Ultrafast x-ray scattering reveals composite amplitude collective mode in the Weyl charge density wave material (TaSe\(_4\))\(_2\)I

We report ultrafast x-ray scattering experiments of the quasi-1D charge density wave (CDW) material (TaSe\(_4\))\(_2\)I following photoexcitation with femtosecond infrared laser pulses. From the time-dependent diffraction signal at the CDW sidebands we identify an amplitude mode derived primarily fr...

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Hauptverfasser: Nguyen, Quynh L, Duncan, Ryan A, Orenstein, Gal, Huang, Yijing, Krapivin, Viktor, de la Pena, Gilberto, Ornelas-Skarin, Chance, Reis, David A, Abbamonte, Peter, Bettler, Simon, Chollet, Matthieu, Hoffmann, Matthias C, Hurley, Matthew, Kim, Soyeun, Kirchmann, Patrick S, Kubota, Yuya, Mahmood, Fahad, Miller, Alexander, Osaka, Taito, Qu, Kejian, Sato, Takahiro, Shoemaker, Daniel P, Sirica, Nicholas, Song, Sanghoon, Stanton, Jade, Teitelbaum, Samuel W, Tilton, Sean E, Togashi, Tadashi, Zhu, Diling, Trigo, Mariano
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container_title arXiv.org
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creator Nguyen, Quynh L
Duncan, Ryan A
Orenstein, Gal
Huang, Yijing
Krapivin, Viktor
de la Pena, Gilberto
Ornelas-Skarin, Chance
Reis, David A
Abbamonte, Peter
Bettler, Simon
Chollet, Matthieu
Hoffmann, Matthias C
Hurley, Matthew
Kim, Soyeun
Kirchmann, Patrick S
Kubota, Yuya
Mahmood, Fahad
Miller, Alexander
Osaka, Taito
Qu, Kejian
Sato, Takahiro
Shoemaker, Daniel P
Sirica, Nicholas
Song, Sanghoon
Stanton, Jade
Teitelbaum, Samuel W
Tilton, Sean E
Togashi, Tadashi
Zhu, Diling
Trigo, Mariano
description We report ultrafast x-ray scattering experiments of the quasi-1D charge density wave (CDW) material (TaSe\(_4\))\(_2\)I following photoexcitation with femtosecond infrared laser pulses. From the time-dependent diffraction signal at the CDW sidebands we identify an amplitude mode derived primarily from the transverse acoustic component of the CDW static distortion. The dynamics of this acoustic amplitude mode are described well by a model of a displacive excitation, which we interpret as mediated through a coupling to the optical phonon component associated with the tetramerization of the Ta chains.
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From the time-dependent diffraction signal at the CDW sidebands we identify an amplitude mode derived primarily from the transverse acoustic component of the CDW static distortion. The dynamics of this acoustic amplitude mode are described well by a model of a displacive excitation, which we interpret as mediated through a coupling to the optical phonon component associated with the tetramerization of the Ta chains.</abstract><cop>Ithaca</cop><pub>Cornell University Library, arXiv.org</pub><oa>free_for_read</oa></addata></record>
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subjects Acoustic waves
Acoustics
Amplitudes
Charge density waves
Charge materials
Displacement
Femtosecond pulses
Free electron lasers
Infrared lasers
Photoexcitation
Sidebands
Tantalum
Terahertz frequencies
X-ray scattering
title Ultrafast x-ray scattering reveals composite amplitude collective mode in the Weyl charge density wave material (TaSe\(_4\))\(_2\)I
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