Influence of wheat stalk nanocellulose on structural, mechanical, thermal, surface and degradation properties of composites with poly(butylene adipate-co-terephthalate)
Structural, mechanical, thermal and surface properties comprising biodegradable aromatic–aliphatic polymer poly(butylene adipate- co -terephthalate) (PBAT) and the wheat stalk-based nanocellulose (NCC) were studied. The materials were found to comprise the compatible and yet phase-segregated constit...
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| Veröffentlicht in: | Polymer bulletin (Berlin, Germany) Germany), 2023-07, Vol.80 (7), p.7599-7625 |
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| creator | Giri, Jyoti Lach, Ralf Henning, Sven Grellmann, Wolfgang Bhasney, Siddharth Mohan Katiyar, Vimal Saiter, Jean-Marc Adhikari, Rameshwar |
| description | Structural, mechanical, thermal and surface properties comprising biodegradable aromatic–aliphatic polymer poly(butylene adipate-
co
-terephthalate) (PBAT) and the wheat stalk-based nanocellulose (NCC) were studied. The materials were found to comprise the compatible and yet phase-segregated constituents which kept their identity in the nanocomposite materials. The NCC phase was found to be homogeneously dispersed in the PBAT matrix inside. Similar to the corresponding microcomposites, the investigated nanocomposites were found to be stable within their desired application temperature as packaging materials. The tensile properties of the nanocomposites degraded in terms of strain at break, tensile strength and tensile modulus. At higher filler content, the reinforcing effect dominated leading to an increase in indentation modulus and hardness, and a decrease in the work of elastic deformation. The wettability and the water absorption capacity of the materials increased with NCC content thereby enhancing the biodegradability of the composites. |
| doi_str_mv | 10.1007/s00289-022-04388-8 |
| format | Article |
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co
-terephthalate) (PBAT) and the wheat stalk-based nanocellulose (NCC) were studied. The materials were found to comprise the compatible and yet phase-segregated constituents which kept their identity in the nanocomposite materials. The NCC phase was found to be homogeneously dispersed in the PBAT matrix inside. Similar to the corresponding microcomposites, the investigated nanocomposites were found to be stable within their desired application temperature as packaging materials. The tensile properties of the nanocomposites degraded in terms of strain at break, tensile strength and tensile modulus. At higher filler content, the reinforcing effect dominated leading to an increase in indentation modulus and hardness, and a decrease in the work of elastic deformation. The wettability and the water absorption capacity of the materials increased with NCC content thereby enhancing the biodegradability of the composites.</description><identifier>ISSN: 0170-0839</identifier><identifier>EISSN: 1436-2449</identifier><identifier>DOI: 10.1007/s00289-022-04388-8</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Cellulose ; Characterization and Evaluation of Materials ; Chemistry ; Chemistry and Materials Science ; Complex Fluids and Microfluidics ; Contact angle ; Elastic deformation ; Fourier transforms ; Load ; Modulus of elasticity ; Molecular weight ; Nanocomposites ; Organic Chemistry ; Original Paper ; Physical Chemistry ; Polyethylene terephthalate ; Polymer Sciences ; Polymers ; Polyvinyl alcohol ; Raw materials ; Soft and Granular Matter ; Spectrum analysis ; Surface properties ; Tensile properties ; Tensile strength ; Terephthalate ; Thermogravimetric analysis ; Water absorption ; Wettability ; Wheat</subject><ispartof>Polymer bulletin (Berlin, Germany), 2023-07, Vol.80 (7), p.7599-7625</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022. Springer Nature or its licensor holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-26bfa79059c09fb4529f2166654851d80db367c3a1d8823356db19ebeb97a1983</citedby><cites>FETCH-LOGICAL-c319t-26bfa79059c09fb4529f2166654851d80db367c3a1d8823356db19ebeb97a1983</cites><orcidid>0000-0003-0489-0154 ; 0000-0002-2231-3839 ; 0000-0002-7350-0204 ; 0000-0003-4750-7653 ; 0000-0003-0590-1468 ; 0000-0002-5936-4410 ; 0000-0003-2896-9318 ; 0000-0002-3724-3562</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s00289-022-04388-8$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2917939187?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>315,781,785,21392,27928,27929,33748,41492,42561,43809,51323,64389,64393,72473</link.rule.ids></links><search><creatorcontrib>Giri, Jyoti</creatorcontrib><creatorcontrib>Lach, Ralf</creatorcontrib><creatorcontrib>Henning, Sven</creatorcontrib><creatorcontrib>Grellmann, Wolfgang</creatorcontrib><creatorcontrib>Bhasney, Siddharth Mohan</creatorcontrib><creatorcontrib>Katiyar, Vimal</creatorcontrib><creatorcontrib>Saiter, Jean-Marc</creatorcontrib><creatorcontrib>Adhikari, Rameshwar</creatorcontrib><title>Influence of wheat stalk nanocellulose on structural, mechanical, thermal, surface and degradation properties of composites with poly(butylene adipate-co-terephthalate)</title><title>Polymer bulletin (Berlin, Germany)</title><addtitle>Polym. Bull</addtitle><description>Structural, mechanical, thermal and surface properties comprising biodegradable aromatic–aliphatic polymer poly(butylene adipate-
co
-terephthalate) (PBAT) and the wheat stalk-based nanocellulose (NCC) were studied. The materials were found to comprise the compatible and yet phase-segregated constituents which kept their identity in the nanocomposite materials. The NCC phase was found to be homogeneously dispersed in the PBAT matrix inside. Similar to the corresponding microcomposites, the investigated nanocomposites were found to be stable within their desired application temperature as packaging materials. The tensile properties of the nanocomposites degraded in terms of strain at break, tensile strength and tensile modulus. At higher filler content, the reinforcing effect dominated leading to an increase in indentation modulus and hardness, and a decrease in the work of elastic deformation. The wettability and the water absorption capacity of the materials increased with NCC content thereby enhancing the biodegradability of the composites.</description><subject>Cellulose</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Complex Fluids and Microfluidics</subject><subject>Contact angle</subject><subject>Elastic deformation</subject><subject>Fourier transforms</subject><subject>Load</subject><subject>Modulus of elasticity</subject><subject>Molecular weight</subject><subject>Nanocomposites</subject><subject>Organic Chemistry</subject><subject>Original Paper</subject><subject>Physical Chemistry</subject><subject>Polyethylene terephthalate</subject><subject>Polymer Sciences</subject><subject>Polymers</subject><subject>Polyvinyl alcohol</subject><subject>Raw materials</subject><subject>Soft and Granular Matter</subject><subject>Spectrum analysis</subject><subject>Surface properties</subject><subject>Tensile properties</subject><subject>Tensile strength</subject><subject>Terephthalate</subject><subject>Thermogravimetric analysis</subject><subject>Water absorption</subject><subject>Wettability</subject><subject>Wheat</subject><issn>0170-0839</issn><issn>1436-2449</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9UU1r3DAQFaGBbLf5AzkZemkhavVhy9KxhCQNLPTSnIUsj9dOtJIryYT9R_mZkbOF3nqaNzPvvRl4CF1R8o0S0n5PhDCpMGEMk5pLieUZ2tCaC8zqWn1AG0Jbgonk6gJ9TOmJlF4IukGvD35wC3gLVRiqlxFMrlI27rnyxgcLzi0upLL0ZRwXm5do3HV1ADsaP9kV5xHiYQVpiYMpRsb3VQ_7aHqTpyKcY5gh5gnSesOGwxzSlEv3MuWxmoM7fumWfHTgi7afZpMB24AzRJjHPBpXBl8_ofPBuASXf-sWPd7d_r75iXe_7h9ufuyw5VRlzEQ3mFaRRlmihq5umBoYFUI0tWxoL0nfcdFabgqWjPNG9B1V0EGnWkOV5Fv0-eRbvv6zQMr6KSzRl5OaKdoqrqhsC4udWDaGlCIMeo7TwcSjpkSviehTIrokot8T0as1P4lSIfs9xH_W_1G9AUZZklo</recordid><startdate>20230701</startdate><enddate>20230701</enddate><creator>Giri, Jyoti</creator><creator>Lach, Ralf</creator><creator>Henning, Sven</creator><creator>Grellmann, Wolfgang</creator><creator>Bhasney, Siddharth Mohan</creator><creator>Katiyar, Vimal</creator><creator>Saiter, Jean-Marc</creator><creator>Adhikari, Rameshwar</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><orcidid>https://orcid.org/0000-0003-0489-0154</orcidid><orcidid>https://orcid.org/0000-0002-2231-3839</orcidid><orcidid>https://orcid.org/0000-0002-7350-0204</orcidid><orcidid>https://orcid.org/0000-0003-4750-7653</orcidid><orcidid>https://orcid.org/0000-0003-0590-1468</orcidid><orcidid>https://orcid.org/0000-0002-5936-4410</orcidid><orcidid>https://orcid.org/0000-0003-2896-9318</orcidid><orcidid>https://orcid.org/0000-0002-3724-3562</orcidid></search><sort><creationdate>20230701</creationdate><title>Influence of wheat stalk nanocellulose on structural, mechanical, thermal, surface and degradation properties of composites with poly(butylene adipate-co-terephthalate)</title><author>Giri, Jyoti ; Lach, Ralf ; Henning, Sven ; Grellmann, Wolfgang ; Bhasney, Siddharth Mohan ; Katiyar, Vimal ; Saiter, Jean-Marc ; Adhikari, Rameshwar</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-26bfa79059c09fb4529f2166654851d80db367c3a1d8823356db19ebeb97a1983</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Cellulose</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Complex Fluids and Microfluidics</topic><topic>Contact angle</topic><topic>Elastic deformation</topic><topic>Fourier transforms</topic><topic>Load</topic><topic>Modulus of elasticity</topic><topic>Molecular weight</topic><topic>Nanocomposites</topic><topic>Organic Chemistry</topic><topic>Original Paper</topic><topic>Physical Chemistry</topic><topic>Polyethylene terephthalate</topic><topic>Polymer Sciences</topic><topic>Polymers</topic><topic>Polyvinyl alcohol</topic><topic>Raw materials</topic><topic>Soft and Granular Matter</topic><topic>Spectrum analysis</topic><topic>Surface properties</topic><topic>Tensile properties</topic><topic>Tensile strength</topic><topic>Terephthalate</topic><topic>Thermogravimetric analysis</topic><topic>Water absorption</topic><topic>Wettability</topic><topic>Wheat</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Giri, Jyoti</creatorcontrib><creatorcontrib>Lach, Ralf</creatorcontrib><creatorcontrib>Henning, Sven</creatorcontrib><creatorcontrib>Grellmann, Wolfgang</creatorcontrib><creatorcontrib>Bhasney, Siddharth Mohan</creatorcontrib><creatorcontrib>Katiyar, Vimal</creatorcontrib><creatorcontrib>Saiter, Jean-Marc</creatorcontrib><creatorcontrib>Adhikari, Rameshwar</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><jtitle>Polymer bulletin (Berlin, Germany)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Giri, Jyoti</au><au>Lach, Ralf</au><au>Henning, Sven</au><au>Grellmann, Wolfgang</au><au>Bhasney, Siddharth Mohan</au><au>Katiyar, Vimal</au><au>Saiter, Jean-Marc</au><au>Adhikari, Rameshwar</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Influence of wheat stalk nanocellulose on structural, mechanical, thermal, surface and degradation properties of composites with poly(butylene adipate-co-terephthalate)</atitle><jtitle>Polymer bulletin (Berlin, Germany)</jtitle><stitle>Polym. 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-terephthalate) (PBAT) and the wheat stalk-based nanocellulose (NCC) were studied. The materials were found to comprise the compatible and yet phase-segregated constituents which kept their identity in the nanocomposite materials. The NCC phase was found to be homogeneously dispersed in the PBAT matrix inside. Similar to the corresponding microcomposites, the investigated nanocomposites were found to be stable within their desired application temperature as packaging materials. The tensile properties of the nanocomposites degraded in terms of strain at break, tensile strength and tensile modulus. At higher filler content, the reinforcing effect dominated leading to an increase in indentation modulus and hardness, and a decrease in the work of elastic deformation. The wettability and the water absorption capacity of the materials increased with NCC content thereby enhancing the biodegradability of the composites.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s00289-022-04388-8</doi><tpages>27</tpages><orcidid>https://orcid.org/0000-0003-0489-0154</orcidid><orcidid>https://orcid.org/0000-0002-2231-3839</orcidid><orcidid>https://orcid.org/0000-0002-7350-0204</orcidid><orcidid>https://orcid.org/0000-0003-4750-7653</orcidid><orcidid>https://orcid.org/0000-0003-0590-1468</orcidid><orcidid>https://orcid.org/0000-0002-5936-4410</orcidid><orcidid>https://orcid.org/0000-0003-2896-9318</orcidid><orcidid>https://orcid.org/0000-0002-3724-3562</orcidid></addata></record> |
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| ispartof | Polymer bulletin (Berlin, Germany), 2023-07, Vol.80 (7), p.7599-7625 |
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| subjects | Cellulose Characterization and Evaluation of Materials Chemistry Chemistry and Materials Science Complex Fluids and Microfluidics Contact angle Elastic deformation Fourier transforms Load Modulus of elasticity Molecular weight Nanocomposites Organic Chemistry Original Paper Physical Chemistry Polyethylene terephthalate Polymer Sciences Polymers Polyvinyl alcohol Raw materials Soft and Granular Matter Spectrum analysis Surface properties Tensile properties Tensile strength Terephthalate Thermogravimetric analysis Water absorption Wettability Wheat |
| title | Influence of wheat stalk nanocellulose on structural, mechanical, thermal, surface and degradation properties of composites with poly(butylene adipate-co-terephthalate) |
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