Water Desalination by Pervaporation Using MIL-101(Cr) and MIL-101(Cr)@GODoped PVA Hybrid Membranes
In this study, MIL-101(Cr) and MIL-101(Cr)@GO were produced and added to the poly (vinyl alcohol) (PVA) membrane for the manufacture of hybrid membranes to use in pervaporative desalination. The MIL-101(Cr) and MIL-101(Cr)@GO additives were identified using Fourier-transform infrared spectroscopy (F...
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| Veröffentlicht in: | Water, air, and soil pollution air, and soil pollution, 2023-02, Vol.234 (2), p.96, Article 96 |
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| description | In this study, MIL-101(Cr) and MIL-101(Cr)@GO were produced and added to the poly (vinyl alcohol) (PVA) membrane for the manufacture of hybrid membranes to use in pervaporative desalination. The MIL-101(Cr) and MIL-101(Cr)@GO additives were identified using Fourier-transform infrared spectroscopy (FTIR) and X-ray powder diffraction (XRD). The hybrid membranes were analyzed by using FTIR (chemical bond structure), XRD (crystallinity and amorphous phase), scanning electron microscope (SEM) (morphologic structure), thermogravimetric analysis (TGA) (thermal features), and contact angle (hydrophility). The effects of MIL-101(Cr) and MIL-101 (Cr)@GO content in the PVA membrane, feed sodium chloride (NaCl) concentration, and operation temperature were assessed for the flux and salt rejection. The addition of MIL-101(Cr) and MIL-101(Cr)@GO to the PVA membrane improved the purification performance in pervaporative desalination applications. The durability of the hybrid membrane for desalination was studied. The optimal loading ratios for MIL-101(Cr) and MIL-101(Cr)@GO were specified as 4 wt% MIL-101(Cr) and 4 wt% MIL-101(Cr)@GO, respectively. Optimum operation parameters were achieved at 60 °C of temperature and a 4 wt% of feed NaCl concentration for both hybrid membranes. Hybrid membranes (MIL-101(Cr)@GO doping) exhibited excellent desalination success with salt rejections of 99.99% and fluxes of 9.7 kg/m
2
h. It was also seen that the hybrid membranes preserved their separation performance during 10 cycles. |
| doi_str_mv | 10.1007/s11270-023-06128-8 |
| format | Article |
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2
h. It was also seen that the hybrid membranes preserved their separation performance during 10 cycles.</description><identifier>ISSN: 0049-6979</identifier><identifier>EISSN: 1573-2932</identifier><identifier>DOI: 10.1007/s11270-023-06128-8</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Additives ; Alcohols ; Analytical methods ; Atmospheric Protection/Air Quality Control/Air Pollution ; Chemical bonds ; Climate Change/Climate Change Impacts ; Contact angle ; Desalination ; Earth and Environmental Science ; Electron microscopes ; Environment ; Environmental monitoring ; Fourier transforms ; Hydrogeology ; Infrared spectroscopy ; Membranes ; Optimization ; Pervaporation ; Salt rejection ; Scanning electron microscopy ; Sodium ; Sodium chloride ; Soil Science & Conservation ; Temperature ; Thermogravimetric analysis ; Water desalting ; Water purification ; Water Quality/Water Pollution ; X ray powder diffraction ; X-ray diffraction</subject><ispartof>Water, air, and soil pollution, 2023-02, Vol.234 (2), p.96, Article 96</ispartof><rights>The Author(s), under exclusive licence to Springer Nature Switzerland AG 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c249t-14052509d09c964462f10b458f5c157e96ebcf09157842d62462544775088e383</citedby><cites>FETCH-LOGICAL-c249t-14052509d09c964462f10b458f5c157e96ebcf09157842d62462544775088e383</cites><orcidid>0000-0001-5240-5876</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11270-023-06128-8$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11270-023-06128-8$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Unlu, Derya</creatorcontrib><title>Water Desalination by Pervaporation Using MIL-101(Cr) and MIL-101(Cr)@GODoped PVA Hybrid Membranes</title><title>Water, air, and soil pollution</title><addtitle>Water Air Soil Pollut</addtitle><description>In this study, MIL-101(Cr) and MIL-101(Cr)@GO were produced and added to the poly (vinyl alcohol) (PVA) membrane for the manufacture of hybrid membranes to use in pervaporative desalination. The MIL-101(Cr) and MIL-101(Cr)@GO additives were identified using Fourier-transform infrared spectroscopy (FTIR) and X-ray powder diffraction (XRD). The hybrid membranes were analyzed by using FTIR (chemical bond structure), XRD (crystallinity and amorphous phase), scanning electron microscope (SEM) (morphologic structure), thermogravimetric analysis (TGA) (thermal features), and contact angle (hydrophility). The effects of MIL-101(Cr) and MIL-101 (Cr)@GO content in the PVA membrane, feed sodium chloride (NaCl) concentration, and operation temperature were assessed for the flux and salt rejection. The addition of MIL-101(Cr) and MIL-101(Cr)@GO to the PVA membrane improved the purification performance in pervaporative desalination applications. The durability of the hybrid membrane for desalination was studied. The optimal loading ratios for MIL-101(Cr) and MIL-101(Cr)@GO were specified as 4 wt% MIL-101(Cr) and 4 wt% MIL-101(Cr)@GO, respectively. Optimum operation parameters were achieved at 60 °C of temperature and a 4 wt% of feed NaCl concentration for both hybrid membranes. Hybrid membranes (MIL-101(Cr)@GO doping) exhibited excellent desalination success with salt rejections of 99.99% and fluxes of 9.7 kg/m
2
h. It was also seen that the hybrid membranes preserved their separation performance during 10 cycles.</description><subject>Additives</subject><subject>Alcohols</subject><subject>Analytical methods</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Chemical bonds</subject><subject>Climate Change/Climate Change Impacts</subject><subject>Contact angle</subject><subject>Desalination</subject><subject>Earth and Environmental Science</subject><subject>Electron microscopes</subject><subject>Environment</subject><subject>Environmental monitoring</subject><subject>Fourier transforms</subject><subject>Hydrogeology</subject><subject>Infrared spectroscopy</subject><subject>Membranes</subject><subject>Optimization</subject><subject>Pervaporation</subject><subject>Salt rejection</subject><subject>Scanning electron microscopy</subject><subject>Sodium</subject><subject>Sodium chloride</subject><subject>Soil Science & Conservation</subject><subject>Temperature</subject><subject>Thermogravimetric analysis</subject><subject>Water desalting</subject><subject>Water purification</subject><subject>Water Quality/Water Pollution</subject><subject>X ray powder diffraction</subject><subject>X-ray 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Desalination by Pervaporation Using MIL-101(Cr) and MIL-101(Cr)@GODoped PVA Hybrid Membranes</title><author>Unlu, Derya</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c249t-14052509d09c964462f10b458f5c157e96ebcf09157842d62462544775088e383</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Additives</topic><topic>Alcohols</topic><topic>Analytical methods</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Chemical bonds</topic><topic>Climate Change/Climate Change Impacts</topic><topic>Contact angle</topic><topic>Desalination</topic><topic>Earth and Environmental Science</topic><topic>Electron microscopes</topic><topic>Environment</topic><topic>Environmental monitoring</topic><topic>Fourier transforms</topic><topic>Hydrogeology</topic><topic>Infrared 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Pollut</stitle><date>2023-02-01</date><risdate>2023</risdate><volume>234</volume><issue>2</issue><spage>96</spage><pages>96-</pages><artnum>96</artnum><issn>0049-6979</issn><eissn>1573-2932</eissn><abstract>In this study, MIL-101(Cr) and MIL-101(Cr)@GO were produced and added to the poly (vinyl alcohol) (PVA) membrane for the manufacture of hybrid membranes to use in pervaporative desalination. The MIL-101(Cr) and MIL-101(Cr)@GO additives were identified using Fourier-transform infrared spectroscopy (FTIR) and X-ray powder diffraction (XRD). The hybrid membranes were analyzed by using FTIR (chemical bond structure), XRD (crystallinity and amorphous phase), scanning electron microscope (SEM) (morphologic structure), thermogravimetric analysis (TGA) (thermal features), and contact angle (hydrophility). The effects of MIL-101(Cr) and MIL-101 (Cr)@GO content in the PVA membrane, feed sodium chloride (NaCl) concentration, and operation temperature were assessed for the flux and salt rejection. The addition of MIL-101(Cr) and MIL-101(Cr)@GO to the PVA membrane improved the purification performance in pervaporative desalination applications. The durability of the hybrid membrane for desalination was studied. The optimal loading ratios for MIL-101(Cr) and MIL-101(Cr)@GO were specified as 4 wt% MIL-101(Cr) and 4 wt% MIL-101(Cr)@GO, respectively. Optimum operation parameters were achieved at 60 °C of temperature and a 4 wt% of feed NaCl concentration for both hybrid membranes. Hybrid membranes (MIL-101(Cr)@GO doping) exhibited excellent desalination success with salt rejections of 99.99% and fluxes of 9.7 kg/m
2
h. It was also seen that the hybrid membranes preserved their separation performance during 10 cycles.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s11270-023-06128-8</doi><orcidid>https://orcid.org/0000-0001-5240-5876</orcidid></addata></record> |
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| ispartof | Water, air, and soil pollution, 2023-02, Vol.234 (2), p.96, Article 96 |
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| subjects | Additives Alcohols Analytical methods Atmospheric Protection/Air Quality Control/Air Pollution Chemical bonds Climate Change/Climate Change Impacts Contact angle Desalination Earth and Environmental Science Electron microscopes Environment Environmental monitoring Fourier transforms Hydrogeology Infrared spectroscopy Membranes Optimization Pervaporation Salt rejection Scanning electron microscopy Sodium Sodium chloride Soil Science & Conservation Temperature Thermogravimetric analysis Water desalting Water purification Water Quality/Water Pollution X ray powder diffraction X-ray diffraction |
| title | Water Desalination by Pervaporation Using MIL-101(Cr) and MIL-101(Cr)@GODoped PVA Hybrid Membranes |
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