially due to a lack of intensive in situ observations. Thus, a field campaign was conducted ov...

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Veröffentlicht in:Journal of geophysical research. Atmospheres 2024-02, Vol.129 (4), p.n/a
Hauptverfasser: Yu, Zeren, Tian, Pengfei, Kang, Chenliang, Song, Xin, Huang, Jianping, Guo, Yumin, Shi, Jinsen, Tang, Chenguang, Zhang, Haotian, Zhang, Zhida, Cao, Xianjie, Liang, Jiening, Zhang, Lei
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container_title Journal of geophysical research. Atmospheres
container_volume 129
creator Yu, Zeren
Tian, Pengfei
Kang, Chenliang
Song, Xin
Huang, Jianping
Guo, Yumin
Shi, Jinsen
Tang, Chenguang
Zhang, Haotian
Zhang, Zhida
Cao, Xianjie
Liang, Jiening
Zhang, Lei
description The physicochemical properties and origins of atmospheric aerosols in the Tibetan Plateau (TP) region are a research topic of great interest, but an in‐depth understanding of this topic is challenging, partially due to a lack of intensive in situ observations. Thus, a field campaign was conducted over Yadong, a remote area on the south slope of the TP from June 11 to 31 August 2021. The aerosol loading was low, with a black carbon mass concentration of 147.4 ± 98.4 ng·m−3. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and increased from 450 to 700 nm wavelength. Organic matter (OM) accounting for 69.6% of the total aerosol mass and relatively high secondary organic carbon ratios, highlighting the importance of secondary formation. An interesting phenomenon observed was that the evolution of aerosols was mainly characterized by diurnal variation, which could not be explained by large‐scale atmospheric processes such as Indian summer monsoon. Instead, it was found that regional mountain‐valley winds between the Himalayas and South Asia transported polluted air masses toward the TP, especially in the afternoon when regional valley wind are expected to be the strongest and the boundary layer in South Asia is deepest. Additionally, daytime local valley wind further elevated these aerosols to higher altitudes on the TP. This paper provides insights into the transport mechanisms of aerosols from South Asia to the TP. These findings are of great importance since aerosols exhibit significant diurnal variations in the TP region. Plain Language Summary Previous studies focused on the analysis of the physical or chemical properties of aerosols on the Tibetan Plateau, but this study provides a comprehensive examination of both. The findings reveal that aerosols on the southern slope of the Tibetan Plateau exhibit strong absorption efficiency. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm), which may be attributed to aerosol secondary generation and coating. Finally, the mechanism of pollutant transport from South Asia to the Tibetan Plateau was analyzed relies on site observations, satellite, and reanalysis data to highlight the link between diurnal variations of pollutants and transport mechanism. The specific transport mechanism be understood uniformly across different scales, including Indian summer monsoon, regional mountain‐valley winds between the Himalayas and South Asia, and local mountain‐valley winds circulation. Key Point
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Thus, a field campaign was conducted over Yadong, a remote area on the south slope of the TP from June 11 to 31 August 2021. The aerosol loading was low, with a black carbon mass concentration of 147.4 ± 98.4 ng·m−3. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and increased from 450 to 700 nm wavelength. Organic matter (OM) accounting for 69.6% of the total aerosol mass and relatively high secondary organic carbon ratios, highlighting the importance of secondary formation. An interesting phenomenon observed was that the evolution of aerosols was mainly characterized by diurnal variation, which could not be explained by large‐scale atmospheric processes such as Indian summer monsoon. Instead, it was found that regional mountain‐valley winds between the Himalayas and South Asia transported polluted air masses toward the TP, especially in the afternoon when regional valley wind are expected to be the strongest and the boundary layer in South Asia is deepest. Additionally, daytime local valley wind further elevated these aerosols to higher altitudes on the TP. This paper provides insights into the transport mechanisms of aerosols from South Asia to the TP. These findings are of great importance since aerosols exhibit significant diurnal variations in the TP region. Plain Language Summary Previous studies focused on the analysis of the physical or chemical properties of aerosols on the Tibetan Plateau, but this study provides a comprehensive examination of both. The findings reveal that aerosols on the southern slope of the Tibetan Plateau exhibit strong absorption efficiency. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm), which may be attributed to aerosol secondary generation and coating. Finally, the mechanism of pollutant transport from South Asia to the Tibetan Plateau was analyzed relies on site observations, satellite, and reanalysis data to highlight the link between diurnal variations of pollutants and transport mechanism. The specific transport mechanism be understood uniformly across different scales, including Indian summer monsoon, regional mountain‐valley winds between the Himalayas and South Asia, and local mountain‐valley winds circulation. Key Points Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and secondary organic matter was the major aerosol component The evolution of aerosols was mainly characterized by diurnal variation that was related to transport mechanism over Yadong The Himalayas‐South Asia regional mountain‐valley winds combined with local mountain‐valley winds transport aerosols to the Tibetan Plateau</description><identifier>ISSN: 2169-897X</identifier><identifier>EISSN: 2169-8996</identifier><identifier>DOI: 10.1029/2023JD040193</identifier><language>eng</language><publisher>Washington: Blackwell Publishing Ltd</publisher><subject>Aerosol absorption ; Aerosols ; Air masses ; Air pollution ; Albedo ; Atmospheric aerosols ; Atmospheric processes ; Black carbon ; Boundary layers ; Chemical properties ; Chemicophysical properties ; Diurnal variations ; Himalayas‐South Asia regional mountain‐valley winds ; in situ observations ; local mountain‐valley winds ; Monsoons ; Mountains ; Organic carbon ; Organic matter ; Physical properties ; Physicochemical processes ; Physicochemical properties ; Plateaus ; Pollutants ; Pollution dispersion ; Pollution transport ; Remote regions ; Satellite observation ; Scattering ; Secondary aerosols ; Slopes ; Summer ; Summer monsoon ; Valley winds ; Valleys ; Wavelength ; Wind ; Winds</subject><ispartof>Journal of geophysical research. Atmospheres, 2024-02, Vol.129 (4), p.n/a</ispartof><rights>2024. American Geophysical Union. All Rights Reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c2640-fbfa5b723c106bcb924645c74bd6281a794841fdd180f3529e90ed9a14d765c43</cites><orcidid>0000-0002-9934-895X ; 0000-0003-2845-797X ; 0000-0002-4342-4159 ; 0000-0001-8140-4928</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1029%2F2023JD040193$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1029%2F2023JD040193$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,27903,27904,45553,45554</link.rule.ids></links><search><creatorcontrib>Yu, Zeren</creatorcontrib><creatorcontrib>Tian, Pengfei</creatorcontrib><creatorcontrib>Kang, Chenliang</creatorcontrib><creatorcontrib>Song, Xin</creatorcontrib><creatorcontrib>Huang, Jianping</creatorcontrib><creatorcontrib>Guo, Yumin</creatorcontrib><creatorcontrib>Shi, Jinsen</creatorcontrib><creatorcontrib>Tang, Chenguang</creatorcontrib><creatorcontrib>Zhang, Haotian</creatorcontrib><creatorcontrib>Zhang, Zhida</creatorcontrib><creatorcontrib>Cao, Xianjie</creatorcontrib><creatorcontrib>Liang, Jiening</creatorcontrib><creatorcontrib>Zhang, Lei</creatorcontrib><title>Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau</title><title>Journal of geophysical research. Atmospheres</title><description>The physicochemical properties and origins of atmospheric aerosols in the Tibetan Plateau (TP) region are a research topic of great interest, but an in‐depth understanding of this topic is challenging, partially due to a lack of intensive in situ observations. Thus, a field campaign was conducted over Yadong, a remote area on the south slope of the TP from June 11 to 31 August 2021. The aerosol loading was low, with a black carbon mass concentration of 147.4 ± 98.4 ng·m−3. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and increased from 450 to 700 nm wavelength. Organic matter (OM) accounting for 69.6% of the total aerosol mass and relatively high secondary organic carbon ratios, highlighting the importance of secondary formation. An interesting phenomenon observed was that the evolution of aerosols was mainly characterized by diurnal variation, which could not be explained by large‐scale atmospheric processes such as Indian summer monsoon. Instead, it was found that regional mountain‐valley winds between the Himalayas and South Asia transported polluted air masses toward the TP, especially in the afternoon when regional valley wind are expected to be the strongest and the boundary layer in South Asia is deepest. Additionally, daytime local valley wind further elevated these aerosols to higher altitudes on the TP. This paper provides insights into the transport mechanisms of aerosols from South Asia to the TP. These findings are of great importance since aerosols exhibit significant diurnal variations in the TP region. Plain Language Summary Previous studies focused on the analysis of the physical or chemical properties of aerosols on the Tibetan Plateau, but this study provides a comprehensive examination of both. The findings reveal that aerosols on the southern slope of the Tibetan Plateau exhibit strong absorption efficiency. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm), which may be attributed to aerosol secondary generation and coating. Finally, the mechanism of pollutant transport from South Asia to the Tibetan Plateau was analyzed relies on site observations, satellite, and reanalysis data to highlight the link between diurnal variations of pollutants and transport mechanism. The specific transport mechanism be understood uniformly across different scales, including Indian summer monsoon, regional mountain‐valley winds between the Himalayas and South Asia, and local mountain‐valley winds circulation. Key Points Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and secondary organic matter was the major aerosol component The evolution of aerosols was mainly characterized by diurnal variation that was related to transport mechanism over Yadong The Himalayas‐South Asia regional mountain‐valley winds combined with local mountain‐valley winds transport aerosols to the Tibetan Plateau</description><subject>Aerosol absorption</subject><subject>Aerosols</subject><subject>Air masses</subject><subject>Air pollution</subject><subject>Albedo</subject><subject>Atmospheric aerosols</subject><subject>Atmospheric processes</subject><subject>Black carbon</subject><subject>Boundary layers</subject><subject>Chemical properties</subject><subject>Chemicophysical properties</subject><subject>Diurnal variations</subject><subject>Himalayas‐South Asia regional mountain‐valley winds</subject><subject>in situ observations</subject><subject>local mountain‐valley winds</subject><subject>Monsoons</subject><subject>Mountains</subject><subject>Organic carbon</subject><subject>Organic matter</subject><subject>Physical properties</subject><subject>Physicochemical processes</subject><subject>Physicochemical properties</subject><subject>Plateaus</subject><subject>Pollutants</subject><subject>Pollution dispersion</subject><subject>Pollution transport</subject><subject>Remote regions</subject><subject>Satellite observation</subject><subject>Scattering</subject><subject>Secondary aerosols</subject><subject>Slopes</subject><subject>Summer</subject><subject>Summer monsoon</subject><subject>Valley winds</subject><subject>Valleys</subject><subject>Wavelength</subject><subject>Wind</subject><subject>Winds</subject><issn>2169-897X</issn><issn>2169-8996</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kN1Kw0AQhYMoWGrvfIAFb1vdv_zsZUi1WiotbQXvwmYzISlJNu5ulT6Jr2tqRbxybmY4fDOHOZ53TfAtwVTcUUzZfIo5JoKdeQNKAjGJhAjOf-fw9dIbWbvDfUWYcZ8PvM9VebCVkjVaGd2BcRXYMUpKaL7FRDedbqF1vSjbHG2NbG2njUPPoErZVraxSBcodo22XQmmUigGo62uLVq-g0ESraHRDlBsQCLdIlcC2ui9K9Gm7h2P20dpW2XgZItWtXQg91feRSFrC6OfPvReHu63yeNksZw9JfFiomjA8aTICulnIWWK4CBTmaA84L4KeZYHNCIyFDzipMhzEuGC-VSAwJALSXgeBr7ibOjdnO52Rr_twbp0p_em7S1TKhgJSMQo6anxiVL9a9ZAkXamaqQ5pASnx_TTv-n3ODvhH1UNh3_ZdD5bT_3eCbMvkK6Gjg</recordid><startdate>20240228</startdate><enddate>20240228</enddate><creator>Yu, Zeren</creator><creator>Tian, Pengfei</creator><creator>Kang, Chenliang</creator><creator>Song, Xin</creator><creator>Huang, Jianping</creator><creator>Guo, Yumin</creator><creator>Shi, Jinsen</creator><creator>Tang, Chenguang</creator><creator>Zhang, Haotian</creator><creator>Zhang, Zhida</creator><creator>Cao, Xianjie</creator><creator>Liang, Jiening</creator><creator>Zhang, Lei</creator><general>Blackwell Publishing Ltd</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7TG</scope><scope>7UA</scope><scope>8FD</scope><scope>C1K</scope><scope>F1W</scope><scope>FR3</scope><scope>H8D</scope><scope>H96</scope><scope>KL.</scope><scope>KR7</scope><scope>L.G</scope><scope>L7M</scope><orcidid>https://orcid.org/0000-0002-9934-895X</orcidid><orcidid>https://orcid.org/0000-0003-2845-797X</orcidid><orcidid>https://orcid.org/0000-0002-4342-4159</orcidid><orcidid>https://orcid.org/0000-0001-8140-4928</orcidid></search><sort><creationdate>20240228</creationdate><title>Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau</title><author>Yu, Zeren ; 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Atmospheres</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yu, Zeren</au><au>Tian, Pengfei</au><au>Kang, Chenliang</au><au>Song, Xin</au><au>Huang, Jianping</au><au>Guo, Yumin</au><au>Shi, Jinsen</au><au>Tang, Chenguang</au><au>Zhang, Haotian</au><au>Zhang, Zhida</au><au>Cao, Xianjie</au><au>Liang, Jiening</au><au>Zhang, Lei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau</atitle><jtitle>Journal of geophysical research. Atmospheres</jtitle><date>2024-02-28</date><risdate>2024</risdate><volume>129</volume><issue>4</issue><epage>n/a</epage><issn>2169-897X</issn><eissn>2169-8996</eissn><abstract>The physicochemical properties and origins of atmospheric aerosols in the Tibetan Plateau (TP) region are a research topic of great interest, but an in‐depth understanding of this topic is challenging, partially due to a lack of intensive in situ observations. Thus, a field campaign was conducted over Yadong, a remote area on the south slope of the TP from June 11 to 31 August 2021. The aerosol loading was low, with a black carbon mass concentration of 147.4 ± 98.4 ng·m−3. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and increased from 450 to 700 nm wavelength. Organic matter (OM) accounting for 69.6% of the total aerosol mass and relatively high secondary organic carbon ratios, highlighting the importance of secondary formation. An interesting phenomenon observed was that the evolution of aerosols was mainly characterized by diurnal variation, which could not be explained by large‐scale atmospheric processes such as Indian summer monsoon. Instead, it was found that regional mountain‐valley winds between the Himalayas and South Asia transported polluted air masses toward the TP, especially in the afternoon when regional valley wind are expected to be the strongest and the boundary layer in South Asia is deepest. Additionally, daytime local valley wind further elevated these aerosols to higher altitudes on the TP. This paper provides insights into the transport mechanisms of aerosols from South Asia to the TP. These findings are of great importance since aerosols exhibit significant diurnal variations in the TP region. Plain Language Summary Previous studies focused on the analysis of the physical or chemical properties of aerosols on the Tibetan Plateau, but this study provides a comprehensive examination of both. The findings reveal that aerosols on the southern slope of the Tibetan Plateau exhibit strong absorption efficiency. Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm), which may be attributed to aerosol secondary generation and coating. Finally, the mechanism of pollutant transport from South Asia to the Tibetan Plateau was analyzed relies on site observations, satellite, and reanalysis data to highlight the link between diurnal variations of pollutants and transport mechanism. The specific transport mechanism be understood uniformly across different scales, including Indian summer monsoon, regional mountain‐valley winds between the Himalayas and South Asia, and local mountain‐valley winds circulation. Key Points Aerosol single‐scattering albedo was low (0.73 ± 0.11 at 550 nm) and secondary organic matter was the major aerosol component The evolution of aerosols was mainly characterized by diurnal variation that was related to transport mechanism over Yadong The Himalayas‐South Asia regional mountain‐valley winds combined with local mountain‐valley winds transport aerosols to the Tibetan Plateau</abstract><cop>Washington</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1029/2023JD040193</doi><tpages>19</tpages><orcidid>https://orcid.org/0000-0002-9934-895X</orcidid><orcidid>https://orcid.org/0000-0003-2845-797X</orcidid><orcidid>https://orcid.org/0000-0002-4342-4159</orcidid><orcidid>https://orcid.org/0000-0001-8140-4928</orcidid></addata></record>
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subjects Aerosol absorption
Aerosols
Air masses
Air pollution
Albedo
Atmospheric aerosols
Atmospheric processes
Black carbon
Boundary layers
Chemical properties
Chemicophysical properties
Diurnal variations
Himalayas‐South Asia regional mountain‐valley winds
in situ observations
local mountain‐valley winds
Monsoons
Mountains
Organic carbon
Organic matter
Physical properties
Physicochemical processes
Physicochemical properties
Plateaus
Pollutants
Pollution dispersion
Pollution transport
Remote regions
Satellite observation
Scattering
Secondary aerosols
Slopes
Summer
Summer monsoon
Valley winds
Valleys
Wavelength
Wind
Winds
title Physical Properties, Chemical Components, and Transport Mechanisms of Atmospheric Aerosols Over a Remote Area on the South Slope of the Tibetan Plateau
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