Construction and performance of composite nanoporous PVDF membrane loaded with TiO2-based catalysts for organic pollutants’ removal
Membrane separation is one of the most effective ways to remove organic dyes in wastewater. Rationally regulating the pore size of separation membranes would contribute to great performance. However, membranes with a uniform pore structure make it difficult to simultaneously realize high flux and ex...
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| Veröffentlicht in: | Journal of materials science 2023-07, Vol.58 (28), p.11631-11646 |
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| creator | Li, Peihang Ran, Hongshun Pan, Yaoyu Xu, Ziqiang Chen, Xueqin Li, Cao Jiang, Bingbing |
| description | Membrane separation is one of the most effective ways to remove organic dyes in wastewater. Rationally regulating the pore size of separation membranes would contribute to great performance. However, membranes with a uniform pore structure make it difficult to simultaneously realize high flux and excellent rejection ratio. Herein, functional composite nanoporous fiber membrane material with visible-light-driven self-cleaning performance was constructed by spinning hypercrosslinked polystyrene nanoparticles (HCPNPs) and TiO
2
-based catalysts into the electrospun membrane of polyvinylidene fluoride (PVDF). The composited fiber membrane with a hierarchical pore structure exhibits unique performances: excellent adsorption capacity for organic dyes, reaching 12 mg·g
−1
(methylene blue), respectively, extraordinary high photocatalytic degradation rate (up to 99%) and gorgeous cycle degradation performance for MB (degradation rate is maintained at 95% after five cycles), and excellent comprehensive performance for the removal of extensive pollutant library including organic dye, and antibiotic pollutant. Therefore, coupled with facile and economical synthesis, we provide a novel idea for advanced membrane construction, which has the potential to be widely used for organic pollutants’ removal in sewage treatment.
Graphical abstract |
| doi_str_mv | 10.1007/s10853-023-08738-3 |
| format | Article |
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2
-based catalysts into the electrospun membrane of polyvinylidene fluoride (PVDF). The composited fiber membrane with a hierarchical pore structure exhibits unique performances: excellent adsorption capacity for organic dyes, reaching 12 mg·g
−1
(methylene blue), respectively, extraordinary high photocatalytic degradation rate (up to 99%) and gorgeous cycle degradation performance for MB (degradation rate is maintained at 95% after five cycles), and excellent comprehensive performance for the removal of extensive pollutant library including organic dye, and antibiotic pollutant. Therefore, coupled with facile and economical synthesis, we provide a novel idea for advanced membrane construction, which has the potential to be widely used for organic pollutants’ removal in sewage treatment.
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2
-based catalysts into the electrospun membrane of polyvinylidene fluoride (PVDF). The composited fiber membrane with a hierarchical pore structure exhibits unique performances: excellent adsorption capacity for organic dyes, reaching 12 mg·g
−1
(methylene blue), respectively, extraordinary high photocatalytic degradation rate (up to 99%) and gorgeous cycle degradation performance for MB (degradation rate is maintained at 95% after five cycles), and excellent comprehensive performance for the removal of extensive pollutant library including organic dye, and antibiotic pollutant. Therefore, coupled with facile and economical synthesis, we provide a novel idea for advanced membrane construction, which has the potential to be widely used for organic pollutants’ removal in sewage treatment.
Graphical abstract</description><subject>Catalysts</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Classical Mechanics</subject><subject>Composites & Nanocomposites</subject><subject>Crystallography and Scattering Methods</subject><subject>Dyes</subject><subject>Electrospinning</subject><subject>Materials Science</subject><subject>Membrane separation</subject><subject>Membranes</subject><subject>Methylene blue</subject><subject>Nanoparticles</subject><subject>Performance degradation</subject><subject>Photodegradation</subject><subject>Pollutants</subject><subject>Polymer Sciences</subject><subject>Polystyrene resins</subject><subject>Polyvinylidene fluorides</subject><subject>Pore size</subject><subject>Separation</subject><subject>Solid Mechanics</subject><subject>Titanium dioxide</subject><subject>Wastewater</subject><issn>0022-2461</issn><issn>1573-4803</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp9kM1KxDAURoMoOI6-gKuA62r-2qZLGR0VBsbF6DbcpunYoU1qkiqzc-ND-Ho-idUR3Lm4XC6c77twEDql5JwSkl8ESmTKE8LGkTmXCd9DE5rmPBGS8H00IYSxhImMHqKjEDaEkDRndILeZ86G6AcdG2cx2Ar3xtfOd2C1wa7G2nW9C0002IJ1vfNuCPj-8WqOO9OVHqzBrYPKVPi1iU941SxZUkIYbw0R2m2IAY992Pk12Ebj3rXtEMHG8Pn2gb3p3Au0x-ighjaYk989RQ_z69XsNlksb-5ml4tEc1rEBJgsBGMFZ7QyoiKClamoMqjLjBGouBBSUpPSklYgykxDKYwuTMrrVDBSZHyKzna9vXfPgwlRbdzg7fhSMSmIzCSVcqTYjtLeheBNrXrfdOC3ihL1rVvtdKtRt_rRrfgY4rtQGGG7Nv6v-p_UF3fEheQ</recordid><startdate>20230701</startdate><enddate>20230701</enddate><creator>Li, Peihang</creator><creator>Ran, Hongshun</creator><creator>Pan, Yaoyu</creator><creator>Xu, Ziqiang</creator><creator>Chen, Xueqin</creator><creator>Li, Cao</creator><creator>Jiang, Bingbing</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>L6V</scope><scope>M7S</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PTHSS</scope><orcidid>https://orcid.org/0000-0001-5750-2819</orcidid><orcidid>https://orcid.org/0000-0003-4349-7478</orcidid></search><sort><creationdate>20230701</creationdate><title>Construction and performance of composite nanoporous PVDF membrane loaded with TiO2-based catalysts for organic pollutants’ removal</title><author>Li, Peihang ; Ran, Hongshun ; Pan, Yaoyu ; Xu, Ziqiang ; Chen, Xueqin ; Li, Cao ; Jiang, Bingbing</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-a2894229321de4d042b54d6afb620ad344881e51b1da4b6cab4ec9e53f5420963</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Catalysts</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Classical Mechanics</topic><topic>Composites & Nanocomposites</topic><topic>Crystallography and Scattering Methods</topic><topic>Dyes</topic><topic>Electrospinning</topic><topic>Materials Science</topic><topic>Membrane separation</topic><topic>Membranes</topic><topic>Methylene blue</topic><topic>Nanoparticles</topic><topic>Performance degradation</topic><topic>Photodegradation</topic><topic>Pollutants</topic><topic>Polymer Sciences</topic><topic>Polystyrene resins</topic><topic>Polyvinylidene fluorides</topic><topic>Pore size</topic><topic>Separation</topic><topic>Solid Mechanics</topic><topic>Titanium dioxide</topic><topic>Wastewater</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Peihang</creatorcontrib><creatorcontrib>Ran, Hongshun</creatorcontrib><creatorcontrib>Pan, Yaoyu</creatorcontrib><creatorcontrib>Xu, Ziqiang</creatorcontrib><creatorcontrib>Chen, Xueqin</creatorcontrib><creatorcontrib>Li, Cao</creatorcontrib><creatorcontrib>Jiang, Bingbing</creatorcontrib><collection>CrossRef</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Engineering Collection</collection><jtitle>Journal of materials science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Peihang</au><au>Ran, Hongshun</au><au>Pan, Yaoyu</au><au>Xu, Ziqiang</au><au>Chen, Xueqin</au><au>Li, Cao</au><au>Jiang, Bingbing</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Construction and performance of composite nanoporous PVDF membrane loaded with TiO2-based catalysts for organic pollutants’ removal</atitle><jtitle>Journal of materials science</jtitle><stitle>J Mater Sci</stitle><date>2023-07-01</date><risdate>2023</risdate><volume>58</volume><issue>28</issue><spage>11631</spage><epage>11646</epage><pages>11631-11646</pages><issn>0022-2461</issn><eissn>1573-4803</eissn><abstract>Membrane separation is one of the most effective ways to remove organic dyes in wastewater. Rationally regulating the pore size of separation membranes would contribute to great performance. However, membranes with a uniform pore structure make it difficult to simultaneously realize high flux and excellent rejection ratio. Herein, functional composite nanoporous fiber membrane material with visible-light-driven self-cleaning performance was constructed by spinning hypercrosslinked polystyrene nanoparticles (HCPNPs) and TiO
2
-based catalysts into the electrospun membrane of polyvinylidene fluoride (PVDF). The composited fiber membrane with a hierarchical pore structure exhibits unique performances: excellent adsorption capacity for organic dyes, reaching 12 mg·g
−1
(methylene blue), respectively, extraordinary high photocatalytic degradation rate (up to 99%) and gorgeous cycle degradation performance for MB (degradation rate is maintained at 95% after five cycles), and excellent comprehensive performance for the removal of extensive pollutant library including organic dye, and antibiotic pollutant. Therefore, coupled with facile and economical synthesis, we provide a novel idea for advanced membrane construction, which has the potential to be widely used for organic pollutants’ removal in sewage treatment.
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| subjects | Catalysts Characterization and Evaluation of Materials Chemistry and Materials Science Classical Mechanics Composites & Nanocomposites Crystallography and Scattering Methods Dyes Electrospinning Materials Science Membrane separation Membranes Methylene blue Nanoparticles Performance degradation Photodegradation Pollutants Polymer Sciences Polystyrene resins Polyvinylidene fluorides Pore size Separation Solid Mechanics Titanium dioxide Wastewater |
| title | Construction and performance of composite nanoporous PVDF membrane loaded with TiO2-based catalysts for organic pollutants’ removal |
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