Synthesis and lead ion absorption of magnetic hydrogel nanocomposite absorbents with semi-IPNs structure
γ-Methacryloxypropyl trimethoxysilane (KH570)-modified magnetic hydrogel nanocomposite absorbents with semi-interpenetrating networks (semi-IPNs-KH570-mHNAs) were synthesized by radical copolymerization via poly(acrylamide-co-acrylic acid), polyvinyl pyrrolidone (PVP) and KH570-modified magnetic nan...
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| Veröffentlicht in: | Polymer bulletin (Berlin, Germany) Germany), 2023-04, Vol.80 (4), p.3633-3647 |
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| creator | Wan, Tao Wang, Jian He, Songsong Wang, Tairan Zheng, Yan Xie, Fangling Tang, Qi |
| description | γ-Methacryloxypropyl trimethoxysilane (KH570)-modified magnetic hydrogel nanocomposite absorbents with semi-interpenetrating networks (semi-IPNs-KH570-mHNAs) were synthesized by radical copolymerization via poly(acrylamide-co-acrylic acid), polyvinyl pyrrolidone (PVP) and KH570-modified magnetic nanoparticles. FTIR and XRD results preliminarily confirmed the target structure of semi-IPNs-KH570-mHNAs without destroying the structure of magnetic nanoparticles during KH570 modification and radical polymerization. Semi-IPNs-KH570-mHNAs with many porous and ravine structure had high adsorption capacity for Pb(II) (450 mg/g). Semi-IPNs-KH570-mHNAs had the best absorption capacity for Pb(II) ion in the synthesis condition of acrylic acid/acrylamide mass ratio of 60:40, 0.8% initiator, acrylic acid (AA) neutralization degree of 70%, 0.2% cross-linker, 12% PVP and 10% KH570-modified magnetic nanoparticles. Besides, semi-IPNs-KH570-mHNAs had good magnetic responsiveness, high thermal stability, reusability which made it a potential application in removing heavy metal ions from the contaminated wastewater. |
| doi_str_mv | 10.1007/s00289-022-04220-3 |
| format | Article |
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FTIR and XRD results preliminarily confirmed the target structure of semi-IPNs-KH570-mHNAs without destroying the structure of magnetic nanoparticles during KH570 modification and radical polymerization. Semi-IPNs-KH570-mHNAs with many porous and ravine structure had high adsorption capacity for Pb(II) (450 mg/g). Semi-IPNs-KH570-mHNAs had the best absorption capacity for Pb(II) ion in the synthesis condition of acrylic acid/acrylamide mass ratio of 60:40, 0.8% initiator, acrylic acid (AA) neutralization degree of 70%, 0.2% cross-linker, 12% PVP and 10% KH570-modified magnetic nanoparticles. Besides, semi-IPNs-KH570-mHNAs had good magnetic responsiveness, high thermal stability, reusability which made it a potential application in removing heavy metal ions from the contaminated wastewater.</description><identifier>ISSN: 0170-0839</identifier><identifier>EISSN: 1436-2449</identifier><identifier>DOI: 10.1007/s00289-022-04220-3</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Absorbents ; Absorption ; Acids ; Acrylamide ; Acrylic acid ; Adsorption ; Characterization and Evaluation of Materials ; Chemical synthesis ; Chemicals ; Chemistry ; Chemistry and Materials Science ; Complex Fluids and Microfluidics ; Copolymerization ; Electron microscopes ; Ethanol ; Heavy metals ; Hydrogels ; Interpenetrating networks ; Lead ; Lead content ; Metal ions ; Nanocomposites ; Nanoparticles ; Organic Chemistry ; Original Paper ; Physical Chemistry ; Polymer Sciences ; Polymers ; Radicals ; Reagents ; Scientific imaging ; Soft and Granular Matter ; Thermal stability</subject><ispartof>Polymer bulletin (Berlin, Germany), 2023-04, Vol.80 (4), p.3633-3647</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-8920b3b085a06a9a1b93e65cf45e4e5a7c841bc8f08937e1e56e00d12717b9df3</citedby><cites>FETCH-LOGICAL-c319t-8920b3b085a06a9a1b93e65cf45e4e5a7c841bc8f08937e1e56e00d12717b9df3</cites><orcidid>0000-0002-8881-6973</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s00289-022-04220-3$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2917934082?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>314,780,784,21386,27922,27923,33742,41486,42555,43803,51317,64383,64387,72239</link.rule.ids></links><search><creatorcontrib>Wan, Tao</creatorcontrib><creatorcontrib>Wang, Jian</creatorcontrib><creatorcontrib>He, Songsong</creatorcontrib><creatorcontrib>Wang, Tairan</creatorcontrib><creatorcontrib>Zheng, Yan</creatorcontrib><creatorcontrib>Xie, Fangling</creatorcontrib><creatorcontrib>Tang, Qi</creatorcontrib><title>Synthesis and lead ion absorption of magnetic hydrogel nanocomposite absorbents with semi-IPNs structure</title><title>Polymer bulletin (Berlin, Germany)</title><addtitle>Polym. Bull</addtitle><description>γ-Methacryloxypropyl trimethoxysilane (KH570)-modified magnetic hydrogel nanocomposite absorbents with semi-interpenetrating networks (semi-IPNs-KH570-mHNAs) were synthesized by radical copolymerization via poly(acrylamide-co-acrylic acid), polyvinyl pyrrolidone (PVP) and KH570-modified magnetic nanoparticles. FTIR and XRD results preliminarily confirmed the target structure of semi-IPNs-KH570-mHNAs without destroying the structure of magnetic nanoparticles during KH570 modification and radical polymerization. Semi-IPNs-KH570-mHNAs with many porous and ravine structure had high adsorption capacity for Pb(II) (450 mg/g). Semi-IPNs-KH570-mHNAs had the best absorption capacity for Pb(II) ion in the synthesis condition of acrylic acid/acrylamide mass ratio of 60:40, 0.8% initiator, acrylic acid (AA) neutralization degree of 70%, 0.2% cross-linker, 12% PVP and 10% KH570-modified magnetic nanoparticles. Besides, semi-IPNs-KH570-mHNAs had good magnetic responsiveness, high thermal stability, reusability which made it a potential application in removing heavy metal ions from the contaminated wastewater.</description><subject>Absorbents</subject><subject>Absorption</subject><subject>Acids</subject><subject>Acrylamide</subject><subject>Acrylic acid</subject><subject>Adsorption</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemical synthesis</subject><subject>Chemicals</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Complex Fluids and Microfluidics</subject><subject>Copolymerization</subject><subject>Electron microscopes</subject><subject>Ethanol</subject><subject>Heavy metals</subject><subject>Hydrogels</subject><subject>Interpenetrating networks</subject><subject>Lead</subject><subject>Lead content</subject><subject>Metal ions</subject><subject>Nanocomposites</subject><subject>Nanoparticles</subject><subject>Organic Chemistry</subject><subject>Original Paper</subject><subject>Physical Chemistry</subject><subject>Polymer Sciences</subject><subject>Polymers</subject><subject>Radicals</subject><subject>Reagents</subject><subject>Scientific imaging</subject><subject>Soft and Granular Matter</subject><subject>Thermal stability</subject><issn>0170-0839</issn><issn>1436-2449</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kE1LxDAQhoMouK7-AU8Bz9FJ0q8cZfELFhXUc0jb6bbLNqlJiuy_t2sFb55mBp73HXgIueRwzQHymwAgCsVACAaJEMDkEVnwRGZMJIk6JgvgOTAopDolZyFsYbqzjC9I-7a3scXQBWpsTXdoato5S00ZnB_iYXUN7c3GYuwq2u5r7za4o9ZYV7l-cKGLONMl2hjoVxdbGrDv2NPrc6Ah-rGKo8dzctKYXcCL37kkH_d376tHtn55eFrdrlkluYqsUAJKWUKRGsiMMrxUErO0apIUE0xNXhUJL6uigULJHDmmGQLUXOQ8L1XdyCW5mnsH7z5HDFFv3ejt9FILxXMlEyjERImZqrwLwWOjB9_1xu81B30wqmejejKqf4xqOYXkHAoTbDfo_6r_SX0D4kh6Zg</recordid><startdate>20230401</startdate><enddate>20230401</enddate><creator>Wan, Tao</creator><creator>Wang, Jian</creator><creator>He, Songsong</creator><creator>Wang, Tairan</creator><creator>Zheng, Yan</creator><creator>Xie, Fangling</creator><creator>Tang, Qi</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><orcidid>https://orcid.org/0000-0002-8881-6973</orcidid></search><sort><creationdate>20230401</creationdate><title>Synthesis and lead ion absorption of magnetic hydrogel nanocomposite absorbents with semi-IPNs structure</title><author>Wan, Tao ; Wang, Jian ; He, Songsong ; Wang, Tairan ; Zheng, Yan ; Xie, Fangling ; Tang, Qi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-8920b3b085a06a9a1b93e65cf45e4e5a7c841bc8f08937e1e56e00d12717b9df3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Absorbents</topic><topic>Absorption</topic><topic>Acids</topic><topic>Acrylamide</topic><topic>Acrylic acid</topic><topic>Adsorption</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemical synthesis</topic><topic>Chemicals</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Complex Fluids and Microfluidics</topic><topic>Copolymerization</topic><topic>Electron microscopes</topic><topic>Ethanol</topic><topic>Heavy metals</topic><topic>Hydrogels</topic><topic>Interpenetrating networks</topic><topic>Lead</topic><topic>Lead content</topic><topic>Metal ions</topic><topic>Nanocomposites</topic><topic>Nanoparticles</topic><topic>Organic Chemistry</topic><topic>Original Paper</topic><topic>Physical Chemistry</topic><topic>Polymer Sciences</topic><topic>Polymers</topic><topic>Radicals</topic><topic>Reagents</topic><topic>Scientific imaging</topic><topic>Soft and Granular Matter</topic><topic>Thermal stability</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wan, Tao</creatorcontrib><creatorcontrib>Wang, Jian</creatorcontrib><creatorcontrib>He, Songsong</creatorcontrib><creatorcontrib>Wang, Tairan</creatorcontrib><creatorcontrib>Zheng, Yan</creatorcontrib><creatorcontrib>Xie, Fangling</creatorcontrib><creatorcontrib>Tang, Qi</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><jtitle>Polymer bulletin (Berlin, Germany)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wan, Tao</au><au>Wang, Jian</au><au>He, Songsong</au><au>Wang, Tairan</au><au>Zheng, Yan</au><au>Xie, Fangling</au><au>Tang, Qi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Synthesis and lead ion absorption of magnetic hydrogel nanocomposite absorbents with semi-IPNs structure</atitle><jtitle>Polymer bulletin (Berlin, Germany)</jtitle><stitle>Polym. Bull</stitle><date>2023-04-01</date><risdate>2023</risdate><volume>80</volume><issue>4</issue><spage>3633</spage><epage>3647</epage><pages>3633-3647</pages><issn>0170-0839</issn><eissn>1436-2449</eissn><abstract>γ-Methacryloxypropyl trimethoxysilane (KH570)-modified magnetic hydrogel nanocomposite absorbents with semi-interpenetrating networks (semi-IPNs-KH570-mHNAs) were synthesized by radical copolymerization via poly(acrylamide-co-acrylic acid), polyvinyl pyrrolidone (PVP) and KH570-modified magnetic nanoparticles. FTIR and XRD results preliminarily confirmed the target structure of semi-IPNs-KH570-mHNAs without destroying the structure of magnetic nanoparticles during KH570 modification and radical polymerization. Semi-IPNs-KH570-mHNAs with many porous and ravine structure had high adsorption capacity for Pb(II) (450 mg/g). Semi-IPNs-KH570-mHNAs had the best absorption capacity for Pb(II) ion in the synthesis condition of acrylic acid/acrylamide mass ratio of 60:40, 0.8% initiator, acrylic acid (AA) neutralization degree of 70%, 0.2% cross-linker, 12% PVP and 10% KH570-modified magnetic nanoparticles. Besides, semi-IPNs-KH570-mHNAs had good magnetic responsiveness, high thermal stability, reusability which made it a potential application in removing heavy metal ions from the contaminated wastewater.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s00289-022-04220-3</doi><tpages>15</tpages><orcidid>https://orcid.org/0000-0002-8881-6973</orcidid></addata></record> |
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| subjects | Absorbents Absorption Acids Acrylamide Acrylic acid Adsorption Characterization and Evaluation of Materials Chemical synthesis Chemicals Chemistry Chemistry and Materials Science Complex Fluids and Microfluidics Copolymerization Electron microscopes Ethanol Heavy metals Hydrogels Interpenetrating networks Lead Lead content Metal ions Nanocomposites Nanoparticles Organic Chemistry Original Paper Physical Chemistry Polymer Sciences Polymers Radicals Reagents Scientific imaging Soft and Granular Matter Thermal stability |
| title | Synthesis and lead ion absorption of magnetic hydrogel nanocomposite absorbents with semi-IPNs structure |
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