Effects of Fe3+ on Dissolution Dynamics of Carbonate Rocks in a Shallow Burial Reservoir
Dissolution of carbonates in acidic fluids, which has attracted much research attention in recent years, is of great significance for the formation of high-quality reservoirs. The dissolution stage under low temperature and low pressure in shallow burial is one of the most important processes of res...
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| creator | Ma, Jiayi Xie, Shuyun Liu, Dan Carranza, Emmanuel John M. He, Zhiliang Zhang, Mohai Wang, Tianyi |
| description | Dissolution of carbonates in acidic fluids, which has attracted much research attention in recent years, is of great significance for the formation of high-quality reservoirs. The dissolution stage under low temperature and low pressure in shallow burial is one of the most important processes of reservoir dissolution and transformation. However, the dissolution dynamics of carbonate rocks in shallow burial and their formation have been controversial for a long time, and there are still disputes in the dissolution processes about how associated minerals and accessory minerals (e.g., pyrite) in carbonate reservoirs influence the formation of secondary pores. Additional metal ions in acidic fluids can change fluid properties and dissolution processes, and consequently affect reservoir quality. However, there are few laboratory studies done on the effect of associated minerals on the dissolution dynamics of carbonates. To clarify the specific impact of Fe-bearing associated minerals and Fe
3+
on the dissolution of carbonates in shallow burial reservoirs, six samples of typical carbonate rocks in the Zigui area of Hubei Province, China were studied. The dissolution kinetics of carbonates in dilute hydrochloric acid and sulfuric acid solutions containing metal ions (Fe
3+
/Ca
2+
/Mn
2+
) at ambient temperature and pressure (T = 25 °C, P = 1 atm) were studied, by laboratory dissolution experiments combined with numerical simulations using PHREEQC. The results show that the Fe
3+
is of great significance on the dissolution of carbonate rocks, while the influences of Ca
2+
and Mn
2+
are relatively weak. The dissolutions degrees of micritic limestone (ZG-L25), dolomitic limestone (ZG-L7) and dolomite (ZG-D9) were better than the other carbonates under the influence of metal ions (Fe
3+
/Ca
2+
/Mn
2+
) in acid solutions. Therefore, the dolomite reservoir of the Cambrian Qinjiamiao Formation, the dolomitic limestone reservoir of the Tianheban Formation and the limestone reservoir of the Triassic Daye Formation in the Zigui area are potential high-quality reservoirs. The carbonate reservoirs associated with Fe-bearing minerals were easier to dissolve and formed secondary pores under shallow burial. This process is beneficial to the formation of high-quality reservoirs. Moreover, the addition of Fe
3+
into hydrochloric acid solution may be conducive to improving the reservoirs acidizing effect. Furthermore, the results gave innovative results from multiple perspectives |
| doi_str_mv | 10.1007/s11053-020-09765-6 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2918337012</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2918337012</sourcerecordid><originalsourceid>FETCH-LOGICAL-c1646-ba84c72dc5b22ebc544ba24ba537f77628b69bdef8f1cf987bcb120d8656f5d13</originalsourceid><addsrcrecordid>eNp9kMtKAzEUhoMoWKsv4CrgUkZzmVxmqbVVoSBUBXchySQ6dTrRZEbp25u2gjsXh3Pgvxz4ADjF6AIjJC4TxojRAhFUoEpwVvA9MMJM0EJWEu9v7iyJklaH4CilJcohKtkIvEy9d7ZPMHg4c_Qchg7eNCmFduibzb3u9KqxW32iowmd7h1cBPueYNNBDR_fdNuGb3g9xEa3cOGSi1-hicfgwOs2uZPfPQbPs-nT5K6YP9zeT67mhcW85IXRsrSC1JYZQpyxrCyNJnkYFV4ITqThlamdlx5bX0lhrMEE1ZIz7lmN6Ric7Xo_YvgcXOrVMgyxyy8VqbCkVCBMsovsXDaGlKLz6iM2Kx3XCiO1Iah2BFUmqLYEFc8hugulbO5eXfyr_if1Awv-cw4</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2918337012</pqid></control><display><type>article</type><title>Effects of Fe3+ on Dissolution Dynamics of Carbonate Rocks in a Shallow Burial Reservoir</title><source>Springer Nature - Complete Springer Journals</source><source>ProQuest Central UK/Ireland</source><source>ProQuest Central</source><creator>Ma, Jiayi ; Xie, Shuyun ; Liu, Dan ; Carranza, Emmanuel John M. ; He, Zhiliang ; Zhang, Mohai ; Wang, Tianyi</creator><creatorcontrib>Ma, Jiayi ; Xie, Shuyun ; Liu, Dan ; Carranza, Emmanuel John M. ; He, Zhiliang ; Zhang, Mohai ; Wang, Tianyi</creatorcontrib><description>Dissolution of carbonates in acidic fluids, which has attracted much research attention in recent years, is of great significance for the formation of high-quality reservoirs. The dissolution stage under low temperature and low pressure in shallow burial is one of the most important processes of reservoir dissolution and transformation. However, the dissolution dynamics of carbonate rocks in shallow burial and their formation have been controversial for a long time, and there are still disputes in the dissolution processes about how associated minerals and accessory minerals (e.g., pyrite) in carbonate reservoirs influence the formation of secondary pores. Additional metal ions in acidic fluids can change fluid properties and dissolution processes, and consequently affect reservoir quality. However, there are few laboratory studies done on the effect of associated minerals on the dissolution dynamics of carbonates. To clarify the specific impact of Fe-bearing associated minerals and Fe
3+
on the dissolution of carbonates in shallow burial reservoirs, six samples of typical carbonate rocks in the Zigui area of Hubei Province, China were studied. The dissolution kinetics of carbonates in dilute hydrochloric acid and sulfuric acid solutions containing metal ions (Fe
3+
/Ca
2+
/Mn
2+
) at ambient temperature and pressure (T = 25 °C, P = 1 atm) were studied, by laboratory dissolution experiments combined with numerical simulations using PHREEQC. The results show that the Fe
3+
is of great significance on the dissolution of carbonate rocks, while the influences of Ca
2+
and Mn
2+
are relatively weak. The dissolutions degrees of micritic limestone (ZG-L25), dolomitic limestone (ZG-L7) and dolomite (ZG-D9) were better than the other carbonates under the influence of metal ions (Fe
3+
/Ca
2+
/Mn
2+
) in acid solutions. Therefore, the dolomite reservoir of the Cambrian Qinjiamiao Formation, the dolomitic limestone reservoir of the Tianheban Formation and the limestone reservoir of the Triassic Daye Formation in the Zigui area are potential high-quality reservoirs. The carbonate reservoirs associated with Fe-bearing minerals were easier to dissolve and formed secondary pores under shallow burial. This process is beneficial to the formation of high-quality reservoirs. Moreover, the addition of Fe
3+
into hydrochloric acid solution may be conducive to improving the reservoirs acidizing effect. Furthermore, the results gave innovative results from multiple perspectives of geo-material science and computational geosciences, which may provide new avenues for in-depth study of carbonate dissolution in shallow burial based on water–rock reaction, chemical dissolution, computational simulation, and geological background.</description><identifier>ISSN: 1520-7439</identifier><identifier>EISSN: 1573-8981</identifier><identifier>DOI: 10.1007/s11053-020-09765-6</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Ambient temperature ; Calcium ; Calcium ions ; Cambrian ; Carbonate rocks ; Carbonates ; Chemistry and Earth Sciences ; Computer applications ; Computer Science ; Dissolution ; Dolomite ; Dolomitic limestone ; Earth and Environmental Science ; Earth Sciences ; Ferric ions ; Fossil Fuels (incl. Carbon Capture) ; Geography ; Hydrochloric acid ; Iron ; Limestone ; Low pressure ; Low temperature ; Manganese ions ; Mathematical Modeling and Industrial Mathematics ; Metal ions ; Mineral Resources ; Minerals ; Original Paper ; Physics ; Pores ; Pyrite ; Reservoirs ; Statistics for Engineering ; Sulfuric acid ; Sustainable Development ; Triassic ; Water depth</subject><ispartof>Natural resources research (New York, N.Y.), 2021-04, Vol.30 (2), p.1291-1303</ispartof><rights>International Association for Mathematical Geosciences 2020</rights><rights>International Association for Mathematical Geosciences 2020.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c1646-ba84c72dc5b22ebc544ba24ba537f77628b69bdef8f1cf987bcb120d8656f5d13</citedby><cites>FETCH-LOGICAL-c1646-ba84c72dc5b22ebc544ba24ba537f77628b69bdef8f1cf987bcb120d8656f5d13</cites><orcidid>0000-0002-7443-6486</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11053-020-09765-6$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2918337012?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>314,776,780,21368,27903,27904,33723,41467,42536,43784,51298,64362,64366,72216</link.rule.ids></links><search><creatorcontrib>Ma, Jiayi</creatorcontrib><creatorcontrib>Xie, Shuyun</creatorcontrib><creatorcontrib>Liu, Dan</creatorcontrib><creatorcontrib>Carranza, Emmanuel John M.</creatorcontrib><creatorcontrib>He, Zhiliang</creatorcontrib><creatorcontrib>Zhang, Mohai</creatorcontrib><creatorcontrib>Wang, Tianyi</creatorcontrib><title>Effects of Fe3+ on Dissolution Dynamics of Carbonate Rocks in a Shallow Burial Reservoir</title><title>Natural resources research (New York, N.Y.)</title><addtitle>Nat Resour Res</addtitle><description>Dissolution of carbonates in acidic fluids, which has attracted much research attention in recent years, is of great significance for the formation of high-quality reservoirs. The dissolution stage under low temperature and low pressure in shallow burial is one of the most important processes of reservoir dissolution and transformation. However, the dissolution dynamics of carbonate rocks in shallow burial and their formation have been controversial for a long time, and there are still disputes in the dissolution processes about how associated minerals and accessory minerals (e.g., pyrite) in carbonate reservoirs influence the formation of secondary pores. Additional metal ions in acidic fluids can change fluid properties and dissolution processes, and consequently affect reservoir quality. However, there are few laboratory studies done on the effect of associated minerals on the dissolution dynamics of carbonates. To clarify the specific impact of Fe-bearing associated minerals and Fe
3+
on the dissolution of carbonates in shallow burial reservoirs, six samples of typical carbonate rocks in the Zigui area of Hubei Province, China were studied. The dissolution kinetics of carbonates in dilute hydrochloric acid and sulfuric acid solutions containing metal ions (Fe
3+
/Ca
2+
/Mn
2+
) at ambient temperature and pressure (T = 25 °C, P = 1 atm) were studied, by laboratory dissolution experiments combined with numerical simulations using PHREEQC. The results show that the Fe
3+
is of great significance on the dissolution of carbonate rocks, while the influences of Ca
2+
and Mn
2+
are relatively weak. The dissolutions degrees of micritic limestone (ZG-L25), dolomitic limestone (ZG-L7) and dolomite (ZG-D9) were better than the other carbonates under the influence of metal ions (Fe
3+
/Ca
2+
/Mn
2+
) in acid solutions. Therefore, the dolomite reservoir of the Cambrian Qinjiamiao Formation, the dolomitic limestone reservoir of the Tianheban Formation and the limestone reservoir of the Triassic Daye Formation in the Zigui area are potential high-quality reservoirs. The carbonate reservoirs associated with Fe-bearing minerals were easier to dissolve and formed secondary pores under shallow burial. This process is beneficial to the formation of high-quality reservoirs. Moreover, the addition of Fe
3+
into hydrochloric acid solution may be conducive to improving the reservoirs acidizing effect. Furthermore, the results gave innovative results from multiple perspectives of geo-material science and computational geosciences, which may provide new avenues for in-depth study of carbonate dissolution in shallow burial based on water–rock reaction, chemical dissolution, computational simulation, and geological background.</description><subject>Ambient temperature</subject><subject>Calcium</subject><subject>Calcium ions</subject><subject>Cambrian</subject><subject>Carbonate rocks</subject><subject>Carbonates</subject><subject>Chemistry and Earth Sciences</subject><subject>Computer applications</subject><subject>Computer Science</subject><subject>Dissolution</subject><subject>Dolomite</subject><subject>Dolomitic limestone</subject><subject>Earth and Environmental Science</subject><subject>Earth Sciences</subject><subject>Ferric ions</subject><subject>Fossil Fuels (incl. Carbon Capture)</subject><subject>Geography</subject><subject>Hydrochloric acid</subject><subject>Iron</subject><subject>Limestone</subject><subject>Low pressure</subject><subject>Low temperature</subject><subject>Manganese ions</subject><subject>Mathematical Modeling and Industrial Mathematics</subject><subject>Metal ions</subject><subject>Mineral Resources</subject><subject>Minerals</subject><subject>Original Paper</subject><subject>Physics</subject><subject>Pores</subject><subject>Pyrite</subject><subject>Reservoirs</subject><subject>Statistics for Engineering</subject><subject>Sulfuric acid</subject><subject>Sustainable Development</subject><subject>Triassic</subject><subject>Water depth</subject><issn>1520-7439</issn><issn>1573-8981</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9kMtKAzEUhoMoWKsv4CrgUkZzmVxmqbVVoSBUBXchySQ6dTrRZEbp25u2gjsXh3Pgvxz4ADjF6AIjJC4TxojRAhFUoEpwVvA9MMJM0EJWEu9v7iyJklaH4CilJcohKtkIvEy9d7ZPMHg4c_Qchg7eNCmFduibzb3u9KqxW32iowmd7h1cBPueYNNBDR_fdNuGb3g9xEa3cOGSi1-hicfgwOs2uZPfPQbPs-nT5K6YP9zeT67mhcW85IXRsrSC1JYZQpyxrCyNJnkYFV4ITqThlamdlx5bX0lhrMEE1ZIz7lmN6Ric7Xo_YvgcXOrVMgyxyy8VqbCkVCBMsovsXDaGlKLz6iM2Kx3XCiO1Iah2BFUmqLYEFc8hugulbO5eXfyr_if1Awv-cw4</recordid><startdate>20210401</startdate><enddate>20210401</enddate><creator>Ma, Jiayi</creator><creator>Xie, Shuyun</creator><creator>Liu, Dan</creator><creator>Carranza, Emmanuel John M.</creator><creator>He, Zhiliang</creator><creator>Zhang, Mohai</creator><creator>Wang, Tianyi</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>BHPHI</scope><scope>BKSAR</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PATMY</scope><scope>PCBAR</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><orcidid>https://orcid.org/0000-0002-7443-6486</orcidid></search><sort><creationdate>20210401</creationdate><title>Effects of Fe3+ on Dissolution Dynamics of Carbonate Rocks in a Shallow Burial Reservoir</title><author>Ma, Jiayi ; Xie, Shuyun ; Liu, Dan ; Carranza, Emmanuel John M. ; He, Zhiliang ; Zhang, Mohai ; Wang, Tianyi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c1646-ba84c72dc5b22ebc544ba24ba537f77628b69bdef8f1cf987bcb120d8656f5d13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Ambient temperature</topic><topic>Calcium</topic><topic>Calcium ions</topic><topic>Cambrian</topic><topic>Carbonate rocks</topic><topic>Carbonates</topic><topic>Chemistry and Earth Sciences</topic><topic>Computer applications</topic><topic>Computer Science</topic><topic>Dissolution</topic><topic>Dolomite</topic><topic>Dolomitic limestone</topic><topic>Earth and Environmental Science</topic><topic>Earth Sciences</topic><topic>Ferric ions</topic><topic>Fossil Fuels (incl. Carbon Capture)</topic><topic>Geography</topic><topic>Hydrochloric acid</topic><topic>Iron</topic><topic>Limestone</topic><topic>Low pressure</topic><topic>Low temperature</topic><topic>Manganese ions</topic><topic>Mathematical Modeling and Industrial Mathematics</topic><topic>Metal ions</topic><topic>Mineral Resources</topic><topic>Minerals</topic><topic>Original Paper</topic><topic>Physics</topic><topic>Pores</topic><topic>Pyrite</topic><topic>Reservoirs</topic><topic>Statistics for Engineering</topic><topic>Sulfuric acid</topic><topic>Sustainable Development</topic><topic>Triassic</topic><topic>Water depth</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ma, Jiayi</creatorcontrib><creatorcontrib>Xie, Shuyun</creatorcontrib><creatorcontrib>Liu, Dan</creatorcontrib><creatorcontrib>Carranza, Emmanuel John M.</creatorcontrib><creatorcontrib>He, Zhiliang</creatorcontrib><creatorcontrib>Zhang, Mohai</creatorcontrib><creatorcontrib>Wang, Tianyi</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central UK/Ireland</collection><collection>Agricultural & Environmental Science Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>Natural Science Collection</collection><collection>Earth, Atmospheric & Aquatic Science Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Environmental Science Database</collection><collection>Earth, Atmospheric & Aquatic Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Environmental Science Collection</collection><jtitle>Natural resources research (New York, N.Y.)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ma, Jiayi</au><au>Xie, Shuyun</au><au>Liu, Dan</au><au>Carranza, Emmanuel John M.</au><au>He, Zhiliang</au><au>Zhang, Mohai</au><au>Wang, Tianyi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effects of Fe3+ on Dissolution Dynamics of Carbonate Rocks in a Shallow Burial Reservoir</atitle><jtitle>Natural resources research (New York, N.Y.)</jtitle><stitle>Nat Resour Res</stitle><date>2021-04-01</date><risdate>2021</risdate><volume>30</volume><issue>2</issue><spage>1291</spage><epage>1303</epage><pages>1291-1303</pages><issn>1520-7439</issn><eissn>1573-8981</eissn><abstract>Dissolution of carbonates in acidic fluids, which has attracted much research attention in recent years, is of great significance for the formation of high-quality reservoirs. The dissolution stage under low temperature and low pressure in shallow burial is one of the most important processes of reservoir dissolution and transformation. However, the dissolution dynamics of carbonate rocks in shallow burial and their formation have been controversial for a long time, and there are still disputes in the dissolution processes about how associated minerals and accessory minerals (e.g., pyrite) in carbonate reservoirs influence the formation of secondary pores. Additional metal ions in acidic fluids can change fluid properties and dissolution processes, and consequently affect reservoir quality. However, there are few laboratory studies done on the effect of associated minerals on the dissolution dynamics of carbonates. To clarify the specific impact of Fe-bearing associated minerals and Fe
3+
on the dissolution of carbonates in shallow burial reservoirs, six samples of typical carbonate rocks in the Zigui area of Hubei Province, China were studied. The dissolution kinetics of carbonates in dilute hydrochloric acid and sulfuric acid solutions containing metal ions (Fe
3+
/Ca
2+
/Mn
2+
) at ambient temperature and pressure (T = 25 °C, P = 1 atm) were studied, by laboratory dissolution experiments combined with numerical simulations using PHREEQC. The results show that the Fe
3+
is of great significance on the dissolution of carbonate rocks, while the influences of Ca
2+
and Mn
2+
are relatively weak. The dissolutions degrees of micritic limestone (ZG-L25), dolomitic limestone (ZG-L7) and dolomite (ZG-D9) were better than the other carbonates under the influence of metal ions (Fe
3+
/Ca
2+
/Mn
2+
) in acid solutions. Therefore, the dolomite reservoir of the Cambrian Qinjiamiao Formation, the dolomitic limestone reservoir of the Tianheban Formation and the limestone reservoir of the Triassic Daye Formation in the Zigui area are potential high-quality reservoirs. The carbonate reservoirs associated with Fe-bearing minerals were easier to dissolve and formed secondary pores under shallow burial. This process is beneficial to the formation of high-quality reservoirs. Moreover, the addition of Fe
3+
into hydrochloric acid solution may be conducive to improving the reservoirs acidizing effect. Furthermore, the results gave innovative results from multiple perspectives of geo-material science and computational geosciences, which may provide new avenues for in-depth study of carbonate dissolution in shallow burial based on water–rock reaction, chemical dissolution, computational simulation, and geological background.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s11053-020-09765-6</doi><tpages>13</tpages><orcidid>https://orcid.org/0000-0002-7443-6486</orcidid></addata></record> |
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| subjects | Ambient temperature Calcium Calcium ions Cambrian Carbonate rocks Carbonates Chemistry and Earth Sciences Computer applications Computer Science Dissolution Dolomite Dolomitic limestone Earth and Environmental Science Earth Sciences Ferric ions Fossil Fuels (incl. Carbon Capture) Geography Hydrochloric acid Iron Limestone Low pressure Low temperature Manganese ions Mathematical Modeling and Industrial Mathematics Metal ions Mineral Resources Minerals Original Paper Physics Pores Pyrite Reservoirs Statistics for Engineering Sulfuric acid Sustainable Development Triassic Water depth |
| title | Effects of Fe3+ on Dissolution Dynamics of Carbonate Rocks in a Shallow Burial Reservoir |
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