A-site stoichiometry and piezoelectric response in thin film PbZr1−xTixO3
Lead zirconate titanate (PZT) films with Zr/Ti ratios of 52/48 and 30/70 annealed at varying partial pressures of PbO within the perovskite phase field exhibited permittivities of 1150 and 600, respectively, with loss tangents of 0.02. Many of the functional properties, including the permittivity, p...
Gespeichert in:
| Veröffentlicht in: | Journal of applied physics 2015-05, Vol.117 (20), p.204104 |
|---|---|
| Hauptverfasser: | , , , , , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | |
|---|---|
| container_issue | 20 |
| container_start_page | 204104 |
| container_title | Journal of applied physics |
| container_volume | 117 |
| creator | Marincel, D. M. Jesse, S. Belianinov, A. Okatan, M. B. Kalinin, S. V. Jackson, T. N. Randall, C. A. Trolier-McKinstry, S. |
| description | Lead zirconate titanate
(PZT)
films with Zr/Ti ratios of 52/48 and 30/70 annealed at varying partial pressures of PbO within the perovskite phase field exhibited permittivities of 1150 and 600, respectively, with loss tangents of 0.02. Many of the functional properties, including the permittivity, piezoelectricity as indicated via the Rayleigh coefficients, and the aging rates were found to be weakly dependent of the lead content in the single phase field. Minor polarization–electric field hysteresis loops and piezoelectric coefficient e31,f values after a hot poling process suggest that the point defect helps stabilize the aligned domain states. Measurements of the local nonlinear response show an increased low response cluster size with decreasing PbO content, indicating that PbO deficiency acts to reduce domain wall motion where it is already low. |
| doi_str_mv | 10.1063/1.4921869 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_scita</sourceid><recordid>TN_cdi_proquest_journals_2845314529</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2845314529</sourcerecordid><originalsourceid>FETCH-LOGICAL-c389t-7ffd37ad37209963a706dd7510eebd69e4ce5e192f7d3e120ee98a8a9a23f3c53</originalsourceid><addsrcrecordid>eNp90M1KAzEQB_AgCtbqwTdY9KSwNR-b3eRYxC8s1EO9eAlpNqEp7WZNUml9As8-ok9iyhY9CB4ygeHHzJ8B4BTBAYIluUKDgmPESr4HeggynleUwn3QgxCjnPGKH4KjEOYQIsQI74HHYR5s1FmIzqqZdUsd_SaTTZ21Vr87vdAqeqsyr0PrmqAz22Rxloqxi2X2NH3x6Ovjcz2x6zE5BgdGLoI-2f198Hx7M7m-z0fju4fr4ShXhPGYV8bUpJLpYch5SWQFy7quKIJaT-uS60JpqhHHpqqJRji1OZNMcomJIYqSPjjr5roQrQgq5Vcz5ZomZRUIl7SiLKHzDrXeva50iGLuVr5JuQRmBSWooJgnddEp5V0IXhvReruUfiMQFNuDCiR2B032srPbjTJa1_zgN-d_oWhr8x_-O_kbkXuEJQ</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2845314529</pqid></control><display><type>article</type><title>A-site stoichiometry and piezoelectric response in thin film PbZr1−xTixO3</title><source>AIP Journals Complete</source><source>Alma/SFX Local Collection</source><creator>Marincel, D. M. ; Jesse, S. ; Belianinov, A. ; Okatan, M. B. ; Kalinin, S. V. ; Jackson, T. N. ; Randall, C. A. ; Trolier-McKinstry, S.</creator><creatorcontrib>Marincel, D. M. ; Jesse, S. ; Belianinov, A. ; Okatan, M. B. ; Kalinin, S. V. ; Jackson, T. N. ; Randall, C. A. ; Trolier-McKinstry, S. ; Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)</creatorcontrib><description>Lead zirconate titanate
(PZT)
films with Zr/Ti ratios of 52/48 and 30/70 annealed at varying partial pressures of PbO within the perovskite phase field exhibited permittivities of 1150 and 600, respectively, with loss tangents of 0.02. Many of the functional properties, including the permittivity, piezoelectricity as indicated via the Rayleigh coefficients, and the aging rates were found to be weakly dependent of the lead content in the single phase field. Minor polarization–electric field hysteresis loops and piezoelectric coefficient e31,f values after a hot poling process suggest that the point defect helps stabilize the aligned domain states. Measurements of the local nonlinear response show an increased low response cluster size with decreasing PbO content, indicating that PbO deficiency acts to reduce domain wall motion where it is already low.</description><identifier>ISSN: 0021-8979</identifier><identifier>EISSN: 1089-7550</identifier><identifier>DOI: 10.1063/1.4921869</identifier><identifier>CODEN: JAPIAU</identifier><language>eng</language><publisher>Melville: American Institute of Physics</publisher><subject>Applied physics ; Domain walls ; Furnaces ; Hysteresis loops ; Lead ; Lead oxides ; Lead zirconate titanate ; MATERIALS SCIENCE ; Nonlinear response ; Piezoelectricity ; Point defects ; Polarization ; Stoichiometry ; Tangents ; Zirconium</subject><ispartof>Journal of applied physics, 2015-05, Vol.117 (20), p.204104</ispartof><rights>AIP Publishing LLC</rights><rights>2015 AIP Publishing LLC.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c389t-7ffd37ad37209963a706dd7510eebd69e4ce5e192f7d3e120ee98a8a9a23f3c53</citedby><cites>FETCH-LOGICAL-c389t-7ffd37ad37209963a706dd7510eebd69e4ce5e192f7d3e120ee98a8a9a23f3c53</cites><orcidid>0000-0001-5354-6152</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://pubs.aip.org/jap/article-lookup/doi/10.1063/1.4921869$$EHTML$$P50$$Gscitation$$H</linktohtml><link.rule.ids>230,314,777,781,791,882,4498,27905,27906,76133</link.rule.ids><backlink>$$Uhttps://www.osti.gov/servlets/purl/1265758$$D View this record in Osti.gov$$Hfree_for_read</backlink></links><search><creatorcontrib>Marincel, D. M.</creatorcontrib><creatorcontrib>Jesse, S.</creatorcontrib><creatorcontrib>Belianinov, A.</creatorcontrib><creatorcontrib>Okatan, M. B.</creatorcontrib><creatorcontrib>Kalinin, S. V.</creatorcontrib><creatorcontrib>Jackson, T. N.</creatorcontrib><creatorcontrib>Randall, C. A.</creatorcontrib><creatorcontrib>Trolier-McKinstry, S.</creatorcontrib><creatorcontrib>Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)</creatorcontrib><title>A-site stoichiometry and piezoelectric response in thin film PbZr1−xTixO3</title><title>Journal of applied physics</title><description>Lead zirconate titanate
(PZT)
films with Zr/Ti ratios of 52/48 and 30/70 annealed at varying partial pressures of PbO within the perovskite phase field exhibited permittivities of 1150 and 600, respectively, with loss tangents of 0.02. Many of the functional properties, including the permittivity, piezoelectricity as indicated via the Rayleigh coefficients, and the aging rates were found to be weakly dependent of the lead content in the single phase field. Minor polarization–electric field hysteresis loops and piezoelectric coefficient e31,f values after a hot poling process suggest that the point defect helps stabilize the aligned domain states. Measurements of the local nonlinear response show an increased low response cluster size with decreasing PbO content, indicating that PbO deficiency acts to reduce domain wall motion where it is already low.</description><subject>Applied physics</subject><subject>Domain walls</subject><subject>Furnaces</subject><subject>Hysteresis loops</subject><subject>Lead</subject><subject>Lead oxides</subject><subject>Lead zirconate titanate</subject><subject>MATERIALS SCIENCE</subject><subject>Nonlinear response</subject><subject>Piezoelectricity</subject><subject>Point defects</subject><subject>Polarization</subject><subject>Stoichiometry</subject><subject>Tangents</subject><subject>Zirconium</subject><issn>0021-8979</issn><issn>1089-7550</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNp90M1KAzEQB_AgCtbqwTdY9KSwNR-b3eRYxC8s1EO9eAlpNqEp7WZNUml9As8-ok9iyhY9CB4ygeHHzJ8B4BTBAYIluUKDgmPESr4HeggynleUwn3QgxCjnPGKH4KjEOYQIsQI74HHYR5s1FmIzqqZdUsd_SaTTZ21Vr87vdAqeqsyr0PrmqAz22Rxloqxi2X2NH3x6Ovjcz2x6zE5BgdGLoI-2f198Hx7M7m-z0fju4fr4ShXhPGYV8bUpJLpYch5SWQFy7quKIJaT-uS60JpqhHHpqqJRji1OZNMcomJIYqSPjjr5roQrQgq5Vcz5ZomZRUIl7SiLKHzDrXeva50iGLuVr5JuQRmBSWooJgnddEp5V0IXhvReruUfiMQFNuDCiR2B032srPbjTJa1_zgN-d_oWhr8x_-O_kbkXuEJQ</recordid><startdate>20150528</startdate><enddate>20150528</enddate><creator>Marincel, D. M.</creator><creator>Jesse, S.</creator><creator>Belianinov, A.</creator><creator>Okatan, M. B.</creator><creator>Kalinin, S. V.</creator><creator>Jackson, T. N.</creator><creator>Randall, C. A.</creator><creator>Trolier-McKinstry, S.</creator><general>American Institute of Physics</general><general>American Institute of Physics (AIP)</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope><scope>OIOZB</scope><scope>OTOTI</scope><orcidid>https://orcid.org/0000-0001-5354-6152</orcidid></search><sort><creationdate>20150528</creationdate><title>A-site stoichiometry and piezoelectric response in thin film PbZr1−xTixO3</title><author>Marincel, D. M. ; Jesse, S. ; Belianinov, A. ; Okatan, M. B. ; Kalinin, S. V. ; Jackson, T. N. ; Randall, C. A. ; Trolier-McKinstry, S.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c389t-7ffd37ad37209963a706dd7510eebd69e4ce5e192f7d3e120ee98a8a9a23f3c53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>Applied physics</topic><topic>Domain walls</topic><topic>Furnaces</topic><topic>Hysteresis loops</topic><topic>Lead</topic><topic>Lead oxides</topic><topic>Lead zirconate titanate</topic><topic>MATERIALS SCIENCE</topic><topic>Nonlinear response</topic><topic>Piezoelectricity</topic><topic>Point defects</topic><topic>Polarization</topic><topic>Stoichiometry</topic><topic>Tangents</topic><topic>Zirconium</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Marincel, D. M.</creatorcontrib><creatorcontrib>Jesse, S.</creatorcontrib><creatorcontrib>Belianinov, A.</creatorcontrib><creatorcontrib>Okatan, M. B.</creatorcontrib><creatorcontrib>Kalinin, S. V.</creatorcontrib><creatorcontrib>Jackson, T. N.</creatorcontrib><creatorcontrib>Randall, C. A.</creatorcontrib><creatorcontrib>Trolier-McKinstry, S.</creatorcontrib><creatorcontrib>Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)</creatorcontrib><collection>CrossRef</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>OSTI.GOV - Hybrid</collection><collection>OSTI.GOV</collection><jtitle>Journal of applied physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Marincel, D. M.</au><au>Jesse, S.</au><au>Belianinov, A.</au><au>Okatan, M. B.</au><au>Kalinin, S. V.</au><au>Jackson, T. N.</au><au>Randall, C. A.</au><au>Trolier-McKinstry, S.</au><aucorp>Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>A-site stoichiometry and piezoelectric response in thin film PbZr1−xTixO3</atitle><jtitle>Journal of applied physics</jtitle><date>2015-05-28</date><risdate>2015</risdate><volume>117</volume><issue>20</issue><spage>204104</spage><pages>204104-</pages><issn>0021-8979</issn><eissn>1089-7550</eissn><coden>JAPIAU</coden><abstract>Lead zirconate titanate
(PZT)
films with Zr/Ti ratios of 52/48 and 30/70 annealed at varying partial pressures of PbO within the perovskite phase field exhibited permittivities of 1150 and 600, respectively, with loss tangents of 0.02. Many of the functional properties, including the permittivity, piezoelectricity as indicated via the Rayleigh coefficients, and the aging rates were found to be weakly dependent of the lead content in the single phase field. Minor polarization–electric field hysteresis loops and piezoelectric coefficient e31,f values after a hot poling process suggest that the point defect helps stabilize the aligned domain states. Measurements of the local nonlinear response show an increased low response cluster size with decreasing PbO content, indicating that PbO deficiency acts to reduce domain wall motion where it is already low.</abstract><cop>Melville</cop><pub>American Institute of Physics</pub><doi>10.1063/1.4921869</doi><tpages>8</tpages><orcidid>https://orcid.org/0000-0001-5354-6152</orcidid><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0021-8979 |
| ispartof | Journal of applied physics, 2015-05, Vol.117 (20), p.204104 |
| issn | 0021-8979 1089-7550 |
| language | eng |
| recordid | cdi_proquest_journals_2845314529 |
| source | AIP Journals Complete; Alma/SFX Local Collection |
| subjects | Applied physics Domain walls Furnaces Hysteresis loops Lead Lead oxides Lead zirconate titanate MATERIALS SCIENCE Nonlinear response Piezoelectricity Point defects Polarization Stoichiometry Tangents Zirconium |
| title | A-site stoichiometry and piezoelectric response in thin film PbZr1−xTixO3 |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-18T20%3A03%3A15IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_scita&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=A-site%20stoichiometry%20and%20piezoelectric%20response%20in%20thin%20film%20PbZr1%E2%88%92xTixO3&rft.jtitle=Journal%20of%20applied%20physics&rft.au=Marincel,%20D.%20M.&rft.aucorp=Oak%20Ridge%20National%20Lab.%20(ORNL),%20Oak%20Ridge,%20TN%20(United%20States).%20Center%20for%20Nanophase%20Materials%20Sciences%20(CNMS)&rft.date=2015-05-28&rft.volume=117&rft.issue=20&rft.spage=204104&rft.pages=204104-&rft.issn=0021-8979&rft.eissn=1089-7550&rft.coden=JAPIAU&rft_id=info:doi/10.1063/1.4921869&rft_dat=%3Cproquest_scita%3E2845314529%3C/proquest_scita%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2845314529&rft_id=info:pmid/&rfr_iscdi=true |