Electrically tunable nonlinear Faraday ellipticity and rotation in WTe2

There has been considerable interest in the nonlinear optical phenomenon in recent years, particularly in two-dimensional materials. Here, we study the optical polarization quantities namely ellipticity and Faraday rotation for the monolayer 1T ′ -WTe 2 two-dimensional (2D) material. We develop a ne...

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Veröffentlicht in:European physical journal plus 2024-01, Vol.139 (1), p.96
Hauptverfasser: Pandey, Vivek, Dasari, Navya Teja, M, Bhargavi, Reddy, Salla Gangi, Bhalla, Pankaj
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Dasari, Navya Teja
M, Bhargavi
Reddy, Salla Gangi
Bhalla, Pankaj
description There has been considerable interest in the nonlinear optical phenomenon in recent years, particularly in two-dimensional materials. Here, we study the optical polarization quantities namely ellipticity and Faraday rotation for the monolayer 1T ′ -WTe 2 two-dimensional (2D) material. We develop a new general approach based on many-body perturbation theory to compute polarization quantities via the second harmonic susceptibility of the material. We find that the nonlinear second-harmonic longitudinal and transverse responses are tunable with the inclination angle made by the out-of-plane field with an axis vertical to the 2D plane. This field breaks the inversion symmetry of the system which is an essential condition for the behavior of the second harmonic susceptibility. Such tunable behavior gives significant variation to the Faraday rotation and ellipticity. Our findings provide valuable information for future experiments on the optical phenomenon in 2D materials.
doi_str_mv 10.1140/epjp/s13360-024-04893-x
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subjects Applied and Technical Physics
Atomic
Complex Systems
Condensed Matter Physics
Electric fields
Electromagnetism
Electrons
Ellipticity
Energy
Faraday effect
Fourier transforms
Inclination angle
Magnetic fields
Mathematical and Computational Physics
Molecular
Nonlinear optics
Optical and Plasma Physics
Optical polarization
Perturbation theory
Physics
Physics and Astronomy
Regular Article
Symmetry
Theoretical
Two dimensional materials
title Electrically tunable nonlinear Faraday ellipticity and rotation in WTe2
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