Mechanistic understanding of 3d-metal phthalocyanine catalysts: heterostructure regulation of dz2 orbitals for efficient CO2 reduction

Heterostructure molecular catalysts have attracted significant attention for their distinctive catalytic activity in the electrocatalytic CO2 reduction reaction. To investigate the intrinsic reaction mechanisms, 3d-transition metal-phthalocyanine-based catalysts were systematically investigated. The...

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Veröffentlicht in:	Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2023-11, Vol.11 (44), p.24359-24370
Hauptverfasser:	Xiao, Jiayong, Masana, Jofrey J, Dong, Hao, Zhang, Hui, Yang, Haolan, Qiu, Ming, Yu, Ying
Format:	Artikel
Sprache:	eng
Schlagworte:	Carbon dioxide Catalysts Catalytic activity Chemical reduction Graphene Heterostructures Metal phthalocyanines Metals Molecular dynamics Orbitals Reaction kinetics Reaction mechanisms Transition metals Volcanoes
Online-Zugang:	Volltext
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