Preparation of PVA/PVDF/PAM-U composite hydrogels by in situ polymerization of ternary DES and their properties study
Preparation of composite hydrogels by in situ polymerization (SP) using choline chloride (ChCl), acrylamide (AM), and urea (U) as raw materials for deep eutectic solvent (DES), with the introduction of PVA and PVDF as fillers into DES. Characterization of the composite hydrogels was conducted using...
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| Veröffentlicht in: | Journal of materials science 2024, Vol.59 (2), p.715-727 |
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| creator | Li, Bin Zhou, Mengjing Wu, Aolin Liu, Haiying Du, Li Su, Lihua |
| description | Preparation of composite hydrogels by in situ polymerization (SP) using choline chloride (ChCl), acrylamide (AM), and urea (U) as raw materials for deep eutectic solvent (DES), with the introduction of PVA and PVDF as fillers into DES. Characterization of the composite hydrogels was conducted using Fourier transform infrared spectroscopy (FTIR) and scanning electron microscopy (SEM). This study analyzed the pressure sensitivity, piezoelectricity, swelling behavior, and mechanical properties of the composite hydrogels. The results indicate that due to the dipole–dipole interactions between PVA and PVDF, the composite hydrogels exhibit excellent pressure sensitivity and piezoelectric performance. When the ratio of PVA to PVDF is 1:1, the composite hydrogels exhibit optimal performance, with a 3.37-fold increase in pressure sensitivity and a 6.49-fold increase in piezoelectricity compared to other ratios. This research provides a method for preparing composite hydrogels with excellent piezoelectric performance and pressure sensitivity. |
| doi_str_mv | 10.1007/s10853-023-09247-z |
| format | Article |
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Characterization of the composite hydrogels was conducted using Fourier transform infrared spectroscopy (FTIR) and scanning electron microscopy (SEM). This study analyzed the pressure sensitivity, piezoelectricity, swelling behavior, and mechanical properties of the composite hydrogels. The results indicate that due to the dipole–dipole interactions between PVA and PVDF, the composite hydrogels exhibit excellent pressure sensitivity and piezoelectric performance. When the ratio of PVA to PVDF is 1:1, the composite hydrogels exhibit optimal performance, with a 3.37-fold increase in pressure sensitivity and a 6.49-fold increase in piezoelectricity compared to other ratios. This research provides a method for preparing composite hydrogels with excellent piezoelectric performance and pressure sensitivity.</description><identifier>ISSN: 0022-2461</identifier><identifier>EISSN: 1573-4803</identifier><identifier>DOI: 10.1007/s10853-023-09247-z</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Acrylamide ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Choline ; Classical Mechanics ; Crystallography and Scattering Methods ; Dipole interactions ; Fourier transforms ; Hydrogels ; Infrared analysis ; Materials Science ; Mechanical properties ; Piezoelectricity ; Polymer Sciences ; Polymerization ; Polymers & Biopolymers ; Raw materials ; Sensitivity analysis ; Solid Mechanics</subject><ispartof>Journal of materials science, 2024, Vol.59 (2), p.715-727</ispartof><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c270t-3e515f66a22db88f246e680249d11c51cfbd32273d59a9e2743feac546c40a4c3</cites><orcidid>0000-0002-8414-0435</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10853-023-09247-z$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10853-023-09247-z$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Li, Bin</creatorcontrib><creatorcontrib>Zhou, Mengjing</creatorcontrib><creatorcontrib>Wu, Aolin</creatorcontrib><creatorcontrib>Liu, Haiying</creatorcontrib><creatorcontrib>Du, Li</creatorcontrib><creatorcontrib>Su, Lihua</creatorcontrib><title>Preparation of PVA/PVDF/PAM-U composite hydrogels by in situ polymerization of ternary DES and their properties study</title><title>Journal of materials science</title><addtitle>J Mater Sci</addtitle><description>Preparation of composite hydrogels by in situ polymerization (SP) using choline chloride (ChCl), acrylamide (AM), and urea (U) as raw materials for deep eutectic solvent (DES), with the introduction of PVA and PVDF as fillers into DES. Characterization of the composite hydrogels was conducted using Fourier transform infrared spectroscopy (FTIR) and scanning electron microscopy (SEM). This study analyzed the pressure sensitivity, piezoelectricity, swelling behavior, and mechanical properties of the composite hydrogels. The results indicate that due to the dipole–dipole interactions between PVA and PVDF, the composite hydrogels exhibit excellent pressure sensitivity and piezoelectric performance. When the ratio of PVA to PVDF is 1:1, the composite hydrogels exhibit optimal performance, with a 3.37-fold increase in pressure sensitivity and a 6.49-fold increase in piezoelectricity compared to other ratios. This research provides a method for preparing composite hydrogels with excellent piezoelectric performance and pressure sensitivity.</description><subject>Acrylamide</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Choline</subject><subject>Classical Mechanics</subject><subject>Crystallography and Scattering Methods</subject><subject>Dipole interactions</subject><subject>Fourier transforms</subject><subject>Hydrogels</subject><subject>Infrared analysis</subject><subject>Materials Science</subject><subject>Mechanical properties</subject><subject>Piezoelectricity</subject><subject>Polymer Sciences</subject><subject>Polymerization</subject><subject>Polymers & Biopolymers</subject><subject>Raw materials</subject><subject>Sensitivity analysis</subject><subject>Solid Mechanics</subject><issn>0022-2461</issn><issn>1573-4803</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kEtPwzAQhC0EEqXwBzhZ4hzqZ5wcq7Y8pCIiQXu1XMdpU7VxsJ1D-usxBMGNw2ql1Xyj2QHgFqN7jJCYeIwyThNE4uSEieR0BkaYC5qwDNFzMEKIkISwFF-CK-_3CCEuCB6BrnCmVU6F2jbQVrBYTyfFev4wKaYvyQpqe2ytr4OBu750dmsOHm56WDcwHjvY2kN_NK4-_fLBuEa5Hs4Xb1A1JQw7UzvYOtsaF2rjoQ9d2V-Di0odvLn52WOweli8z56S5evj82y6TDQRKCTUcMyrNFWElJssq2J-k2aIsLzEWHOsq01JCRG05LnKDRGMVkZpzlLNkGKajsHd4BsDfHTGB7m3XQx48JLkmHIhMsSjigwq7az3zlSydfUxfiExkl_1yqFeGeuV3_XKU4ToAPkobrbG_Vn_Q30Cigp-ZA</recordid><startdate>2024</startdate><enddate>2024</enddate><creator>Li, Bin</creator><creator>Zhou, Mengjing</creator><creator>Wu, Aolin</creator><creator>Liu, Haiying</creator><creator>Du, Li</creator><creator>Su, Lihua</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-8414-0435</orcidid></search><sort><creationdate>2024</creationdate><title>Preparation of PVA/PVDF/PAM-U composite hydrogels by in situ polymerization of ternary DES and their properties study</title><author>Li, Bin ; Zhou, Mengjing ; Wu, Aolin ; Liu, Haiying ; Du, Li ; Su, Lihua</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c270t-3e515f66a22db88f246e680249d11c51cfbd32273d59a9e2743feac546c40a4c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Acrylamide</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Choline</topic><topic>Classical Mechanics</topic><topic>Crystallography and Scattering Methods</topic><topic>Dipole interactions</topic><topic>Fourier transforms</topic><topic>Hydrogels</topic><topic>Infrared analysis</topic><topic>Materials Science</topic><topic>Mechanical properties</topic><topic>Piezoelectricity</topic><topic>Polymer Sciences</topic><topic>Polymerization</topic><topic>Polymers & Biopolymers</topic><topic>Raw materials</topic><topic>Sensitivity analysis</topic><topic>Solid Mechanics</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Bin</creatorcontrib><creatorcontrib>Zhou, Mengjing</creatorcontrib><creatorcontrib>Wu, Aolin</creatorcontrib><creatorcontrib>Liu, Haiying</creatorcontrib><creatorcontrib>Du, Li</creatorcontrib><creatorcontrib>Su, Lihua</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of materials science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Bin</au><au>Zhou, Mengjing</au><au>Wu, Aolin</au><au>Liu, Haiying</au><au>Du, Li</au><au>Su, Lihua</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Preparation of PVA/PVDF/PAM-U composite hydrogels by in situ polymerization of ternary DES and their properties study</atitle><jtitle>Journal of materials science</jtitle><stitle>J Mater Sci</stitle><date>2024</date><risdate>2024</risdate><volume>59</volume><issue>2</issue><spage>715</spage><epage>727</epage><pages>715-727</pages><issn>0022-2461</issn><eissn>1573-4803</eissn><abstract>Preparation of composite hydrogels by in situ polymerization (SP) using choline chloride (ChCl), acrylamide (AM), and urea (U) as raw materials for deep eutectic solvent (DES), with the introduction of PVA and PVDF as fillers into DES. Characterization of the composite hydrogels was conducted using Fourier transform infrared spectroscopy (FTIR) and scanning electron microscopy (SEM). This study analyzed the pressure sensitivity, piezoelectricity, swelling behavior, and mechanical properties of the composite hydrogels. The results indicate that due to the dipole–dipole interactions between PVA and PVDF, the composite hydrogels exhibit excellent pressure sensitivity and piezoelectric performance. When the ratio of PVA to PVDF is 1:1, the composite hydrogels exhibit optimal performance, with a 3.37-fold increase in pressure sensitivity and a 6.49-fold increase in piezoelectricity compared to other ratios. This research provides a method for preparing composite hydrogels with excellent piezoelectric performance and pressure sensitivity.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10853-023-09247-z</doi><tpages>13</tpages><orcidid>https://orcid.org/0000-0002-8414-0435</orcidid></addata></record> |
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| subjects | Acrylamide Characterization and Evaluation of Materials Chemistry and Materials Science Choline Classical Mechanics Crystallography and Scattering Methods Dipole interactions Fourier transforms Hydrogels Infrared analysis Materials Science Mechanical properties Piezoelectricity Polymer Sciences Polymerization Polymers & Biopolymers Raw materials Sensitivity analysis Solid Mechanics |
| title | Preparation of PVA/PVDF/PAM-U composite hydrogels by in situ polymerization of ternary DES and their properties study |
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