Preparation of zero-valent iron-nickle bimetallic composite for Se(IV) adsorption from aqueous solution
79 Se is one of the important radionuclides in the safety evaluation of high-level radioactive waste repository due to its long half-life and highly fissionable radioactivity. Nanoscale zero valent iron-nickel bimetallic composite (Fe 0 /Ni 0 ) was fabricated by liquid phase reduction method for Se(...
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| Veröffentlicht in: | Journal of radioanalytical and nuclear chemistry 2023-03, Vol.332 (3), p.785-796 |
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| container_title | Journal of radioanalytical and nuclear chemistry |
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| creator | Du, Yanjun Fu, Xiaohui Zhou, Qing Zhao, Jiankun Wu, Hexi Li, Xiaoyan Liu, Yibao Le, Zhanggao |
| description | 79
Se is one of the important radionuclides in the safety evaluation of high-level radioactive waste repository due to its long half-life and highly fissionable radioactivity. Nanoscale zero valent iron-nickel bimetallic composite (Fe
0
/Ni
0
) was fabricated by liquid phase reduction method for Se(IV) adsorption from aqueous solution. The effects of pH, solid–liquid ratio, time, temperature, initial concentration of Se(IV) on the adsorption of Se(IV) by Fe
0
/Ni
0
were investigated. Fe
0
/Ni
0
was characterized by SEM, XPS, XRD, FT-IR, BET and Zeta potential, and the mechanism of removing Se(IV) was analyzed. The results showed that Fe
0
/Ni
0
had a good removal effect on Se(IV). When pH was 3.5, the solid–liquid ratio was 0.3 g L
−1
, the reaction time was 40 min, the maximum adsorption capacity of Se(IV) by Fe
0
/Ni
0
could reach 180 mg g
−1
. The research results can provide a theoretical basis for the treatment of wastewater containing Se(IV). |
| doi_str_mv | 10.1007/s10967-023-08789-5 |
| format | Article |
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Se is one of the important radionuclides in the safety evaluation of high-level radioactive waste repository due to its long half-life and highly fissionable radioactivity. Nanoscale zero valent iron-nickel bimetallic composite (Fe
0
/Ni
0
) was fabricated by liquid phase reduction method for Se(IV) adsorption from aqueous solution. The effects of pH, solid–liquid ratio, time, temperature, initial concentration of Se(IV) on the adsorption of Se(IV) by Fe
0
/Ni
0
were investigated. Fe
0
/Ni
0
was characterized by SEM, XPS, XRD, FT-IR, BET and Zeta potential, and the mechanism of removing Se(IV) was analyzed. The results showed that Fe
0
/Ni
0
had a good removal effect on Se(IV). When pH was 3.5, the solid–liquid ratio was 0.3 g L
−1
, the reaction time was 40 min, the maximum adsorption capacity of Se(IV) by Fe
0
/Ni
0
could reach 180 mg g
−1
. The research results can provide a theoretical basis for the treatment of wastewater containing Se(IV).</description><identifier>ISSN: 0236-5731</identifier><identifier>EISSN: 1588-2780</identifier><identifier>DOI: 10.1007/s10967-023-08789-5</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Adsorption ; Aqueous solutions ; Bimetals ; Chemistry ; Chemistry and Materials Science ; Diagnostic Radiology ; Hadrons ; Heavy Ions ; High level radioactive wastes ; Inorganic Chemistry ; Iron ; Liquid phases ; Nuclear Chemistry ; Nuclear energy ; Nuclear Physics ; Nuclear safety ; Physical Chemistry ; Purification ; Radioactive waste sites ; Radioactive wastes ; Radioactivity ; Radioisotopes ; Sewage ; Wastewater ; Wastewater treatment ; X ray photoelectron spectroscopy ; Zeta potential</subject><ispartof>Journal of radioanalytical and nuclear chemistry, 2023-03, Vol.332 (3), p.785-796</ispartof><rights>Akadémiai Kiadó, Budapest, Hungary 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><rights>COPYRIGHT 2023 Springer</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c358t-4a0af33820c18ff4070c509cb548313a4d98ab11ae8c3f32c0ede8d1960c89343</citedby><cites>FETCH-LOGICAL-c358t-4a0af33820c18ff4070c509cb548313a4d98ab11ae8c3f32c0ede8d1960c89343</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10967-023-08789-5$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10967-023-08789-5$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Du, Yanjun</creatorcontrib><creatorcontrib>Fu, Xiaohui</creatorcontrib><creatorcontrib>Zhou, Qing</creatorcontrib><creatorcontrib>Zhao, Jiankun</creatorcontrib><creatorcontrib>Wu, Hexi</creatorcontrib><creatorcontrib>Li, Xiaoyan</creatorcontrib><creatorcontrib>Liu, Yibao</creatorcontrib><creatorcontrib>Le, Zhanggao</creatorcontrib><title>Preparation of zero-valent iron-nickle bimetallic composite for Se(IV) adsorption from aqueous solution</title><title>Journal of radioanalytical and nuclear chemistry</title><addtitle>J Radioanal Nucl Chem</addtitle><description>79
Se is one of the important radionuclides in the safety evaluation of high-level radioactive waste repository due to its long half-life and highly fissionable radioactivity. Nanoscale zero valent iron-nickel bimetallic composite (Fe
0
/Ni
0
) was fabricated by liquid phase reduction method for Se(IV) adsorption from aqueous solution. The effects of pH, solid–liquid ratio, time, temperature, initial concentration of Se(IV) on the adsorption of Se(IV) by Fe
0
/Ni
0
were investigated. Fe
0
/Ni
0
was characterized by SEM, XPS, XRD, FT-IR, BET and Zeta potential, and the mechanism of removing Se(IV) was analyzed. The results showed that Fe
0
/Ni
0
had a good removal effect on Se(IV). When pH was 3.5, the solid–liquid ratio was 0.3 g L
−1
, the reaction time was 40 min, the maximum adsorption capacity of Se(IV) by Fe
0
/Ni
0
could reach 180 mg g
−1
. The research results can provide a theoretical basis for the treatment of wastewater containing Se(IV).</description><subject>Adsorption</subject><subject>Aqueous solutions</subject><subject>Bimetals</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Diagnostic Radiology</subject><subject>Hadrons</subject><subject>Heavy Ions</subject><subject>High level radioactive wastes</subject><subject>Inorganic Chemistry</subject><subject>Iron</subject><subject>Liquid phases</subject><subject>Nuclear Chemistry</subject><subject>Nuclear energy</subject><subject>Nuclear Physics</subject><subject>Nuclear safety</subject><subject>Physical Chemistry</subject><subject>Purification</subject><subject>Radioactive waste sites</subject><subject>Radioactive wastes</subject><subject>Radioactivity</subject><subject>Radioisotopes</subject><subject>Sewage</subject><subject>Wastewater</subject><subject>Wastewater treatment</subject><subject>X ray photoelectron spectroscopy</subject><subject>Zeta potential</subject><issn>0236-5731</issn><issn>1588-2780</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNp9kU1LxDAQhoMouH78AU8BL3rIOmnSJj3K4sfCgoIf15BNkyXaNjXpCvrrjVbwJnMYmLzPzGRehE4ozCmAuEgU6koQKBgBKWRNyh00o6WUpBASdtEsv1SkFIzuo4OUXgCglpLN0OY-2kFHPfrQ4-Dwp42BvOvW9iP2MfSk9-a1tXjtOzvqtvUGm9ANIfnRYhcifrBny-dzrJsU4vDTxcXQYf22tWGbcArt9rt6hPacbpM9_s2H6On66nFxS1Z3N8vF5YoYVsqRcA3aMSYLMFQ6x0GAKaE265JLRpnmTS31mlJtpWGOFQZsY2VD6wqMrBlnh-h06jvEkFdIo3oJ29jnkSpfQlSccl5k1XxSbfJPle9dGKM2ORrbeRN663yuXwpOq1oIzjJQTICJIaVonRqi73T8UBTUtwNqckDlO6sfB1SZITZBKYv7jY1_u_xDfQGUCYnH</recordid><startdate>20230301</startdate><enddate>20230301</enddate><creator>Du, Yanjun</creator><creator>Fu, Xiaohui</creator><creator>Zhou, Qing</creator><creator>Zhao, Jiankun</creator><creator>Wu, Hexi</creator><creator>Li, Xiaoyan</creator><creator>Liu, Yibao</creator><creator>Le, Zhanggao</creator><general>Springer International Publishing</general><general>Springer</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>20230301</creationdate><title>Preparation of zero-valent iron-nickle bimetallic composite for Se(IV) adsorption from aqueous solution</title><author>Du, Yanjun ; Fu, Xiaohui ; Zhou, Qing ; Zhao, Jiankun ; Wu, Hexi ; Li, Xiaoyan ; Liu, Yibao ; Le, Zhanggao</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c358t-4a0af33820c18ff4070c509cb548313a4d98ab11ae8c3f32c0ede8d1960c89343</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Adsorption</topic><topic>Aqueous solutions</topic><topic>Bimetals</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Diagnostic Radiology</topic><topic>Hadrons</topic><topic>Heavy Ions</topic><topic>High level radioactive wastes</topic><topic>Inorganic Chemistry</topic><topic>Iron</topic><topic>Liquid phases</topic><topic>Nuclear Chemistry</topic><topic>Nuclear energy</topic><topic>Nuclear Physics</topic><topic>Nuclear safety</topic><topic>Physical Chemistry</topic><topic>Purification</topic><topic>Radioactive waste sites</topic><topic>Radioactive wastes</topic><topic>Radioactivity</topic><topic>Radioisotopes</topic><topic>Sewage</topic><topic>Wastewater</topic><topic>Wastewater treatment</topic><topic>X ray photoelectron spectroscopy</topic><topic>Zeta potential</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Du, Yanjun</creatorcontrib><creatorcontrib>Fu, Xiaohui</creatorcontrib><creatorcontrib>Zhou, Qing</creatorcontrib><creatorcontrib>Zhao, Jiankun</creatorcontrib><creatorcontrib>Wu, Hexi</creatorcontrib><creatorcontrib>Li, Xiaoyan</creatorcontrib><creatorcontrib>Liu, Yibao</creatorcontrib><creatorcontrib>Le, Zhanggao</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Du, Yanjun</au><au>Fu, Xiaohui</au><au>Zhou, Qing</au><au>Zhao, Jiankun</au><au>Wu, Hexi</au><au>Li, Xiaoyan</au><au>Liu, Yibao</au><au>Le, Zhanggao</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Preparation of zero-valent iron-nickle bimetallic composite for Se(IV) adsorption from aqueous solution</atitle><jtitle>Journal of radioanalytical and nuclear chemistry</jtitle><stitle>J Radioanal Nucl Chem</stitle><date>2023-03-01</date><risdate>2023</risdate><volume>332</volume><issue>3</issue><spage>785</spage><epage>796</epage><pages>785-796</pages><issn>0236-5731</issn><eissn>1588-2780</eissn><abstract>79
Se is one of the important radionuclides in the safety evaluation of high-level radioactive waste repository due to its long half-life and highly fissionable radioactivity. Nanoscale zero valent iron-nickel bimetallic composite (Fe
0
/Ni
0
) was fabricated by liquid phase reduction method for Se(IV) adsorption from aqueous solution. The effects of pH, solid–liquid ratio, time, temperature, initial concentration of Se(IV) on the adsorption of Se(IV) by Fe
0
/Ni
0
were investigated. Fe
0
/Ni
0
was characterized by SEM, XPS, XRD, FT-IR, BET and Zeta potential, and the mechanism of removing Se(IV) was analyzed. The results showed that Fe
0
/Ni
0
had a good removal effect on Se(IV). When pH was 3.5, the solid–liquid ratio was 0.3 g L
−1
, the reaction time was 40 min, the maximum adsorption capacity of Se(IV) by Fe
0
/Ni
0
could reach 180 mg g
−1
. The research results can provide a theoretical basis for the treatment of wastewater containing Se(IV).</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s10967-023-08789-5</doi><tpages>12</tpages></addata></record> |
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| subjects | Adsorption Aqueous solutions Bimetals Chemistry Chemistry and Materials Science Diagnostic Radiology Hadrons Heavy Ions High level radioactive wastes Inorganic Chemistry Iron Liquid phases Nuclear Chemistry Nuclear energy Nuclear Physics Nuclear safety Physical Chemistry Purification Radioactive waste sites Radioactive wastes Radioactivity Radioisotopes Sewage Wastewater Wastewater treatment X ray photoelectron spectroscopy Zeta potential |
| title | Preparation of zero-valent iron-nickle bimetallic composite for Se(IV) adsorption from aqueous solution |
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