In situ preparation of FeOx nanoparticles embedded N-doped laser-induced graphene for flexible in-plane micro-supercapacitors
Laser direct writing of polyimide (PI) film to induce porous graphene as a flexible electrode facilitates the development of efficient, low-cost, and large-scale preparation of flexible planar micro-supercapacitors (MSCs). Nevertheless, current flexible MSCs based on laser-induced graphene (LIG) fac...
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Veröffentlicht in: | Ionics 2023, Vol.29 (1), p.419-427 |
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description | Laser direct writing of polyimide (PI) film to induce porous graphene as a flexible electrode facilitates the development of efficient, low-cost, and large-scale preparation of flexible planar micro-supercapacitors (MSCs). Nevertheless, current flexible MSCs based on laser-induced graphene (LIG) face bottlenecks such as poor LIG electrode wettability, inhomogeneous doping of heterogeneous components, and limited electrochemical performance. In view of this, a simple and effective process for in situ fabrication of flexible FeO
x
nanoparticles embedded N-doped LIG (FeO
x
@NLIG) electrode is developed by laser direct writing in this study. The as-assembled in-plane FeO
x
@NLIG MSCs exhibit an excellent areal specific capacitance of 13.82 mF cm
−2
, a remarkable energy density of 1.228 mW h cm
−2
at a high power density of 0.024 mW cm
−2
, good flexibility, and conspicuous cycling stability. Besides, these high-performance in-plane FeO
x
@NLIG MSCs as a vital micro-energy storage component can be easily miniaturized, modularized, and integrated to suit customized needs of wearable electronics due to great advantages in terms of identicality and stability of the as-fabricated FeO
x
@NLIG.
Graphical abstract |
doi_str_mv | 10.1007/s11581-022-04795-x |
format | Article |
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x
nanoparticles embedded N-doped LIG (FeO
x
@NLIG) electrode is developed by laser direct writing in this study. The as-assembled in-plane FeO
x
@NLIG MSCs exhibit an excellent areal specific capacitance of 13.82 mF cm
−2
, a remarkable energy density of 1.228 mW h cm
−2
at a high power density of 0.024 mW cm
−2
, good flexibility, and conspicuous cycling stability. Besides, these high-performance in-plane FeO
x
@NLIG MSCs as a vital micro-energy storage component can be easily miniaturized, modularized, and integrated to suit customized needs of wearable electronics due to great advantages in terms of identicality and stability of the as-fabricated FeO
x
@NLIG.
Graphical abstract</description><identifier>ISSN: 0947-7047</identifier><identifier>EISSN: 1862-0760</identifier><identifier>DOI: 10.1007/s11581-022-04795-x</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Chemistry ; Chemistry and Materials Science ; Condensed Matter Physics ; Direct laser writing ; Electrochemical analysis ; Electrochemistry ; Electrodes ; Energy Storage ; Graphene ; Lasers ; Nanoparticles ; Optical and Electronic Materials ; Original Paper ; Renewable and Green Energy ; Stability ; Supercapacitors ; Wettability</subject><ispartof>Ionics, 2023, Vol.29 (1), p.419-427</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-3102a06f3c5330c692b7b735b805a7d8e3524708124fb49f9b7d71496ea28b813</citedby><cites>FETCH-LOGICAL-c319t-3102a06f3c5330c692b7b735b805a7d8e3524708124fb49f9b7d71496ea28b813</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11581-022-04795-x$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11581-022-04795-x$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>315,781,785,27928,27929,41492,42561,51323</link.rule.ids></links><search><creatorcontrib>Zhao, Jiang</creatorcontrib><creatorcontrib>Zhang, Da</creatorcontrib><creatorcontrib>Wang, Shumeng</creatorcontrib><creatorcontrib>Wang, Zhitong</creatorcontrib><creatorcontrib>Xu, Rongqing</creatorcontrib><title>In situ preparation of FeOx nanoparticles embedded N-doped laser-induced graphene for flexible in-plane micro-supercapacitors</title><title>Ionics</title><addtitle>Ionics</addtitle><description>Laser direct writing of polyimide (PI) film to induce porous graphene as a flexible electrode facilitates the development of efficient, low-cost, and large-scale preparation of flexible planar micro-supercapacitors (MSCs). Nevertheless, current flexible MSCs based on laser-induced graphene (LIG) face bottlenecks such as poor LIG electrode wettability, inhomogeneous doping of heterogeneous components, and limited electrochemical performance. In view of this, a simple and effective process for in situ fabrication of flexible FeO
x
nanoparticles embedded N-doped LIG (FeO
x
@NLIG) electrode is developed by laser direct writing in this study. The as-assembled in-plane FeO
x
@NLIG MSCs exhibit an excellent areal specific capacitance of 13.82 mF cm
−2
, a remarkable energy density of 1.228 mW h cm
−2
at a high power density of 0.024 mW cm
−2
, good flexibility, and conspicuous cycling stability. Besides, these high-performance in-plane FeO
x
@NLIG MSCs as a vital micro-energy storage component can be easily miniaturized, modularized, and integrated to suit customized needs of wearable electronics due to great advantages in terms of identicality and stability of the as-fabricated FeO
x
@NLIG.
Graphical abstract</description><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Condensed Matter Physics</subject><subject>Direct laser writing</subject><subject>Electrochemical analysis</subject><subject>Electrochemistry</subject><subject>Electrodes</subject><subject>Energy Storage</subject><subject>Graphene</subject><subject>Lasers</subject><subject>Nanoparticles</subject><subject>Optical and Electronic Materials</subject><subject>Original Paper</subject><subject>Renewable and Green Energy</subject><subject>Stability</subject><subject>Supercapacitors</subject><subject>Wettability</subject><issn>0947-7047</issn><issn>1862-0760</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNp9kE9LxDAQxYMouK5-AU8Bz9H8aZv2KIurC4t70XNI2-mapZvEpIV68LsbreDN02Nm3psZfghdM3rLKJV3kbG8ZIRyTmgmq5xMJ2jByiKVsqCnaEGrTBKZZufoIsYDpUXBuFygz43F0Qwj9gG8DnowzmLX4TXsJmy1dak5mKaHiOFYQ9tCi59J63zSXkcIxNh2bFK1D9q_gQXcuYC7HiZT94CNJb7XqXs0TXAkjh5Co71uzOBCvERnne4jXP3qEr2uH15WT2S7e9ys7rekEawaiGCUa1p0osmFoE1R8VrWUuR1SXMt2xJEzjNJS8azrs6qrqplK1lWFaB5WZdMLNHNvNcH9z5CHNTBjcGmk4rLBIKxTPLk4rMrfRpjgE75YI46fChG1TdmNWNWCbP6waymFBJzKCaz3UP4W_1P6gtByoGu</recordid><startdate>2023</startdate><enddate>2023</enddate><creator>Zhao, Jiang</creator><creator>Zhang, Da</creator><creator>Wang, Shumeng</creator><creator>Wang, Zhitong</creator><creator>Xu, Rongqing</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>2023</creationdate><title>In situ preparation of FeOx nanoparticles embedded N-doped laser-induced graphene for flexible in-plane micro-supercapacitors</title><author>Zhao, Jiang ; Zhang, Da ; Wang, Shumeng ; Wang, Zhitong ; Xu, Rongqing</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-3102a06f3c5330c692b7b735b805a7d8e3524708124fb49f9b7d71496ea28b813</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Condensed Matter Physics</topic><topic>Direct laser writing</topic><topic>Electrochemical analysis</topic><topic>Electrochemistry</topic><topic>Electrodes</topic><topic>Energy Storage</topic><topic>Graphene</topic><topic>Lasers</topic><topic>Nanoparticles</topic><topic>Optical and Electronic Materials</topic><topic>Original Paper</topic><topic>Renewable and Green Energy</topic><topic>Stability</topic><topic>Supercapacitors</topic><topic>Wettability</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhao, Jiang</creatorcontrib><creatorcontrib>Zhang, Da</creatorcontrib><creatorcontrib>Wang, Shumeng</creatorcontrib><creatorcontrib>Wang, Zhitong</creatorcontrib><creatorcontrib>Xu, Rongqing</creatorcontrib><collection>CrossRef</collection><jtitle>Ionics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhao, Jiang</au><au>Zhang, Da</au><au>Wang, Shumeng</au><au>Wang, Zhitong</au><au>Xu, Rongqing</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>In situ preparation of FeOx nanoparticles embedded N-doped laser-induced graphene for flexible in-plane micro-supercapacitors</atitle><jtitle>Ionics</jtitle><stitle>Ionics</stitle><date>2023</date><risdate>2023</risdate><volume>29</volume><issue>1</issue><spage>419</spage><epage>427</epage><pages>419-427</pages><issn>0947-7047</issn><eissn>1862-0760</eissn><abstract>Laser direct writing of polyimide (PI) film to induce porous graphene as a flexible electrode facilitates the development of efficient, low-cost, and large-scale preparation of flexible planar micro-supercapacitors (MSCs). Nevertheless, current flexible MSCs based on laser-induced graphene (LIG) face bottlenecks such as poor LIG electrode wettability, inhomogeneous doping of heterogeneous components, and limited electrochemical performance. In view of this, a simple and effective process for in situ fabrication of flexible FeO
x
nanoparticles embedded N-doped LIG (FeO
x
@NLIG) electrode is developed by laser direct writing in this study. The as-assembled in-plane FeO
x
@NLIG MSCs exhibit an excellent areal specific capacitance of 13.82 mF cm
−2
, a remarkable energy density of 1.228 mW h cm
−2
at a high power density of 0.024 mW cm
−2
, good flexibility, and conspicuous cycling stability. Besides, these high-performance in-plane FeO
x
@NLIG MSCs as a vital micro-energy storage component can be easily miniaturized, modularized, and integrated to suit customized needs of wearable electronics due to great advantages in terms of identicality and stability of the as-fabricated FeO
x
@NLIG.
Graphical abstract</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s11581-022-04795-x</doi><tpages>9</tpages></addata></record> |
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subjects | Chemistry Chemistry and Materials Science Condensed Matter Physics Direct laser writing Electrochemical analysis Electrochemistry Electrodes Energy Storage Graphene Lasers Nanoparticles Optical and Electronic Materials Original Paper Renewable and Green Energy Stability Supercapacitors Wettability |
title | In situ preparation of FeOx nanoparticles embedded N-doped laser-induced graphene for flexible in-plane micro-supercapacitors |
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