$Synthesis and physical properties of Ce$_2$Rh$_{3+\delta}$Sb$_4$ single crystals$

Synthesis and physical properties of Ce$_2$Rh$_{3+\delta}$Sb$_4$ single crystals

Millimeter-sized Ce$_2$Rh$_{3+\delta}$Sb$_4$ ($\delta\approx 1/8$) single crystals were synthesized by a Bi-flux method and their physical properties were studied by a combination of electrical transport, magnetic and thermodynamic measurements. The resistivity anisotropy \(\rho_{a,b}/\rho_{...

Ausführliche Beschreibung

Gespeichert in:

Bibliographische Detailangaben
Veröffentlicht in:	arXiv.org 2023-08
Hauptverfasser:	Cheng, Kangqiao, Zou, Shuo, Bu, Huanpeng, Zhang, Jiawen, Song, Shijie, Guo, Hanjie, Yuan, Huiqiu, Luo, Yongkang
Format:	Artikel
Sprache:	eng
Schlagworte:	Anisotropy Antiferromagnetism Magnetic permeability Magnetic properties Physical properties Single crystals
Online-Zugang:	Volltext
Tags:	Tag hinzufügen Keine Tags, Fügen Sie den ersten Tag hinzu!

container_end_page
container_issue
container_start_page
container_title	arXiv.org
container_volume
creator	Cheng, Kangqiao Zou, Shuo Bu, Huanpeng Zhang, Jiawen Song, Shijie Guo, Hanjie Yuan, Huiqiu Luo, Yongkang
description	Millimeter-sized Ce$_2$Rh$_{3+\delta}$Sb$_4$ ($\delta\approx 1/8$) single crystals were synthesized by a Bi-flux method and their physical properties were studied by a combination of electrical transport, magnetic and thermodynamic measurements. The resistivity anisotropy $\rho_{a,b}/\rho_{c}\sim2$, manifesting a quasi-one-dimensional electronic character. Magnetic susceptibility measurements confirm $\mathbf{ab}$ as the magnetic easy plane. A long-range antiferromagnetic transition occurs at $T_N=1.4$ K, while clear short-range ordering can be detected well above $T_N$. The low ordering temperature is ascribed to the large Ce-Ce distance as well as the geometric frustration. Kondo scale is estimated to be about 2.4 K, comparable to the strength of magnetic exchange. Ce$_2$Rh$_{3+\delta}$Sb$_4$, therefore, represents a rare example of dense Kondo lattice whose Ruderman-Kittel-Kasuya-Yosida exchange and Kondo coupling are both weak but competing.
doi_str_mv	10.48550/arxiv.2305.08669
format	Article
fullrecord	<record><control><sourceid>proquest</sourceid><recordid>TN_cdi_proquest_journals_2814210554</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2814210554</sourcerecordid><originalsourceid>FETCH-proquest_journals_28142105543</originalsourceid><addsrcrecordid>eNqNzEFrgzAcBfAwGEy2foDdArtUSl38J3HuXFp6bsdOAck0zoiozT-Wyth3bw79AD394L3HI-Q1ZYnIpWTv2l3sOQHOZMLyLPt8IBFwnq5zAfBEFogtYwyyD5CSR-T7OPe-MWiR6r6iYzOjLXVHRzeMxnlrkA413Ri1LEDFhyb4x1eqMp3X_yo-_oRAqJii7X87Q0s3o9cdvpDHOmAWN5_J2277tdmvw-9pMuiLdphcH6oC8lRAyqQU_L7VFeDZRhk</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2814210554</pqid></control><display><type>article</type><title>Synthesis and physical properties of Ce$_2$Rh$_{3+\delta}$Sb$_4$ single crystals</title><source>Free E- Journals</source><creator>Cheng, Kangqiao ; Zou, Shuo ; Bu, Huanpeng ; Zhang, Jiawen ; Song, Shijie ; Guo, Hanjie ; Yuan, Huiqiu ; Luo, Yongkang</creator><creatorcontrib>Cheng, Kangqiao ; Zou, Shuo ; Bu, Huanpeng ; Zhang, Jiawen ; Song, Shijie ; Guo, Hanjie ; Yuan, Huiqiu ; Luo, Yongkang</creatorcontrib><description>Millimeter-sized Ce$_2$Rh$_{3+\delta}$Sb$_4$ ($\delta\approx 1/8$) single crystals were synthesized by a Bi-flux method and their physical properties were studied by a combination of electrical transport, magnetic and thermodynamic measurements. The resistivity anisotropy $\rho_{a,b}/\rho_{c}\sim2$, manifesting a quasi-one-dimensional electronic character. Magnetic susceptibility measurements confirm $\mathbf{ab}$ as the magnetic easy plane. A long-range antiferromagnetic transition occurs at $T_N=1.4$ K, while clear short-range ordering can be detected well above $T_N$. The low ordering temperature is ascribed to the large Ce-Ce distance as well as the geometric frustration. Kondo scale is estimated to be about 2.4 K, comparable to the strength of magnetic exchange. Ce$_2$Rh$_{3+\delta}$Sb$_4$, therefore, represents a rare example of dense Kondo lattice whose Ruderman-Kittel-Kasuya-Yosida exchange and Kondo coupling are both weak but competing.</description><identifier>EISSN: 2331-8422</identifier><identifier>DOI: 10.48550/arxiv.2305.08669</identifier><language>eng</language><publisher>Ithaca: Cornell University Library, arXiv.org</publisher><subject>Anisotropy ; Antiferromagnetism ; Magnetic permeability ; Magnetic properties ; Physical properties ; Single crystals</subject><ispartof>arXiv.org, 2023-08</ispartof><rights>2023. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>776,780,27904</link.rule.ids></links><search><creatorcontrib>Cheng, Kangqiao</creatorcontrib><creatorcontrib>Zou, Shuo</creatorcontrib><creatorcontrib>Bu, Huanpeng</creatorcontrib><creatorcontrib>Zhang, Jiawen</creatorcontrib><creatorcontrib>Song, Shijie</creatorcontrib><creatorcontrib>Guo, Hanjie</creatorcontrib><creatorcontrib>Yuan, Huiqiu</creatorcontrib><creatorcontrib>Luo, Yongkang</creatorcontrib><title>Synthesis and physical properties of Ce$_2$Rh$_{3+\delta}$Sb$_4$ single crystals</title><title>arXiv.org</title><description>Millimeter-sized Ce$_2$Rh$_{3+\delta}$Sb$_4$ ($\delta\approx 1/8$) single crystals were synthesized by a Bi-flux method and their physical properties were studied by a combination of electrical transport, magnetic and thermodynamic measurements. The resistivity anisotropy $\rho_{a,b}/\rho_{c}\sim2$, manifesting a quasi-one-dimensional electronic character. Magnetic susceptibility measurements confirm $\mathbf{ab}$ as the magnetic easy plane. A long-range antiferromagnetic transition occurs at $T_N=1.4$ K, while clear short-range ordering can be detected well above $T_N$. The low ordering temperature is ascribed to the large Ce-Ce distance as well as the geometric frustration. Kondo scale is estimated to be about 2.4 K, comparable to the strength of magnetic exchange. Ce$_2$Rh$_{3+\delta}$Sb$_4$, therefore, represents a rare example of dense Kondo lattice whose Ruderman-Kittel-Kasuya-Yosida exchange and Kondo coupling are both weak but competing.</description><subject>Anisotropy</subject><subject>Antiferromagnetism</subject><subject>Magnetic permeability</subject><subject>Magnetic properties</subject><subject>Physical properties</subject><subject>Single crystals</subject><issn>2331-8422</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNqNzEFrgzAcBfAwGEy2foDdArtUSl38J3HuXFp6bsdOAck0zoiozT-Wyth3bw79AD394L3HI-Q1ZYnIpWTv2l3sOQHOZMLyLPt8IBFwnq5zAfBEFogtYwyyD5CSR-T7OPe-MWiR6r6iYzOjLXVHRzeMxnlrkA413Ri1LEDFhyb4x1eqMp3X_yo-_oRAqJii7X87Q0s3o9cdvpDHOmAWN5_J2277tdmvw-9pMuiLdphcH6oC8lRAyqQU_L7VFeDZRhk</recordid><startdate>20230816</startdate><enddate>20230816</enddate><creator>Cheng, Kangqiao</creator><creator>Zou, Shuo</creator><creator>Bu, Huanpeng</creator><creator>Zhang, Jiawen</creator><creator>Song, Shijie</creator><creator>Guo, Hanjie</creator><creator>Yuan, Huiqiu</creator><creator>Luo, Yongkang</creator><general>Cornell University Library, arXiv.org</general><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>HCIFZ</scope><scope>L6V</scope><scope>M7S</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PTHSS</scope></search><sort><creationdate>20230816</creationdate><title>Synthesis and physical properties of Ce$_2$Rh$_{3+\delta}$Sb$_4$ single crystals</title><author>Cheng, Kangqiao ; Zou, Shuo ; Bu, Huanpeng ; Zhang, Jiawen ; Song, Shijie ; Guo, Hanjie ; Yuan, Huiqiu ; Luo, Yongkang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-proquest_journals_28142105543</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Anisotropy</topic><topic>Antiferromagnetism</topic><topic>Magnetic permeability</topic><topic>Magnetic properties</topic><topic>Physical properties</topic><topic>Single crystals</topic><toplevel>online_resources</toplevel><creatorcontrib>Cheng, Kangqiao</creatorcontrib><creatorcontrib>Zou, Shuo</creatorcontrib><creatorcontrib>Bu, Huanpeng</creatorcontrib><creatorcontrib>Zhang, Jiawen</creatorcontrib><creatorcontrib>Song, Shijie</creatorcontrib><creatorcontrib>Guo, Hanjie</creatorcontrib><creatorcontrib>Yuan, Huiqiu</creatorcontrib><creatorcontrib>Luo, Yongkang</creatorcontrib><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Engineering Collection</collection><collection>Engineering Database</collection><collection>Publicly Available Content Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Engineering Collection</collection></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Cheng, Kangqiao</au><au>Zou, Shuo</au><au>Bu, Huanpeng</au><au>Zhang, Jiawen</au><au>Song, Shijie</au><au>Guo, Hanjie</au><au>Yuan, Huiqiu</au><au>Luo, Yongkang</au><format>book</format><genre>document</genre><ristype>GEN</ristype><atitle>Synthesis and physical properties of Ce$_2$Rh$_{3+\delta}$Sb$_4$ single crystals</atitle><jtitle>arXiv.org</jtitle><date>2023-08-16</date><risdate>2023</risdate><eissn>2331-8422</eissn><abstract>Millimeter-sized Ce$_2$Rh$_{3+\delta}$Sb$_4$ ($\delta\approx 1/8$) single crystals were synthesized by a Bi-flux method and their physical properties were studied by a combination of electrical transport, magnetic and thermodynamic measurements. The resistivity anisotropy $\rho_{a,b}/\rho_{c}\sim2$, manifesting a quasi-one-dimensional electronic character. Magnetic susceptibility measurements confirm $\mathbf{ab}$ as the magnetic easy plane. A long-range antiferromagnetic transition occurs at $T_N=1.4$ K, while clear short-range ordering can be detected well above $T_N$. The low ordering temperature is ascribed to the large Ce-Ce distance as well as the geometric frustration. Kondo scale is estimated to be about 2.4 K, comparable to the strength of magnetic exchange. Ce$_2$Rh$_{3+\delta}$Sb$_4$, therefore, represents a rare example of dense Kondo lattice whose Ruderman-Kittel-Kasuya-Yosida exchange and Kondo coupling are both weak but competing.</abstract><cop>Ithaca</cop><pub>Cornell University Library, arXiv.org</pub><doi>10.48550/arxiv.2305.08669</doi><oa>free_for_read</oa></addata></record>
fulltext	fulltext
identifier	EISSN: 2331-8422
ispartof	arXiv.org, 2023-08
issn	2331-8422
language	eng
recordid	cdi_proquest_journals_2814210554
source	Free E- Journals
subjects	Anisotropy Antiferromagnetism Magnetic permeability Magnetic properties Physical properties Single crystals
title	Synthesis and physical properties of Ce$_2$Rh$_{3+\delta}$Sb$_4$ single crystals
url	https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-26T12%3A24%3A00IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest&rft_val_fmt=info:ofi/fmt:kev:mtx:book&rft.genre=document&rft.atitle=Synthesis%20and%20physical%20properties%20of%20Ce%5C(_2%5C)Rh%5C(_%7B3+%5Cdelta%7D%5C)Sb%5C(_4%5C)%20single%20crystals&rft.jtitle=arXiv.org&rft.au=Cheng,%20Kangqiao&rft.date=2023-08-16&rft.eissn=2331-8422&rft_id=info:doi/10.48550/arxiv.2305.08669&rft_dat=%3Cproquest%3E2814210554%3C/proquest%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2814210554&rft_id=info:pmid/&rfr_iscdi=true

Synthesis and physical properties of Ce\(_2\)Rh\(_{3+\delta}\)Sb\(_4\) single crystals