Highest degradation of aromatic dyes by new MgO@PANI-o-PDA core–shell nanocomposites
Because of tremendous demand of different, innovative and convenient synthetic techniques, the present research establishes a remarkable synthetic protocol for new core–shell nanocomposites (CSNCs) containing magnesium oxide. MgO@poly(aniline-co-o-phenylenediamine) (MgO@PANI-o-PDA) CSNCs were genera...
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| Veröffentlicht in: | Polymer bulletin (Berlin, Germany) Germany), 2022-06, Vol.79 (6), p.3741-3758 |
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| container_title | Polymer bulletin (Berlin, Germany) |
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| creator | Al-Hussaini, Ayman S. Mohamedein, Abdullah M. Hassan, Mohamed E. R. |
| description | Because of tremendous demand of different, innovative and convenient synthetic techniques, the present research establishes a remarkable synthetic protocol for new core–shell nanocomposites (CSNCs) containing magnesium oxide. MgO@poly(aniline-co-o-phenylenediamine) (MgO@PANI-o-PDA) CSNCs were generated employing equimolar ratios of the applicable moieties and several MgO weights through polycondensation. The CSNCs structures were confirmed by varied characterizations. The linkage between MgO and PANI-o-PDA was detected through FTIR bands. The CSNCs characters have core–shell structures as well as small size 41–66 nm. Under irradiation, the CSNCs afford the highest photocatalysis efficacy toward MB dye degradation. Realistic explanations of the photocatalytic efficiency results of CSNCs toward MB were substantiated. From DLS results, the CSNC system is either one of the good or the best systems having narrow PDI and incipient instability. This pathway is an original, simplistic, economical and advantageous procedure to develop potential CSNCs in the objective of pioneering constructions.
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| doi_str_mv | 10.1007/s00289-021-03682-1 |
| format | Article |
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Graphic abstract</description><subject>Aniline</subject><subject>Banded structure</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Chloride</subject><subject>Complex Fluids and Microfluidics</subject><subject>Core-shell structure</subject><subject>Degradation</subject><subject>Dyes</subject><subject>Magnesium</subject><subject>Magnesium oxide</subject><subject>Metal oxides</subject><subject>Nanocomposites</subject><subject>Nanoparticles</subject><subject>Organic Chemistry</subject><subject>Original Paper</subject><subject>Phenylenediamine</subject><subject>Photocatalysis</subject><subject>Physical Chemistry</subject><subject>Pollutants</subject><subject>Polyanilines</subject><subject>Polymer Sciences</subject><subject>Polymerization</subject><subject>Soft and Granular Matter</subject><subject>Superconductors (materials)</subject><issn>0170-0839</issn><issn>1436-2449</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kMtKAzEUhoMoWKsv4CrgOnpyaTLZWby1UG0X6jZkJpnplHZSkxbpznfwDX0Sp47gztXhwPf_h_MhdE7hkgKoqwTAMk2AUQJcZozQA9SjgkvChNCHqAdUAYGM62N0ktIC2l1K2kOvo7qa-7TBzlfROrupQ4NDiW0Mq3YpsNv5hPMdbvw7fqym17Ph05gEMrsd4iJE__XxmeZ-ucSNbUIRVuuQ6o1Pp-iotMvkz35nH73c3z3fjMhk-jC-GU5IwaneEGUtG4hcOc3y3DmQA66UdaALx0VuMzeQslRANS9UzrxW0KJCSAkgCmkp76OLrncdw9u2_cMswjY27UnDNFVaUcZES7GOKmJIKfrSrGO9snFnKJi9P9P5M60_8-PP7Kt5F0ot3FQ-_lX_k_oG2hxyqw</recordid><startdate>20220601</startdate><enddate>20220601</enddate><creator>Al-Hussaini, Ayman S.</creator><creator>Mohamedein, Abdullah M.</creator><creator>Hassan, Mohamed E. R.</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><orcidid>https://orcid.org/0000-0002-6212-3706</orcidid></search><sort><creationdate>20220601</creationdate><title>Highest degradation of aromatic dyes by new MgO@PANI-o-PDA core–shell nanocomposites</title><author>Al-Hussaini, Ayman S. ; Mohamedein, Abdullah M. ; Hassan, Mohamed E. R.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-7aa254b7d92bbdd065377ad09cd34ba8d566f70193c7b2e9707d94466004c6a13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Aniline</topic><topic>Banded structure</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Chloride</topic><topic>Complex Fluids and Microfluidics</topic><topic>Core-shell structure</topic><topic>Degradation</topic><topic>Dyes</topic><topic>Magnesium</topic><topic>Magnesium oxide</topic><topic>Metal oxides</topic><topic>Nanocomposites</topic><topic>Nanoparticles</topic><topic>Organic Chemistry</topic><topic>Original Paper</topic><topic>Phenylenediamine</topic><topic>Photocatalysis</topic><topic>Physical Chemistry</topic><topic>Pollutants</topic><topic>Polyanilines</topic><topic>Polymer Sciences</topic><topic>Polymerization</topic><topic>Soft and Granular Matter</topic><topic>Superconductors (materials)</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Al-Hussaini, Ayman S.</creatorcontrib><creatorcontrib>Mohamedein, Abdullah M.</creatorcontrib><creatorcontrib>Hassan, Mohamed E. 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R.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Highest degradation of aromatic dyes by new MgO@PANI-o-PDA core–shell nanocomposites</atitle><jtitle>Polymer bulletin (Berlin, Germany)</jtitle><stitle>Polym. Bull</stitle><date>2022-06-01</date><risdate>2022</risdate><volume>79</volume><issue>6</issue><spage>3741</spage><epage>3758</epage><pages>3741-3758</pages><issn>0170-0839</issn><eissn>1436-2449</eissn><abstract>Because of tremendous demand of different, innovative and convenient synthetic techniques, the present research establishes a remarkable synthetic protocol for new core–shell nanocomposites (CSNCs) containing magnesium oxide. MgO@poly(aniline-co-o-phenylenediamine) (MgO@PANI-o-PDA) CSNCs were generated employing equimolar ratios of the applicable moieties and several MgO weights through polycondensation. The CSNCs structures were confirmed by varied characterizations. The linkage between MgO and PANI-o-PDA was detected through FTIR bands. The CSNCs characters have core–shell structures as well as small size 41–66 nm. Under irradiation, the CSNCs afford the highest photocatalysis efficacy toward MB dye degradation. Realistic explanations of the photocatalytic efficiency results of CSNCs toward MB were substantiated. From DLS results, the CSNC system is either one of the good or the best systems having narrow PDI and incipient instability. This pathway is an original, simplistic, economical and advantageous procedure to develop potential CSNCs in the objective of pioneering constructions.
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| subjects | Aniline Banded structure Characterization and Evaluation of Materials Chemistry Chemistry and Materials Science Chloride Complex Fluids and Microfluidics Core-shell structure Degradation Dyes Magnesium Magnesium oxide Metal oxides Nanocomposites Nanoparticles Organic Chemistry Original Paper Phenylenediamine Photocatalysis Physical Chemistry Pollutants Polyanilines Polymer Sciences Polymerization Soft and Granular Matter Superconductors (materials) |
| title | Highest degradation of aromatic dyes by new MgO@PANI-o-PDA core–shell nanocomposites |
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