Growth and Characterization of High-Quality Orthorhombic Phase CsPbBr3 Perovskite Single Crystals for Optoelectronic Applications
Caesium lead bromide (CsPbBr 3 ) has received a lot of interest as a model compound suitable for photovoltaics and many other optoelectronic applications. However, growing significant volumes of CsPbBr 3 single crystals is difficult. Herein, a facile room temperature crystal growth strategy is used...
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| Veröffentlicht in: | Journal of electronic materials 2023, Vol.52 (1), p.718-729 |
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| creator | Sujith, P. Pratheek, M. Parne, Saidi Reddy Predeep, P. |
| description | Caesium lead bromide (CsPbBr
3
) has received a lot of interest as a model compound suitable for photovoltaics and many other optoelectronic applications. However, growing significant volumes of CsPbBr
3
single crystals is difficult. Herein, a facile room temperature crystal growth strategy is used to generate high-quality and large single crystals of single-phase orthorhombic-CsPbBr
3
perovskite at room temperature. The optical, structural, and electrical properties of this crystal are also studied here. It has been found that the single crystals grown at room temperature show better thermal stability and complete sublimation without any decomposition leaving a clue that this material can be thermally deposited into thin films with ease. This significant aspect has also been successfully verified here by thermally depositing a fine and high-quality film of CsPbBr
3
using single-crystal powder as the source.
Graphical Abstract |
| doi_str_mv | 10.1007/s11664-022-10042-w |
| format | Article |
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3
) has received a lot of interest as a model compound suitable for photovoltaics and many other optoelectronic applications. However, growing significant volumes of CsPbBr
3
single crystals is difficult. Herein, a facile room temperature crystal growth strategy is used to generate high-quality and large single crystals of single-phase orthorhombic-CsPbBr
3
perovskite at room temperature. The optical, structural, and electrical properties of this crystal are also studied here. It has been found that the single crystals grown at room temperature show better thermal stability and complete sublimation without any decomposition leaving a clue that this material can be thermally deposited into thin films with ease. This significant aspect has also been successfully verified here by thermally depositing a fine and high-quality film of CsPbBr
3
using single-crystal powder as the source.
Graphical Abstract</description><identifier>ISSN: 0361-5235</identifier><identifier>EISSN: 1543-186X</identifier><identifier>DOI: 10.1007/s11664-022-10042-w</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Cesium ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Crystal growth ; Electrical properties ; Electronics and Microelectronics ; Instrumentation ; Materials Science ; Optical and Electronic Materials ; Optical properties ; Optoelectronics ; Original Research Article ; Orthorhombic phase ; Perovskites ; Photovoltaic cells ; Room temperature ; Single crystals ; Solid State Physics ; Solvents ; Sublimation ; Temperature ; Thermal stability ; Thin films</subject><ispartof>Journal of electronic materials, 2023, Vol.52 (1), p.718-729</ispartof><rights>The Minerals, Metals & Materials Society 2022. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c249t-75d74f9c3ed0a6c708315b30cc3b38150156309b1630f6b5e9335ce1409f4a493</citedby><cites>FETCH-LOGICAL-c249t-75d74f9c3ed0a6c708315b30cc3b38150156309b1630f6b5e9335ce1409f4a493</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11664-022-10042-w$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11664-022-10042-w$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27922,27923,41486,42555,51317</link.rule.ids></links><search><creatorcontrib>Sujith, P.</creatorcontrib><creatorcontrib>Pratheek, M.</creatorcontrib><creatorcontrib>Parne, Saidi Reddy</creatorcontrib><creatorcontrib>Predeep, P.</creatorcontrib><title>Growth and Characterization of High-Quality Orthorhombic Phase CsPbBr3 Perovskite Single Crystals for Optoelectronic Applications</title><title>Journal of electronic materials</title><addtitle>J. Electron. Mater</addtitle><description>Caesium lead bromide (CsPbBr
3
) has received a lot of interest as a model compound suitable for photovoltaics and many other optoelectronic applications. However, growing significant volumes of CsPbBr
3
single crystals is difficult. Herein, a facile room temperature crystal growth strategy is used to generate high-quality and large single crystals of single-phase orthorhombic-CsPbBr
3
perovskite at room temperature. The optical, structural, and electrical properties of this crystal are also studied here. It has been found that the single crystals grown at room temperature show better thermal stability and complete sublimation without any decomposition leaving a clue that this material can be thermally deposited into thin films with ease. This significant aspect has also been successfully verified here by thermally depositing a fine and high-quality film of CsPbBr
3
using single-crystal powder as the source.
Graphical Abstract</description><subject>Cesium</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Crystal growth</subject><subject>Electrical properties</subject><subject>Electronics and Microelectronics</subject><subject>Instrumentation</subject><subject>Materials Science</subject><subject>Optical and Electronic Materials</subject><subject>Optical properties</subject><subject>Optoelectronics</subject><subject>Original Research Article</subject><subject>Orthorhombic phase</subject><subject>Perovskites</subject><subject>Photovoltaic cells</subject><subject>Room temperature</subject><subject>Single crystals</subject><subject>Solid State Physics</subject><subject>Solvents</subject><subject>Sublimation</subject><subject>Temperature</subject><subject>Thermal stability</subject><subject>Thin films</subject><issn>0361-5235</issn><issn>1543-186X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><sourceid>8G5</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><sourceid>GUQSH</sourceid><sourceid>M2O</sourceid><recordid>eNp9kE1LAzEQhoMoWD_-gKeA52iySfbjWItfILSigreQTbPd1HWzTlJLvfnPjVbw5mWGYd5nXuZF6ITRM0ZpcR4Yy3NBaJaRNIuMrHfQiEnBCSvz5100ojxnRGZc7qODEJaUMslKNkKf1-DXscW6n-NJq0GbaMF96Oh8j32Db9yiJfcr3bm4wVOIrYfWv9bO4Fmrg8WTMKsvgOOZBf8eXly0-MH1iy5tYBOi7gJuPODpEL3trIng-8SOh6Fz5sckHKG9Jsns8W8_RE9Xl4-TG3I3vb6djO-IyUQVSSHnhWgqw-2c6twUtORM1pwaw2teMpkeyjmtapZqk9fSVpxLY5mgVSO0qPghOt3eHcC_rWyIaulX0CdLlRWiYJzSskyqbKsy4EMA26gB3KuGjWJUfUettlGrFLX6iVqtE8S3UEjifmHh7_Q_1BfUP4M0</recordid><startdate>2023</startdate><enddate>2023</enddate><creator>Sujith, P.</creator><creator>Pratheek, M.</creator><creator>Parne, Saidi Reddy</creator><creator>Predeep, P.</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7XB</scope><scope>88I</scope><scope>8AF</scope><scope>8AO</scope><scope>8FE</scope><scope>8FG</scope><scope>8FK</scope><scope>8G5</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>GNUQQ</scope><scope>GUQSH</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>L6V</scope><scope>M2O</scope><scope>M2P</scope><scope>M7S</scope><scope>MBDVC</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>PTHSS</scope><scope>Q9U</scope><scope>S0X</scope></search><sort><creationdate>2023</creationdate><title>Growth and Characterization of High-Quality Orthorhombic Phase CsPbBr3 Perovskite Single Crystals for Optoelectronic Applications</title><author>Sujith, P. ; Pratheek, M. ; Parne, Saidi Reddy ; Predeep, P.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c249t-75d74f9c3ed0a6c708315b30cc3b38150156309b1630f6b5e9335ce1409f4a493</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Cesium</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Crystal growth</topic><topic>Electrical properties</topic><topic>Electronics and Microelectronics</topic><topic>Instrumentation</topic><topic>Materials Science</topic><topic>Optical and Electronic Materials</topic><topic>Optical properties</topic><topic>Optoelectronics</topic><topic>Original Research Article</topic><topic>Orthorhombic phase</topic><topic>Perovskites</topic><topic>Photovoltaic cells</topic><topic>Room temperature</topic><topic>Single crystals</topic><topic>Solid State Physics</topic><topic>Solvents</topic><topic>Sublimation</topic><topic>Temperature</topic><topic>Thermal stability</topic><topic>Thin films</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Sujith, P.</creatorcontrib><creatorcontrib>Pratheek, M.</creatorcontrib><creatorcontrib>Parne, Saidi Reddy</creatorcontrib><creatorcontrib>Predeep, P.</creatorcontrib><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Science Database (Alumni Edition)</collection><collection>STEM Database</collection><collection>ProQuest Pharma Collection</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>Research Library (Alumni Edition)</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ProQuest Central Student</collection><collection>Research Library Prep</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>ProQuest Engineering Collection</collection><collection>Research Library</collection><collection>Science Database</collection><collection>Engineering Database</collection><collection>Research Library (Corporate)</collection><collection>Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>Engineering Collection</collection><collection>ProQuest Central Basic</collection><collection>SIRS Editorial</collection><jtitle>Journal of electronic materials</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Sujith, P.</au><au>Pratheek, M.</au><au>Parne, Saidi Reddy</au><au>Predeep, P.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Growth and Characterization of High-Quality Orthorhombic Phase CsPbBr3 Perovskite Single Crystals for Optoelectronic Applications</atitle><jtitle>Journal of electronic materials</jtitle><stitle>J. Electron. Mater</stitle><date>2023</date><risdate>2023</risdate><volume>52</volume><issue>1</issue><spage>718</spage><epage>729</epage><pages>718-729</pages><issn>0361-5235</issn><eissn>1543-186X</eissn><abstract>Caesium lead bromide (CsPbBr
3
) has received a lot of interest as a model compound suitable for photovoltaics and many other optoelectronic applications. However, growing significant volumes of CsPbBr
3
single crystals is difficult. Herein, a facile room temperature crystal growth strategy is used to generate high-quality and large single crystals of single-phase orthorhombic-CsPbBr
3
perovskite at room temperature. The optical, structural, and electrical properties of this crystal are also studied here. It has been found that the single crystals grown at room temperature show better thermal stability and complete sublimation without any decomposition leaving a clue that this material can be thermally deposited into thin films with ease. This significant aspect has also been successfully verified here by thermally depositing a fine and high-quality film of CsPbBr
3
using single-crystal powder as the source.
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| subjects | Cesium Characterization and Evaluation of Materials Chemistry and Materials Science Crystal growth Electrical properties Electronics and Microelectronics Instrumentation Materials Science Optical and Electronic Materials Optical properties Optoelectronics Original Research Article Orthorhombic phase Perovskites Photovoltaic cells Room temperature Single crystals Solid State Physics Solvents Sublimation Temperature Thermal stability Thin films |
| title | Growth and Characterization of High-Quality Orthorhombic Phase CsPbBr3 Perovskite Single Crystals for Optoelectronic Applications |
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