Thermal modulation of reaction equilibria controls mass transfer in CO2-binding organic liquids

CO2-Binding organic liquids (CO2BOLs) are non-aqueous solvents which may reduce the parasitic energy of carbon capture processes. These solvents exhibit surprising mass transfer behavior: at fixed pressure driving force, the flux of CO2 into CO2BOLs decreases exponentially with increased temperature...

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Veröffentlicht in:	Energy & environmental science 2023-02, Vol.16 (2), p.484-490
Hauptverfasser:	Moore, Thomas, Varni, Anthony J, Pang, Simon H, Akhade, Sneha A, Li, Sichi, Nguyen, Du T, Stolaroff, Joshuah K
Format:	Artikel
Sprache:	eng
Schlagworte:	Amines Binding Carbon dioxide Carbon sequestration Chemical reactions Density functional theory First principles Fluctuations Hexanol Mass transfer Organic liquids Solvents
Online-Zugang:	Volltext
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