Facile Preparation and Adsorption Behavior Studies of Poly(acrylic acid)-Based Hydrogels Reinforced by Hydrogen Bonds for Methylene Blue Dye
To suppress the extreme swelling of poly(acrylic acid) (PAA) hydrogels, two series of PAA-based hydrogels with additional non-covalent crosslinks were successfully synthesized by incorporating allyloxypolyethyleneglycol (APEG) or polyvinylpyrrolidone (PVP) to form hydrogen bonds. The developed hydro...
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| Veröffentlicht in: | Journal of polymers and the environment 2023-02, Vol.31 (2), p.552-564 |
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| creator | Yao, Jiale Yang, He Zuo, Danying Xu, Jing Zhang, Hongwei |
| description | To suppress the extreme swelling of poly(acrylic acid) (PAA) hydrogels, two series of PAA-based hydrogels with additional non-covalent crosslinks were successfully synthesized by incorporating allyloxypolyethyleneglycol (APEG) or polyvinylpyrrolidone (PVP) to form hydrogen bonds. The developed hydrogels were characterized by scanning electron microscopy (SEM) and Fourier transform infrared (FTIR). The swelling and methylene blue (MB) adsorption experiments of them were performed. Both series of hydrogels exhibited moderate swelling ratios of 213–235 g g
−1
and excellent removal efficiency of MB (> 92%). Based on kinetic assessments, the MB adsorption process could be well-described by the pseudo-second-order kinetic and Langmuir isotherm models, suggesting a monolayer chemisorption mechanism. The maximum theoretical adsorption capacity (
q
m
) of the PAA-based hydrogel with PVP could achieve 2483.2 mg g
−1
. Regeneration experiments showed that both series of hydrogels could endure adsorption/desorption for at least 5 consecutive cycles with MB removal efficiency of higher than 80%. Therefore, it was believed that this study could provide a facile method to develop hydrogel adsorbents and a promising adsorbent material with high adsorption capacity for the removal of MB from dye-containing wastewater. |
| doi_str_mv | 10.1007/s10924-022-02610-2 |
| format | Article |
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−1
and excellent removal efficiency of MB (> 92%). Based on kinetic assessments, the MB adsorption process could be well-described by the pseudo-second-order kinetic and Langmuir isotherm models, suggesting a monolayer chemisorption mechanism. The maximum theoretical adsorption capacity (
q
m
) of the PAA-based hydrogel with PVP could achieve 2483.2 mg g
−1
. Regeneration experiments showed that both series of hydrogels could endure adsorption/desorption for at least 5 consecutive cycles with MB removal efficiency of higher than 80%. Therefore, it was believed that this study could provide a facile method to develop hydrogel adsorbents and a promising adsorbent material with high adsorption capacity for the removal of MB from dye-containing wastewater.</description><identifier>ISSN: 1566-2543</identifier><identifier>EISSN: 1572-8919</identifier><identifier>DOI: 10.1007/s10924-022-02610-2</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Acrylic acid ; Acrylics ; Adsorbents ; Adsorption ; Chemisorption ; Chemistry ; Chemistry and Materials Science ; Dyes ; Environmental Chemistry ; Environmental Engineering/Biotechnology ; Fourier transforms ; Hydrogels ; Hydrogen bonding ; Hydrogen bonds ; Industrial Chemistry/Chemical Engineering ; Materials Science ; Methylene blue ; Original Paper ; Polyacrylic acid ; Polymer Sciences ; Polyvinylpyrrolidone ; Scanning electron microscopy ; Swelling ratio ; Wastewater</subject><ispartof>Journal of polymers and the environment, 2023-02, Vol.31 (2), p.552-564</ispartof><rights>The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-393c225a7eb69cea12e9427e6f61410a878ffc3d9e6efbb3240de2672fadddf83</citedby><cites>FETCH-LOGICAL-c319t-393c225a7eb69cea12e9427e6f61410a878ffc3d9e6efbb3240de2672fadddf83</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10924-022-02610-2$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10924-022-02610-2$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Yao, Jiale</creatorcontrib><creatorcontrib>Yang, He</creatorcontrib><creatorcontrib>Zuo, Danying</creatorcontrib><creatorcontrib>Xu, Jing</creatorcontrib><creatorcontrib>Zhang, Hongwei</creatorcontrib><title>Facile Preparation and Adsorption Behavior Studies of Poly(acrylic acid)-Based Hydrogels Reinforced by Hydrogen Bonds for Methylene Blue Dye</title><title>Journal of polymers and the environment</title><addtitle>J Polym Environ</addtitle><description>To suppress the extreme swelling of poly(acrylic acid) (PAA) hydrogels, two series of PAA-based hydrogels with additional non-covalent crosslinks were successfully synthesized by incorporating allyloxypolyethyleneglycol (APEG) or polyvinylpyrrolidone (PVP) to form hydrogen bonds. The developed hydrogels were characterized by scanning electron microscopy (SEM) and Fourier transform infrared (FTIR). The swelling and methylene blue (MB) adsorption experiments of them were performed. Both series of hydrogels exhibited moderate swelling ratios of 213–235 g g
−1
and excellent removal efficiency of MB (> 92%). Based on kinetic assessments, the MB adsorption process could be well-described by the pseudo-second-order kinetic and Langmuir isotherm models, suggesting a monolayer chemisorption mechanism. The maximum theoretical adsorption capacity (
q
m
) of the PAA-based hydrogel with PVP could achieve 2483.2 mg g
−1
. Regeneration experiments showed that both series of hydrogels could endure adsorption/desorption for at least 5 consecutive cycles with MB removal efficiency of higher than 80%. Therefore, it was believed that this study could provide a facile method to develop hydrogel adsorbents and a promising adsorbent material with high adsorption capacity for the removal of MB from dye-containing wastewater.</description><subject>Acrylic acid</subject><subject>Acrylics</subject><subject>Adsorbents</subject><subject>Adsorption</subject><subject>Chemisorption</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Dyes</subject><subject>Environmental Chemistry</subject><subject>Environmental Engineering/Biotechnology</subject><subject>Fourier transforms</subject><subject>Hydrogels</subject><subject>Hydrogen bonding</subject><subject>Hydrogen bonds</subject><subject>Industrial Chemistry/Chemical Engineering</subject><subject>Materials Science</subject><subject>Methylene blue</subject><subject>Original Paper</subject><subject>Polyacrylic acid</subject><subject>Polymer Sciences</subject><subject>Polyvinylpyrrolidone</subject><subject>Scanning electron microscopy</subject><subject>Swelling ratio</subject><subject>Wastewater</subject><issn>1566-2543</issn><issn>1572-8919</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNp9UMtOwzAQjBBIlMIPcLLEBQ4BP9I4PraFUqQiKh5ny7XXbaoQFztByj_w0bgtiBuH1e7OzsxKkyTnBF8TjPlNIFjQLMWUxsoJTulB0iMDTtNCEHG4nfM8pYOMHScnIawxxiIKe8nXROmyAjT3sFFeNaWrkaoNGprg_Ga3jmClPkvn0UvTmhICchbNXdVdKu27qtQoOpirdKQCGDTtjHdLqAJ6hrK2zusILrpfPLq52gQUD-gRmlVXQQ1oVLWAbjs4TY6sqgKc_fR-8ja5ex1P09nT_cN4OEs1I6JJmWCa0oHisMiFBkUoiIxyyG1OMoJVwQtrNTMCcrCLBaMZNkBzTq0yxtiC9ZOLve_Gu48WQiPXrvV1fCkp55hxzAsSWXTP0t6F4MHKjS_fle8kwXKbutynLmPqcpe6pFHE9qIQyfUS_J_1P6pvfzyGzQ</recordid><startdate>20230201</startdate><enddate>20230201</enddate><creator>Yao, Jiale</creator><creator>Yang, He</creator><creator>Zuo, Danying</creator><creator>Xu, Jing</creator><creator>Zhang, Hongwei</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7SR</scope><scope>7XB</scope><scope>88I</scope><scope>8AO</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>8FK</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>BHPHI</scope><scope>BKSAR</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>M2P</scope><scope>PATMY</scope><scope>PCBAR</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope></search><sort><creationdate>20230201</creationdate><title>Facile Preparation and Adsorption Behavior Studies of Poly(acrylic acid)-Based Hydrogels Reinforced by Hydrogen Bonds for Methylene Blue Dye</title><author>Yao, Jiale ; Yang, He ; Zuo, Danying ; Xu, Jing ; Zhang, Hongwei</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-393c225a7eb69cea12e9427e6f61410a878ffc3d9e6efbb3240de2672fadddf83</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Acrylic acid</topic><topic>Acrylics</topic><topic>Adsorbents</topic><topic>Adsorption</topic><topic>Chemisorption</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Dyes</topic><topic>Environmental Chemistry</topic><topic>Environmental Engineering/Biotechnology</topic><topic>Fourier transforms</topic><topic>Hydrogels</topic><topic>Hydrogen bonding</topic><topic>Hydrogen bonds</topic><topic>Industrial Chemistry/Chemical Engineering</topic><topic>Materials Science</topic><topic>Methylene blue</topic><topic>Original Paper</topic><topic>Polyacrylic acid</topic><topic>Polymer Sciences</topic><topic>Polyvinylpyrrolidone</topic><topic>Scanning electron microscopy</topic><topic>Swelling ratio</topic><topic>Wastewater</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yao, Jiale</creatorcontrib><creatorcontrib>Yang, He</creatorcontrib><creatorcontrib>Zuo, Danying</creatorcontrib><creatorcontrib>Xu, Jing</creatorcontrib><creatorcontrib>Zhang, Hongwei</creatorcontrib><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Engineered Materials Abstracts</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest Pharma Collection</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central UK/Ireland</collection><collection>Agricultural & Environmental Science Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>Natural Science Collection</collection><collection>Earth, Atmospheric & Aquatic Science Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>Materials Research Database</collection><collection>Materials Science Database</collection><collection>Science Database</collection><collection>Environmental Science Database</collection><collection>Earth, Atmospheric & Aquatic Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Environmental Science Collection</collection><collection>ProQuest Central Basic</collection><jtitle>Journal of polymers and the environment</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Yao, Jiale</au><au>Yang, He</au><au>Zuo, Danying</au><au>Xu, Jing</au><au>Zhang, Hongwei</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Facile Preparation and Adsorption Behavior Studies of Poly(acrylic acid)-Based Hydrogels Reinforced by Hydrogen Bonds for Methylene Blue Dye</atitle><jtitle>Journal of polymers and the environment</jtitle><stitle>J Polym Environ</stitle><date>2023-02-01</date><risdate>2023</risdate><volume>31</volume><issue>2</issue><spage>552</spage><epage>564</epage><pages>552-564</pages><issn>1566-2543</issn><eissn>1572-8919</eissn><abstract>To suppress the extreme swelling of poly(acrylic acid) (PAA) hydrogels, two series of PAA-based hydrogels with additional non-covalent crosslinks were successfully synthesized by incorporating allyloxypolyethyleneglycol (APEG) or polyvinylpyrrolidone (PVP) to form hydrogen bonds. The developed hydrogels were characterized by scanning electron microscopy (SEM) and Fourier transform infrared (FTIR). The swelling and methylene blue (MB) adsorption experiments of them were performed. Both series of hydrogels exhibited moderate swelling ratios of 213–235 g g
−1
and excellent removal efficiency of MB (> 92%). Based on kinetic assessments, the MB adsorption process could be well-described by the pseudo-second-order kinetic and Langmuir isotherm models, suggesting a monolayer chemisorption mechanism. The maximum theoretical adsorption capacity (
q
m
) of the PAA-based hydrogel with PVP could achieve 2483.2 mg g
−1
. Regeneration experiments showed that both series of hydrogels could endure adsorption/desorption for at least 5 consecutive cycles with MB removal efficiency of higher than 80%. Therefore, it was believed that this study could provide a facile method to develop hydrogel adsorbents and a promising adsorbent material with high adsorption capacity for the removal of MB from dye-containing wastewater.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10924-022-02610-2</doi><tpages>13</tpages></addata></record> |
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| subjects | Acrylic acid Acrylics Adsorbents Adsorption Chemisorption Chemistry Chemistry and Materials Science Dyes Environmental Chemistry Environmental Engineering/Biotechnology Fourier transforms Hydrogels Hydrogen bonding Hydrogen bonds Industrial Chemistry/Chemical Engineering Materials Science Methylene blue Original Paper Polyacrylic acid Polymer Sciences Polyvinylpyrrolidone Scanning electron microscopy Swelling ratio Wastewater |
| title | Facile Preparation and Adsorption Behavior Studies of Poly(acrylic acid)-Based Hydrogels Reinforced by Hydrogen Bonds for Methylene Blue Dye |
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