Fabrication of waste paper/graphene oxide three-dimensional aerogel with dual adsorption capacity toward methylene blue and ciprofloxacin
To effectively treat the pollutant in sewage, a new-type three-dimensional aerogel based on graphene oxide and waste paper was fabricated via simple mixing and freeze-drying processes. Therein, waste paper was activated in advance, and polyvinyl alcohol served as physical crosslinking agent. The res...
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Veröffentlicht in: | Journal of the Iranian Chemical Society 2023-04, Vol.20 (4), p.801-816 |
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creator | Yang, Fengjuan Zhang, Jinglin Lin, Tongyao Ke, Liying Huang, Langhuan Deng, Sui-Ping Zhang, Jingxian Tan, Shaozao Xiong, Yongqiang Lu, Ming |
description | To effectively treat the pollutant in sewage, a new-type three-dimensional aerogel based on graphene oxide and waste paper was fabricated via simple mixing and freeze-drying processes. Therein, waste paper was activated in advance, and polyvinyl alcohol served as physical crosslinking agent. The results showed that the obtained aerogel with porous three-dimensional network structure exhibited good thermal stability. When it acted as adsorbent for treating organic dye (methylene blue) and antibiotic (ciprofloxacin), the adsorption process was explored. In single system, the pseudo-first-order and pseudo-second-order kinetic models were used to discuss the detail about the aerogel adsorbing pollutant. Moreover, the Langmuir and Freundlich adsorption models were applied to describe the equilibrium isotherms and calculate the isotherm constants. Thermodynamic results stated that the adsorption of pollutant onto aerogel was feasible and spontaneous. In binary system, the adsorption capacity of methylene blue by aerogel increased, while the adsorption capacity of ciprofloxacin by aerogel declined. The pseudo-second-order kinetics was consistent with the adsorption of pollutant by aerogel in such binary system. This study would provide a new boulevard to develop environmental, low-cost and high-efficiency adsorbent for removing pollutant from wastewater.
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doi_str_mv | 10.1007/s13738-022-02714-5 |
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Graphical abstract</description><identifier>ISSN: 1735-207X</identifier><identifier>EISSN: 1735-2428</identifier><identifier>DOI: 10.1007/s13738-022-02714-5</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorbents ; Adsorption ; Aerogels ; Analytical Chemistry ; Binary system ; Biochemistry ; Chemistry ; Chemistry and Materials Science ; Crosslinking ; Graphene ; Inorganic Chemistry ; Isotherms ; Methylene blue ; Organic Chemistry ; Original Paper ; Physical Chemistry ; Pollutants ; Polyvinyl alcohol ; Thermal stability ; Wastewater treatment</subject><ispartof>Journal of the Iranian Chemical Society, 2023-04, Vol.20 (4), p.801-816</ispartof><rights>Iranian Chemical Society 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-513c7a6ece4db4220278a3f13603d712894f00fc5e10b64a5e4bae1b42731533</citedby><cites>FETCH-LOGICAL-c319t-513c7a6ece4db4220278a3f13603d712894f00fc5e10b64a5e4bae1b42731533</cites><orcidid>0000-0002-4669-0401</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s13738-022-02714-5$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s13738-022-02714-5$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Yang, Fengjuan</creatorcontrib><creatorcontrib>Zhang, Jinglin</creatorcontrib><creatorcontrib>Lin, Tongyao</creatorcontrib><creatorcontrib>Ke, Liying</creatorcontrib><creatorcontrib>Huang, Langhuan</creatorcontrib><creatorcontrib>Deng, Sui-Ping</creatorcontrib><creatorcontrib>Zhang, Jingxian</creatorcontrib><creatorcontrib>Tan, Shaozao</creatorcontrib><creatorcontrib>Xiong, Yongqiang</creatorcontrib><creatorcontrib>Lu, Ming</creatorcontrib><title>Fabrication of waste paper/graphene oxide three-dimensional aerogel with dual adsorption capacity toward methylene blue and ciprofloxacin</title><title>Journal of the Iranian Chemical Society</title><addtitle>J IRAN CHEM SOC</addtitle><description>To effectively treat the pollutant in sewage, a new-type three-dimensional aerogel based on graphene oxide and waste paper was fabricated via simple mixing and freeze-drying processes. Therein, waste paper was activated in advance, and polyvinyl alcohol served as physical crosslinking agent. The results showed that the obtained aerogel with porous three-dimensional network structure exhibited good thermal stability. When it acted as adsorbent for treating organic dye (methylene blue) and antibiotic (ciprofloxacin), the adsorption process was explored. In single system, the pseudo-first-order and pseudo-second-order kinetic models were used to discuss the detail about the aerogel adsorbing pollutant. Moreover, the Langmuir and Freundlich adsorption models were applied to describe the equilibrium isotherms and calculate the isotherm constants. Thermodynamic results stated that the adsorption of pollutant onto aerogel was feasible and spontaneous. In binary system, the adsorption capacity of methylene blue by aerogel increased, while the adsorption capacity of ciprofloxacin by aerogel declined. The pseudo-second-order kinetics was consistent with the adsorption of pollutant by aerogel in such binary system. This study would provide a new boulevard to develop environmental, low-cost and high-efficiency adsorbent for removing pollutant from wastewater.
Graphical abstract</description><subject>Adsorbents</subject><subject>Adsorption</subject><subject>Aerogels</subject><subject>Analytical Chemistry</subject><subject>Binary system</subject><subject>Biochemistry</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Crosslinking</subject><subject>Graphene</subject><subject>Inorganic Chemistry</subject><subject>Isotherms</subject><subject>Methylene blue</subject><subject>Organic Chemistry</subject><subject>Original Paper</subject><subject>Physical Chemistry</subject><subject>Pollutants</subject><subject>Polyvinyl alcohol</subject><subject>Thermal stability</subject><subject>Wastewater treatment</subject><issn>1735-207X</issn><issn>1735-2428</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNp9kM9Kw0AQxoMoWKsv4GnBc-z-yWbboxSrQsFLD96WyWbSpKTZuLul7SP41m5axZuHYYbh933DfElyz-gjo1RNPBNKTFPKeSzFslReJCOmhEx5xqeXvzNVH9fJjfcbSqWiMhslXwsoXGMgNLYjtiJ78AFJDz26ydpBX2OHxB6aEkmoHWJaNlvsfKShJYDOrrEl-ybUpNwNm9Jb15_MDPRgmnAkwe7BlWSLoT62g13R7pBAVxLT9M5WrT1EsLtNripoPd799HGyWjyv5q_p8v3lbf60TI1gs5BKJoyCHA1mZZFxHt-dgqiYyKkoFePTWVZRWhmJjBZ5BhKzApBFVAkmhRgnD2fbePpzhz7ojd25-I3XXM0UFSrnA8XPlHHWe4eV7l2zBXfUjOohcX1OXMfE9SlxLaNInEU-wt0a3Z_1P6pvR22Gng</recordid><startdate>20230401</startdate><enddate>20230401</enddate><creator>Yang, Fengjuan</creator><creator>Zhang, Jinglin</creator><creator>Lin, Tongyao</creator><creator>Ke, Liying</creator><creator>Huang, Langhuan</creator><creator>Deng, Sui-Ping</creator><creator>Zhang, Jingxian</creator><creator>Tan, Shaozao</creator><creator>Xiong, Yongqiang</creator><creator>Lu, Ming</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-4669-0401</orcidid></search><sort><creationdate>20230401</creationdate><title>Fabrication of waste paper/graphene oxide three-dimensional aerogel with dual adsorption capacity toward methylene blue and ciprofloxacin</title><author>Yang, Fengjuan ; Zhang, Jinglin ; Lin, Tongyao ; Ke, Liying ; Huang, Langhuan ; Deng, Sui-Ping ; Zhang, Jingxian ; Tan, Shaozao ; Xiong, Yongqiang ; Lu, Ming</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-513c7a6ece4db4220278a3f13603d712894f00fc5e10b64a5e4bae1b42731533</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Adsorbents</topic><topic>Adsorption</topic><topic>Aerogels</topic><topic>Analytical Chemistry</topic><topic>Binary system</topic><topic>Biochemistry</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Crosslinking</topic><topic>Graphene</topic><topic>Inorganic Chemistry</topic><topic>Isotherms</topic><topic>Methylene blue</topic><topic>Organic Chemistry</topic><topic>Original Paper</topic><topic>Physical Chemistry</topic><topic>Pollutants</topic><topic>Polyvinyl alcohol</topic><topic>Thermal stability</topic><topic>Wastewater treatment</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yang, Fengjuan</creatorcontrib><creatorcontrib>Zhang, Jinglin</creatorcontrib><creatorcontrib>Lin, Tongyao</creatorcontrib><creatorcontrib>Ke, Liying</creatorcontrib><creatorcontrib>Huang, Langhuan</creatorcontrib><creatorcontrib>Deng, Sui-Ping</creatorcontrib><creatorcontrib>Zhang, Jingxian</creatorcontrib><creatorcontrib>Tan, Shaozao</creatorcontrib><creatorcontrib>Xiong, Yongqiang</creatorcontrib><creatorcontrib>Lu, Ming</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of the Iranian Chemical Society</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yang, Fengjuan</au><au>Zhang, Jinglin</au><au>Lin, Tongyao</au><au>Ke, Liying</au><au>Huang, Langhuan</au><au>Deng, Sui-Ping</au><au>Zhang, Jingxian</au><au>Tan, Shaozao</au><au>Xiong, Yongqiang</au><au>Lu, Ming</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Fabrication of waste paper/graphene oxide three-dimensional aerogel with dual adsorption capacity toward methylene blue and ciprofloxacin</atitle><jtitle>Journal of the Iranian Chemical Society</jtitle><stitle>J IRAN CHEM SOC</stitle><date>2023-04-01</date><risdate>2023</risdate><volume>20</volume><issue>4</issue><spage>801</spage><epage>816</epage><pages>801-816</pages><issn>1735-207X</issn><eissn>1735-2428</eissn><abstract>To effectively treat the pollutant in sewage, a new-type three-dimensional aerogel based on graphene oxide and waste paper was fabricated via simple mixing and freeze-drying processes. Therein, waste paper was activated in advance, and polyvinyl alcohol served as physical crosslinking agent. The results showed that the obtained aerogel with porous three-dimensional network structure exhibited good thermal stability. When it acted as adsorbent for treating organic dye (methylene blue) and antibiotic (ciprofloxacin), the adsorption process was explored. In single system, the pseudo-first-order and pseudo-second-order kinetic models were used to discuss the detail about the aerogel adsorbing pollutant. Moreover, the Langmuir and Freundlich adsorption models were applied to describe the equilibrium isotherms and calculate the isotherm constants. Thermodynamic results stated that the adsorption of pollutant onto aerogel was feasible and spontaneous. In binary system, the adsorption capacity of methylene blue by aerogel increased, while the adsorption capacity of ciprofloxacin by aerogel declined. The pseudo-second-order kinetics was consistent with the adsorption of pollutant by aerogel in such binary system. This study would provide a new boulevard to develop environmental, low-cost and high-efficiency adsorbent for removing pollutant from wastewater.
Graphical abstract</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s13738-022-02714-5</doi><tpages>16</tpages><orcidid>https://orcid.org/0000-0002-4669-0401</orcidid></addata></record> |
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subjects | Adsorbents Adsorption Aerogels Analytical Chemistry Binary system Biochemistry Chemistry Chemistry and Materials Science Crosslinking Graphene Inorganic Chemistry Isotherms Methylene blue Organic Chemistry Original Paper Physical Chemistry Pollutants Polyvinyl alcohol Thermal stability Wastewater treatment |
title | Fabrication of waste paper/graphene oxide three-dimensional aerogel with dual adsorption capacity toward methylene blue and ciprofloxacin |
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