Wet-Type Packed-Bed Nonthermal Plasma for Simultaneous Removal of PM and VOCs

Several regulations on exhaust gases have been introduced to curb hazardous exhaust of volatile organic compounds (VOCs) and particulate matter (PM) from the paint and printing industries. VOCs produce photochemical oxidants and suspended PM such as PM 2.5 , which is now recognized as a global envir...

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Veröffentlicht in:Plasma chemistry and plasma processing 2024, Vol.44 (1), p.239-255
Hauptverfasser: Shimada, Takumi, Yamasaki, Haruhiko, Kuroki, Tomoyuki, Kang, Jinkyu, Kim, Dong-Wook, Yagi, Tadao, Okubo, Masaaki
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container_end_page 255
container_issue 1
container_start_page 239
container_title Plasma chemistry and plasma processing
container_volume 44
creator Shimada, Takumi
Yamasaki, Haruhiko
Kuroki, Tomoyuki
Kang, Jinkyu
Kim, Dong-Wook
Yagi, Tadao
Okubo, Masaaki
description Several regulations on exhaust gases have been introduced to curb hazardous exhaust of volatile organic compounds (VOCs) and particulate matter (PM) from the paint and printing industries. VOCs produce photochemical oxidants and suspended PM such as PM 2.5 , which is now recognized as a global environmental problem. We assess a nonthermal plasma technique for controlling VOC emissions, especially, propose a wet-type packed-bed plasma reactor to extend the treatment of water-non-soluble VOCs. This paper proposes a wet-type packed-bed plasma reactor to extend the treatment of water-non-soluble VOCs. The proposed technique is evaluated through the simultaneous removal of nanoparticles and toluene at a relatively high flow rate. Simultaneous treatment of the VOCs and nanoparticles using the reactor indicates that the average particle collection efficiency is 94%, and the removal efficiency of 60 ppm toluene is 73% with a gas flow rate of 10 L/min. The resultant byproducts are benzaldehyde (C 6 H 5 CHO), benzyl alcohol (C 6 H 5 CH 2 OH), phenol (C 6 H 5 OH), ozone, formic acid, and acetic acid, and some are easily dissolved and removed by the sodium hydroxide solution film. A smaller pellet diameter leads to more efficient toluene removal at lower specific energy values, while the ozone concentration does not change. However, the ozone concentration can be greatly suppressed by dissolving the ozone in the alkali solution film.
doi_str_mv 10.1007/s11090-023-10403-1
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subjects Acetic acid
Benzaldehyde
Benzyl alcohol
Characterization and Evaluation of Materials
Chemistry
Chemistry and Materials Science
Classical Mechanics
Energy value
Exhaust gases
Flow velocity
Formic acid
Gas flow
Inorganic Chemistry
Mechanical Engineering
Nanoparticles
Original Paper
Oxidizing agents
Ozone
Particulate emissions
Photochemical oxidants
Plasma
Sodium hydroxide
Specific energy
Toluene
VOCs
Volatile organic compounds
title Wet-Type Packed-Bed Nonthermal Plasma for Simultaneous Removal of PM and VOCs
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