Fabrication of Ni-MOFs/MWCNTs by in situ growth for high-performance supercapacitor electrode materials
Metal–organic frameworks (MOFs) have low conductivity, which is not conducive to further application. To address the issue, in this work, using carboxylation multiwall carbon nanotubes (MWCNTs-COOH) as carbon materials, benzene-1,4-dicarboxylic acid (PTA) as organic ligands, nickel nitrate hexahydra...
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| Veröffentlicht in: | Journal of materials science. Materials in electronics 2023-10, Vol.34 (28), p.1920, Article 1920 |
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| creator | Wang, Jia-Wei Meng, Tian-Li Ma, Ying-Xia Lei, Lei Li, Jing Ran, Fen |
| description | Metal–organic frameworks (MOFs) have low conductivity, which is not conducive to further application. To address the issue, in this work, using carboxylation multiwall carbon nanotubes (MWCNTs-COOH) as carbon materials, benzene-1,4-dicarboxylic acid (PTA) as organic ligands, nickel nitrate hexahydrate (Ni(NO
3
)
2
·6H
2
O) as transition metal ions precursors, MWCNTs decorated with nickel MOFs (Ni-MOFs/MWCNTs) nanohybrids were fabricated via in situ growth by a one-pot solvothermal method. The electrochemical properties of the Ni-MOFs/MWCNTs nanohybrids obtained by adjusting the dosage of MWCNTs-COOH and the experimental conditions as electrode materials for supercapacitors (SCs) were investigated. The results showed that the Ni-MOFs nanoflowers self-assembled by nanorods were in situ growth on the MWCNTs, which could avoid the agglomeration of Ni-MOFs and MWCNTs, enhance the specific surface area, and expose more active sites to improve the electrochemical properties. The specific capacity of the Ni-MOFs/MWCNTs nanohybrids as electrode materials obtained at the optimal experimental conditions was 749.6 C g
−1
at 1.0 A g
−1
. |
| doi_str_mv | 10.1007/s10854-023-11286-w |
| format | Article |
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3
)
2
·6H
2
O) as transition metal ions precursors, MWCNTs decorated with nickel MOFs (Ni-MOFs/MWCNTs) nanohybrids were fabricated via in situ growth by a one-pot solvothermal method. The electrochemical properties of the Ni-MOFs/MWCNTs nanohybrids obtained by adjusting the dosage of MWCNTs-COOH and the experimental conditions as electrode materials for supercapacitors (SCs) were investigated. The results showed that the Ni-MOFs nanoflowers self-assembled by nanorods were in situ growth on the MWCNTs, which could avoid the agglomeration of Ni-MOFs and MWCNTs, enhance the specific surface area, and expose more active sites to improve the electrochemical properties. The specific capacity of the Ni-MOFs/MWCNTs nanohybrids as electrode materials obtained at the optimal experimental conditions was 749.6 C g
−1
at 1.0 A g
−1
.</description><identifier>ISSN: 0957-4522</identifier><identifier>EISSN: 1573-482X</identifier><identifier>DOI: 10.1007/s10854-023-11286-w</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Benzene ; Carboxylation ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Dicarboxylic acids ; Electrochemical analysis ; Electrode materials ; Electrodes ; Low conductivity ; Materials Science ; Metal-organic frameworks ; Multi wall carbon nanotubes ; Nanorods ; Nickel ; Optical and Electronic Materials ; Self-assembly ; Supercapacitors ; Terephthalic acid ; Transition metals</subject><ispartof>Journal of materials science. Materials in electronics, 2023-10, Vol.34 (28), p.1920, Article 1920</ispartof><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-92058c7e7f7b19a3a57c49cfa2d6fdab56364a1b0a98f6bbad25a55feb51ebbf3</citedby><cites>FETCH-LOGICAL-c319t-92058c7e7f7b19a3a57c49cfa2d6fdab56364a1b0a98f6bbad25a55feb51ebbf3</cites><orcidid>0000-0002-1024-3968</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10854-023-11286-w$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10854-023-11286-w$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27923,27924,41487,42556,51318</link.rule.ids></links><search><creatorcontrib>Wang, Jia-Wei</creatorcontrib><creatorcontrib>Meng, Tian-Li</creatorcontrib><creatorcontrib>Ma, Ying-Xia</creatorcontrib><creatorcontrib>Lei, Lei</creatorcontrib><creatorcontrib>Li, Jing</creatorcontrib><creatorcontrib>Ran, Fen</creatorcontrib><title>Fabrication of Ni-MOFs/MWCNTs by in situ growth for high-performance supercapacitor electrode materials</title><title>Journal of materials science. Materials in electronics</title><addtitle>J Mater Sci: Mater Electron</addtitle><description>Metal–organic frameworks (MOFs) have low conductivity, which is not conducive to further application. To address the issue, in this work, using carboxylation multiwall carbon nanotubes (MWCNTs-COOH) as carbon materials, benzene-1,4-dicarboxylic acid (PTA) as organic ligands, nickel nitrate hexahydrate (Ni(NO
3
)
2
·6H
2
O) as transition metal ions precursors, MWCNTs decorated with nickel MOFs (Ni-MOFs/MWCNTs) nanohybrids were fabricated via in situ growth by a one-pot solvothermal method. The electrochemical properties of the Ni-MOFs/MWCNTs nanohybrids obtained by adjusting the dosage of MWCNTs-COOH and the experimental conditions as electrode materials for supercapacitors (SCs) were investigated. The results showed that the Ni-MOFs nanoflowers self-assembled by nanorods were in situ growth on the MWCNTs, which could avoid the agglomeration of Ni-MOFs and MWCNTs, enhance the specific surface area, and expose more active sites to improve the electrochemical properties. The specific capacity of the Ni-MOFs/MWCNTs nanohybrids as electrode materials obtained at the optimal experimental conditions was 749.6 C g
−1
at 1.0 A g
−1
.</description><subject>Benzene</subject><subject>Carboxylation</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Dicarboxylic acids</subject><subject>Electrochemical analysis</subject><subject>Electrode materials</subject><subject>Electrodes</subject><subject>Low conductivity</subject><subject>Materials Science</subject><subject>Metal-organic frameworks</subject><subject>Multi wall carbon nanotubes</subject><subject>Nanorods</subject><subject>Nickel</subject><subject>Optical and Electronic Materials</subject><subject>Self-assembly</subject><subject>Supercapacitors</subject><subject>Terephthalic acid</subject><subject>Transition metals</subject><issn>0957-4522</issn><issn>1573-482X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kFFLwzAUhYMoOKd_wKeAz3FJ2jTtowynwtxeJvoWkjTpMra2Jilj_95oBd98OvdyzzkXPgBuCb4nGPNZILhkOcI0Q4TQskDHMzAhjGcoL-nHOZjginGUM0ovwVUIO4xxkWflBDQLqbzTMrquhZ2FK4de14swe32frzYBqhN0LQwuDrDx3TFuoe083Lpmi3rj03yQrTYwDGnTspfaxXQ3e6Oj72oDDzIa7-Q-XIMLm8Tc_OoUvC0eN_NntFw_vcwflkhnpIqoopiVmhtuuSKVzCTjOq-0lbQubC0VK7Iil0RhWZW2UErWlEnGrFGMGKVsNgV3Y2_vu8_BhCh23eDb9FLQkpOK05zlyUVHl_ZdCN5Y0Xt3kP4kCBbfQMUIVCSg4geoOKZQNoZCMreN8X_V_6S-AGrYe18</recordid><startdate>20231001</startdate><enddate>20231001</enddate><creator>Wang, Jia-Wei</creator><creator>Meng, Tian-Li</creator><creator>Ma, Ying-Xia</creator><creator>Lei, Lei</creator><creator>Li, Jing</creator><creator>Ran, Fen</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>F28</scope><scope>FR3</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>L7M</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>S0W</scope><orcidid>https://orcid.org/0000-0002-1024-3968</orcidid></search><sort><creationdate>20231001</creationdate><title>Fabrication of Ni-MOFs/MWCNTs by in situ growth for high-performance supercapacitor electrode materials</title><author>Wang, Jia-Wei ; Meng, Tian-Li ; Ma, Ying-Xia ; Lei, Lei ; Li, Jing ; Ran, Fen</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-92058c7e7f7b19a3a57c49cfa2d6fdab56364a1b0a98f6bbad25a55feb51ebbf3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Benzene</topic><topic>Carboxylation</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Dicarboxylic acids</topic><topic>Electrochemical analysis</topic><topic>Electrode materials</topic><topic>Electrodes</topic><topic>Low conductivity</topic><topic>Materials Science</topic><topic>Metal-organic frameworks</topic><topic>Multi wall carbon nanotubes</topic><topic>Nanorods</topic><topic>Nickel</topic><topic>Optical and Electronic Materials</topic><topic>Self-assembly</topic><topic>Supercapacitors</topic><topic>Terephthalic acid</topic><topic>Transition metals</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Jia-Wei</creatorcontrib><creatorcontrib>Meng, Tian-Li</creatorcontrib><creatorcontrib>Ma, Ying-Xia</creatorcontrib><creatorcontrib>Lei, Lei</creatorcontrib><creatorcontrib>Li, Jing</creatorcontrib><creatorcontrib>Ran, Fen</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>DELNET Engineering & Technology Collection</collection><jtitle>Journal of materials science. Materials in electronics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wang, Jia-Wei</au><au>Meng, Tian-Li</au><au>Ma, Ying-Xia</au><au>Lei, Lei</au><au>Li, Jing</au><au>Ran, Fen</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Fabrication of Ni-MOFs/MWCNTs by in situ growth for high-performance supercapacitor electrode materials</atitle><jtitle>Journal of materials science. Materials in electronics</jtitle><stitle>J Mater Sci: Mater Electron</stitle><date>2023-10-01</date><risdate>2023</risdate><volume>34</volume><issue>28</issue><spage>1920</spage><pages>1920-</pages><artnum>1920</artnum><issn>0957-4522</issn><eissn>1573-482X</eissn><abstract>Metal–organic frameworks (MOFs) have low conductivity, which is not conducive to further application. To address the issue, in this work, using carboxylation multiwall carbon nanotubes (MWCNTs-COOH) as carbon materials, benzene-1,4-dicarboxylic acid (PTA) as organic ligands, nickel nitrate hexahydrate (Ni(NO
3
)
2
·6H
2
O) as transition metal ions precursors, MWCNTs decorated with nickel MOFs (Ni-MOFs/MWCNTs) nanohybrids were fabricated via in situ growth by a one-pot solvothermal method. The electrochemical properties of the Ni-MOFs/MWCNTs nanohybrids obtained by adjusting the dosage of MWCNTs-COOH and the experimental conditions as electrode materials for supercapacitors (SCs) were investigated. The results showed that the Ni-MOFs nanoflowers self-assembled by nanorods were in situ growth on the MWCNTs, which could avoid the agglomeration of Ni-MOFs and MWCNTs, enhance the specific surface area, and expose more active sites to improve the electrochemical properties. The specific capacity of the Ni-MOFs/MWCNTs nanohybrids as electrode materials obtained at the optimal experimental conditions was 749.6 C g
−1
at 1.0 A g
−1
.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10854-023-11286-w</doi><orcidid>https://orcid.org/0000-0002-1024-3968</orcidid></addata></record> |
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| source | SpringerLink Journals - AutoHoldings |
| subjects | Benzene Carboxylation Characterization and Evaluation of Materials Chemistry and Materials Science Dicarboxylic acids Electrochemical analysis Electrode materials Electrodes Low conductivity Materials Science Metal-organic frameworks Multi wall carbon nanotubes Nanorods Nickel Optical and Electronic Materials Self-assembly Supercapacitors Terephthalic acid Transition metals |
| title | Fabrication of Ni-MOFs/MWCNTs by in situ growth for high-performance supercapacitor electrode materials |
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