Synthesis and characterization of multi-responsive poly(N-isopropylacrylamide)-sodium alginate-graphene oxide composite hydrogels
The multi-responsive ternary poly(N-isopropyl acrylamide) (PNIPAM)/ /sodium alginate (SA)/graphene oxide (GO) composite hydrogels were prepared. The influence of GO content on the microstructure and physical properties of the composite hydrogel was researched. The ternary composite hydrogels exhibit...
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| Veröffentlicht in: | Polymer bulletin (Berlin, Germany) Germany), 2023-10, Vol.80 (10), p.10825-10842 |
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| creator | Zhang, Yiqiang Yang, Fuguo Huang, Huabo Zhao, Rui Huang, Juan Li, Liang Yu, Xianghua |
| description | The multi-responsive ternary poly(N-isopropyl acrylamide) (PNIPAM)/ /sodium alginate (SA)/graphene oxide (GO) composite hydrogels were prepared. The influence of GO content on the microstructure and physical properties of the composite hydrogel was researched. The ternary composite hydrogels exhibited significantly larger mechanical strength and higher water uptake compared to binary PNIPAM/SA composite hydrogels. The effects of temperature, pH, and contact time on the adsorption capacity of rhodamine B (RB) for the PNIPAM/SA/GO ternary composite hydrogels were further investigated. The adsorption kinetic and isotherm for the adsorption behavior of the ternary composite hydrogel were well fitted with the pseudo-second-order kinetic model and Langmuir model, respectively. Besides, the PNIPAM/SA/GO ternary composite hydrogel could be easily removed from the dye solutions and reused without the obvious decrease of its performance. It indicated that the ternary composite hydrogel could serve as an effective adsorbent for the removal of organic pollutants. |
| doi_str_mv | 10.1007/s00289-022-04581-9 |
| format | Article |
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The influence of GO content on the microstructure and physical properties of the composite hydrogel was researched. The ternary composite hydrogels exhibited significantly larger mechanical strength and higher water uptake compared to binary PNIPAM/SA composite hydrogels. The effects of temperature, pH, and contact time on the adsorption capacity of rhodamine B (RB) for the PNIPAM/SA/GO ternary composite hydrogels were further investigated. The adsorption kinetic and isotherm for the adsorption behavior of the ternary composite hydrogel were well fitted with the pseudo-second-order kinetic model and Langmuir model, respectively. Besides, the PNIPAM/SA/GO ternary composite hydrogel could be easily removed from the dye solutions and reused without the obvious decrease of its performance. It indicated that the ternary composite hydrogel could serve as an effective adsorbent for the removal of organic pollutants.</description><identifier>ISSN: 0170-0839</identifier><identifier>EISSN: 1436-2449</identifier><identifier>DOI: 10.1007/s00289-022-04581-9</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Acrylamide ; Adsorption ; Aqueous solutions ; Characterization and Evaluation of Materials ; Chemistry ; Chemistry and Materials Science ; Complex Fluids and Microfluidics ; Fourier transforms ; Free radicals ; Graphene ; Hydrogels ; Organic Chemistry ; Original Paper ; Phase transitions ; Physical Chemistry ; Physical properties ; Polyisopropyl acrylamide ; Polymer Sciences ; Polymerization ; Polymers ; Radiation ; Rhodamine ; Scanning electron microscopy ; Sodium alginate ; Soft and Granular Matter ; Spectrum analysis ; Temperature effects ; Water pollution</subject><ispartof>Polymer bulletin (Berlin, Germany), 2023-10, Vol.80 (10), p.10825-10842</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-595cd74d3a556adbc875d7d7c5b64ff1080f46d682e6ea9af8811dc188e4c0ef3</citedby><cites>FETCH-LOGICAL-c319t-595cd74d3a556adbc875d7d7c5b64ff1080f46d682e6ea9af8811dc188e4c0ef3</cites><orcidid>0000-0003-4601-8890</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s00289-022-04581-9$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2917958695?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>314,776,780,21367,27901,27902,33721,41464,42533,43781,51294</link.rule.ids></links><search><creatorcontrib>Zhang, Yiqiang</creatorcontrib><creatorcontrib>Yang, Fuguo</creatorcontrib><creatorcontrib>Huang, Huabo</creatorcontrib><creatorcontrib>Zhao, Rui</creatorcontrib><creatorcontrib>Huang, Juan</creatorcontrib><creatorcontrib>Li, Liang</creatorcontrib><creatorcontrib>Yu, Xianghua</creatorcontrib><title>Synthesis and characterization of multi-responsive poly(N-isopropylacrylamide)-sodium alginate-graphene oxide composite hydrogels</title><title>Polymer bulletin (Berlin, Germany)</title><addtitle>Polym. Bull</addtitle><description>The multi-responsive ternary poly(N-isopropyl acrylamide) (PNIPAM)/ /sodium alginate (SA)/graphene oxide (GO) composite hydrogels were prepared. The influence of GO content on the microstructure and physical properties of the composite hydrogel was researched. The ternary composite hydrogels exhibited significantly larger mechanical strength and higher water uptake compared to binary PNIPAM/SA composite hydrogels. The effects of temperature, pH, and contact time on the adsorption capacity of rhodamine B (RB) for the PNIPAM/SA/GO ternary composite hydrogels were further investigated. The adsorption kinetic and isotherm for the adsorption behavior of the ternary composite hydrogel were well fitted with the pseudo-second-order kinetic model and Langmuir model, respectively. Besides, the PNIPAM/SA/GO ternary composite hydrogel could be easily removed from the dye solutions and reused without the obvious decrease of its performance. It indicated that the ternary composite hydrogel could serve as an effective adsorbent for the removal of organic pollutants.</description><subject>Acrylamide</subject><subject>Adsorption</subject><subject>Aqueous solutions</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Complex Fluids and Microfluidics</subject><subject>Fourier transforms</subject><subject>Free radicals</subject><subject>Graphene</subject><subject>Hydrogels</subject><subject>Organic Chemistry</subject><subject>Original Paper</subject><subject>Phase transitions</subject><subject>Physical Chemistry</subject><subject>Physical properties</subject><subject>Polyisopropyl acrylamide</subject><subject>Polymer Sciences</subject><subject>Polymerization</subject><subject>Polymers</subject><subject>Radiation</subject><subject>Rhodamine</subject><subject>Scanning electron microscopy</subject><subject>Sodium alginate</subject><subject>Soft and Granular Matter</subject><subject>Spectrum analysis</subject><subject>Temperature effects</subject><subject>Water pollution</subject><issn>0170-0839</issn><issn>1436-2449</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp9kE9LxDAQxYMouK5-AU8BL3qIJm2TJkcR_8GiB_UcYjLdjbRNTbpivfnNja7gzcsMw7z3ZvghdMjoKaO0PkuUFlIRWhSEVlwyorbQjFWlIEVVqW00o6ymhMpS7aK9lF5onoVgM_T5MPXjCpJP2PQO25WJxo4Q_YcZfehxaHC3bkdPIqQh9Mm_AR5COx3fEZ_CEMMwtcbGXDrv4ISk4Py6w6Zd-t6MQJbRDCvoAYf3vMc2dENIfgS8mlwMS2jTPtppTJvg4LfP0dPV5ePFDVncX99enC-ILZkaCVfcurpypeFcGPdsZc1d7WrLn0XVNIxK2lTCCVmAAKNMIyVjzjIpobIUmnKOjja5-enXNaRRv4R17PNJXShWKy6F4llVbFQ2hpQiNHqIvjNx0ozqb9R6g1pn1PoHtVbZVG5MKYv7JcS_6H9cX7aQhgM</recordid><startdate>20231001</startdate><enddate>20231001</enddate><creator>Zhang, Yiqiang</creator><creator>Yang, Fuguo</creator><creator>Huang, Huabo</creator><creator>Zhao, Rui</creator><creator>Huang, Juan</creator><creator>Li, Liang</creator><creator>Yu, Xianghua</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PHGZM</scope><scope>PHGZT</scope><scope>PKEHL</scope><scope>PQEST</scope><scope>PQGLB</scope><scope>PQQKQ</scope><scope>PQUKI</scope><orcidid>https://orcid.org/0000-0003-4601-8890</orcidid></search><sort><creationdate>20231001</creationdate><title>Synthesis and characterization of multi-responsive poly(N-isopropylacrylamide)-sodium alginate-graphene oxide composite hydrogels</title><author>Zhang, Yiqiang ; Yang, Fuguo ; Huang, Huabo ; Zhao, Rui ; Huang, Juan ; Li, Liang ; Yu, Xianghua</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-595cd74d3a556adbc875d7d7c5b64ff1080f46d682e6ea9af8811dc188e4c0ef3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Acrylamide</topic><topic>Adsorption</topic><topic>Aqueous solutions</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Complex Fluids and Microfluidics</topic><topic>Fourier transforms</topic><topic>Free radicals</topic><topic>Graphene</topic><topic>Hydrogels</topic><topic>Organic Chemistry</topic><topic>Original Paper</topic><topic>Phase transitions</topic><topic>Physical Chemistry</topic><topic>Physical properties</topic><topic>Polyisopropyl acrylamide</topic><topic>Polymer Sciences</topic><topic>Polymerization</topic><topic>Polymers</topic><topic>Radiation</topic><topic>Rhodamine</topic><topic>Scanning electron microscopy</topic><topic>Sodium alginate</topic><topic>Soft and Granular Matter</topic><topic>Spectrum analysis</topic><topic>Temperature effects</topic><topic>Water pollution</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Yiqiang</creatorcontrib><creatorcontrib>Yang, Fuguo</creatorcontrib><creatorcontrib>Huang, Huabo</creatorcontrib><creatorcontrib>Zhao, Rui</creatorcontrib><creatorcontrib>Huang, Juan</creatorcontrib><creatorcontrib>Li, Liang</creatorcontrib><creatorcontrib>Yu, Xianghua</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest Central (New)</collection><collection>ProQuest One Academic (New)</collection><collection>ProQuest One Academic Middle East (New)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Applied & Life Sciences</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><jtitle>Polymer bulletin (Berlin, Germany)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, Yiqiang</au><au>Yang, Fuguo</au><au>Huang, Huabo</au><au>Zhao, Rui</au><au>Huang, Juan</au><au>Li, Liang</au><au>Yu, Xianghua</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Synthesis and characterization of multi-responsive poly(N-isopropylacrylamide)-sodium alginate-graphene oxide composite hydrogels</atitle><jtitle>Polymer bulletin (Berlin, Germany)</jtitle><stitle>Polym. Bull</stitle><date>2023-10-01</date><risdate>2023</risdate><volume>80</volume><issue>10</issue><spage>10825</spage><epage>10842</epage><pages>10825-10842</pages><issn>0170-0839</issn><eissn>1436-2449</eissn><abstract>The multi-responsive ternary poly(N-isopropyl acrylamide) (PNIPAM)/ /sodium alginate (SA)/graphene oxide (GO) composite hydrogels were prepared. The influence of GO content on the microstructure and physical properties of the composite hydrogel was researched. The ternary composite hydrogels exhibited significantly larger mechanical strength and higher water uptake compared to binary PNIPAM/SA composite hydrogels. The effects of temperature, pH, and contact time on the adsorption capacity of rhodamine B (RB) for the PNIPAM/SA/GO ternary composite hydrogels were further investigated. The adsorption kinetic and isotherm for the adsorption behavior of the ternary composite hydrogel were well fitted with the pseudo-second-order kinetic model and Langmuir model, respectively. Besides, the PNIPAM/SA/GO ternary composite hydrogel could be easily removed from the dye solutions and reused without the obvious decrease of its performance. It indicated that the ternary composite hydrogel could serve as an effective adsorbent for the removal of organic pollutants.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s00289-022-04581-9</doi><tpages>18</tpages><orcidid>https://orcid.org/0000-0003-4601-8890</orcidid></addata></record> |
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| subjects | Acrylamide Adsorption Aqueous solutions Characterization and Evaluation of Materials Chemistry Chemistry and Materials Science Complex Fluids and Microfluidics Fourier transforms Free radicals Graphene Hydrogels Organic Chemistry Original Paper Phase transitions Physical Chemistry Physical properties Polyisopropyl acrylamide Polymer Sciences Polymerization Polymers Radiation Rhodamine Scanning electron microscopy Sodium alginate Soft and Granular Matter Spectrum analysis Temperature effects Water pollution |
| title | Synthesis and characterization of multi-responsive poly(N-isopropylacrylamide)-sodium alginate-graphene oxide composite hydrogels |
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