Two-dimensional covalent organic frameworks for electrocatalysis: Achievements, challenges, and opportunities

Covalent organic frameworks (COFs) represent an emerging class of crystalline porous polymers with high porosity, good stability, and adjustable structure, and their excellent characteristics lay a solid foundation for electrocatalysis. This review systematically introduces the design principles of...

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Veröffentlicht in:Nano research 2023-07, Vol.16 (7), p.8570-8595
Hauptverfasser: Zhao, Ruoyu, Wang, Teng, Li, Junjun, Shi, Yongxia, Hou, Man, Yang, Yong, Zhang, Zhicheng, Lei, Shengbin
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container_end_page 8595
container_issue 7
container_start_page 8570
container_title Nano research
container_volume 16
creator Zhao, Ruoyu
Wang, Teng
Li, Junjun
Shi, Yongxia
Hou, Man
Yang, Yong
Zhang, Zhicheng
Lei, Shengbin
description Covalent organic frameworks (COFs) represent an emerging class of crystalline porous polymers with high porosity, good stability, and adjustable structure, and their excellent characteristics lay a solid foundation for electrocatalysis. This review systematically introduces the design principles of the catalytic sites in two-dimensional (2D) COF-based electrocatalysts and analyzes the relationship between 2D COF structure and their electrocatalytic performances. In particular, the recent progress in the field of 2D COFs as electrocatalysts is comprehensively summarized. Finally, we discuss the current shortcomings and challenges on tailoring 2D COF for high-performance electrocatalysts in details, and look forward to promoting more researches on 2D COF-based electrocatalysts.
doi_str_mv 10.1007/s12274-022-5307-1
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subjects Accelerating clean energy innovations via nanotechnology toward achieving circular economy
Active sites
Atomic/Molecular Structure and Spectra
Biomedicine
Biotechnology
Carbon dioxide
Catalysis
Chemistry and Materials Science
Composite materials
Condensed Matter Physics
Electrocatalysis
Electrocatalysts
Energy
Fuel cells
Graphene
Materials Science
Nanotechnology
Nitrogen
Polymers
Porosity
Review Article
Two dimensional analysis
title Two-dimensional covalent organic frameworks for electrocatalysis: Achievements, challenges, and opportunities
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